Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films

Titanium nitride (TiN) is a typical inorganic compound capable of achieving resistance modulation by adjusting the element ratio. In this work, to deeply investigate the resistance-tunable characteristics and electron emission properties of TiN, we prepared 10 sets of TiN films by adjusting the magn...

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Main Authors: Yang Xia, Dan Wang
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Inorganics
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Online Access:https://www.mdpi.com/2304-6740/13/6/201
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author Yang Xia
Dan Wang
author_facet Yang Xia
Dan Wang
author_sort Yang Xia
collection DOAJ
description Titanium nitride (TiN) is a typical inorganic compound capable of achieving resistance modulation by adjusting the element ratio. In this work, to deeply investigate the resistance-tunable characteristics and electron emission properties of TiN, we prepared 10 sets of TiN films by adjusting the magnetron sputtering parameters. The microscopic analyses show that the film thicknesses ranged from about 355 to 459 nm. Moreover, with the process parameters used in this work, TiN nanostructures are formed more easily when the nitrogen flow rate is ≤5 sccm, and compact TiN films are formed more easily when the nitrogen flow rate is ≥10 sccm. Elemental analyses showed that the N:Ti atomic ratios of the TiN films ranged from about 0.587 to 1.40. The results of surface analysis showed the presence of a certain amount of oxygen on the surface of the TiN film, indicating that the surface TiN may exist in the form of TiN:O. The electrical resistance test showed that the resistivity of the TiN coating ranges from 1.59 × 10<sup>−4</sup> to 1.83 × 10<sup>−1</sup> Ω·m. And the closer the N:Ti atomic ratio is to one, the lower the TiN film resistivity is. The electron emission coefficient (EEC) results show that among the film samples from #3 to #10, sample #8 has the lowest EEC, with a peak EEC of only 1.61. By comparing the resistivity and EEC data, a novel phenomenon was discovered: a decrease in the resistivity of TiN films leads to a decrease in their EEC values. The results show that the resistivity and EEC of TiN films can be adjusted according to the film-forming components, which is important for the application of TiN in the electronics industry.
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spelling doaj-art-30afc1597e7c4e5788321ea193fc85e52025-08-20T03:27:14ZengMDPI AGInorganics2304-67402025-06-0113620110.3390/inorganics13060201Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride FilmsYang Xia0Dan Wang1School of Intelligent Manufacturing, Chongqing Technology and Businesses Institute, Chongqing 401520, ChinaSchool of Microelectronics, Xi’an Jiaotong University, Xi’an 710049, ChinaTitanium nitride (TiN) is a typical inorganic compound capable of achieving resistance modulation by adjusting the element ratio. In this work, to deeply investigate the resistance-tunable characteristics and electron emission properties of TiN, we prepared 10 sets of TiN films by adjusting the magnetron sputtering parameters. The microscopic analyses show that the film thicknesses ranged from about 355 to 459 nm. Moreover, with the process parameters used in this work, TiN nanostructures are formed more easily when the nitrogen flow rate is ≤5 sccm, and compact TiN films are formed more easily when the nitrogen flow rate is ≥10 sccm. Elemental analyses showed that the N:Ti atomic ratios of the TiN films ranged from about 0.587 to 1.40. The results of surface analysis showed the presence of a certain amount of oxygen on the surface of the TiN film, indicating that the surface TiN may exist in the form of TiN:O. The electrical resistance test showed that the resistivity of the TiN coating ranges from 1.59 × 10<sup>−4</sup> to 1.83 × 10<sup>−1</sup> Ω·m. And the closer the N:Ti atomic ratio is to one, the lower the TiN film resistivity is. The electron emission coefficient (EEC) results show that among the film samples from #3 to #10, sample #8 has the lowest EEC, with a peak EEC of only 1.61. By comparing the resistivity and EEC data, a novel phenomenon was discovered: a decrease in the resistivity of TiN films leads to a decrease in their EEC values. The results show that the resistivity and EEC of TiN films can be adjusted according to the film-forming components, which is important for the application of TiN in the electronics industry.https://www.mdpi.com/2304-6740/13/6/201titanium nitrideatomic ratioelectrical resistivityelectron emission
spellingShingle Yang Xia
Dan Wang
Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films
Inorganics
titanium nitride
atomic ratio
electrical resistivity
electron emission
title Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films
title_full Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films
title_fullStr Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films
title_full_unstemmed Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films
title_short Effect of Sputtering Process Parameters on Physical Properties and Electron Emission Level of Titanium Nitride Films
title_sort effect of sputtering process parameters on physical properties and electron emission level of titanium nitride films
topic titanium nitride
atomic ratio
electrical resistivity
electron emission
url https://www.mdpi.com/2304-6740/13/6/201
work_keys_str_mv AT yangxia effectofsputteringprocessparametersonphysicalpropertiesandelectronemissionleveloftitaniumnitridefilms
AT danwang effectofsputteringprocessparametersonphysicalpropertiesandelectronemissionleveloftitaniumnitridefilms