Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles

Thermogravimetric analysis (TGA) was performed on six samples of pine wood, poplar sawdust and olive residue, and the kinetic parameters were evaluated by using isoconversional models. The hemicellulose, cellulose and lignin contents were also estimated using the Fraser–Suzuki deconvolution method....

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Main Authors: Roberto Paredes, Blanca Castells, Alberto Tascón
Format: Article
Language:English
Published: MDPI AG 2024-10-01
Series:Fire
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Online Access:https://www.mdpi.com/2571-6255/7/11/396
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author Roberto Paredes
Blanca Castells
Alberto Tascón
author_facet Roberto Paredes
Blanca Castells
Alberto Tascón
author_sort Roberto Paredes
collection DOAJ
description Thermogravimetric analysis (TGA) was performed on six samples of pine wood, poplar sawdust and olive residue, and the kinetic parameters were evaluated by using isoconversional models. The hemicellulose, cellulose and lignin contents were also estimated using the Fraser–Suzuki deconvolution method. In addition, a range of thermodynamic parameters and combustion indices was calculated. Significant correlations were found between the kinetic, thermodynamic and combustion parameters. The ignition index showed an inverse relationship with the activation energy, whereas the burnout index correlated with enthalpy values for most samples. Higher heating rates during TGA increased ignition and combustion efficiencies but decreased combustion stability. Differences in behaviour were detected between the olive residues, which had a much higher lignin content (51.2–56.9%), and the woody biomass samples (24.2–29.2%). Moreover, the sample with the highest ash content also exhibited some distinctive characteristics, including the lowest high heating value and ignition index, coupled with the highest activation energy, indicating a less favourable combustion behaviour than the other samples. The particle size of the samples was also found to be critical for both combustion efficiency and safety.
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spelling doaj-art-31b6bedf28e54976bc830e0fbe805dc02025-08-20T02:28:09ZengMDPI AGFire2571-62552024-10-0171139610.3390/fire7110396Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion ProfilesRoberto Paredes0Blanca Castells1Alberto Tascón2Department of Geological and Mining Engineering, E.T.S. Ingenieros de Minas y Energía, Universidad Politécnica de Madrid, C/Ríos Rosas 21, 28003 Madrid, SpainDepartment of Energy and Fuels, E.T.S. Ingenieros de Minas y Energía, Universidad Politécnica de Madrid, C/Ríos Rosas 21, 28003 Madrid, SpainDepartment of Agriculture and Food Science, Universidad de La Rioja, C/Madre de Dios 53, 26006 Logroño, SpainThermogravimetric analysis (TGA) was performed on six samples of pine wood, poplar sawdust and olive residue, and the kinetic parameters were evaluated by using isoconversional models. The hemicellulose, cellulose and lignin contents were also estimated using the Fraser–Suzuki deconvolution method. In addition, a range of thermodynamic parameters and combustion indices was calculated. Significant correlations were found between the kinetic, thermodynamic and combustion parameters. The ignition index showed an inverse relationship with the activation energy, whereas the burnout index correlated with enthalpy values for most samples. Higher heating rates during TGA increased ignition and combustion efficiencies but decreased combustion stability. Differences in behaviour were detected between the olive residues, which had a much higher lignin content (51.2–56.9%), and the woody biomass samples (24.2–29.2%). Moreover, the sample with the highest ash content also exhibited some distinctive characteristics, including the lowest high heating value and ignition index, coupled with the highest activation energy, indicating a less favourable combustion behaviour than the other samples. The particle size of the samples was also found to be critical for both combustion efficiency and safety.https://www.mdpi.com/2571-6255/7/11/396biomasssolid biofuelsthermogravimetric analysiscombustion kineticsentropyenthalpy
spellingShingle Roberto Paredes
Blanca Castells
Alberto Tascón
Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles
Fire
biomass
solid biofuels
thermogravimetric analysis
combustion kinetics
entropy
enthalpy
title Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles
title_full Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles
title_fullStr Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles
title_full_unstemmed Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles
title_short Thermogravimetric Assessment of Biomass: Unravelling Kinetic, Chemical Composition and Combustion Profiles
title_sort thermogravimetric assessment of biomass unravelling kinetic chemical composition and combustion profiles
topic biomass
solid biofuels
thermogravimetric analysis
combustion kinetics
entropy
enthalpy
url https://www.mdpi.com/2571-6255/7/11/396
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AT blancacastells thermogravimetricassessmentofbiomassunravellingkineticchemicalcompositionandcombustionprofiles
AT albertotascon thermogravimetricassessmentofbiomassunravellingkineticchemicalcompositionandcombustionprofiles