Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling

Abstract Effective heat dissipation remains a grand challenge for energy-dense devices and systems. As heterogeneous integration becomes increasingly inevitable in electronics, thermal resistance at interfaces has emerged as a critical bottleneck for thermal management. However, existing thermal int...

Full description

Saved in:
Bibliographic Details
Main Authors: Rui Cheng, Qixian Wang, Zexiao Wang, Lin Jing, Ana V. Garcia-Caraveo, Zhuo Li, Yibai Zhong, Xiu Liu, Xiao Luo, Tianyi Huang, Hyeong Seok Yun, Hakan Salihoglu, Loren Russell, Navid Kazem, Tianyi Chen, Sheng Shen
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-56163-8
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1832594539831885824
author Rui Cheng
Qixian Wang
Zexiao Wang
Lin Jing
Ana V. Garcia-Caraveo
Zhuo Li
Yibai Zhong
Xiu Liu
Xiao Luo
Tianyi Huang
Hyeong Seok Yun
Hakan Salihoglu
Loren Russell
Navid Kazem
Tianyi Chen
Sheng Shen
author_facet Rui Cheng
Qixian Wang
Zexiao Wang
Lin Jing
Ana V. Garcia-Caraveo
Zhuo Li
Yibai Zhong
Xiu Liu
Xiao Luo
Tianyi Huang
Hyeong Seok Yun
Hakan Salihoglu
Loren Russell
Navid Kazem
Tianyi Chen
Sheng Shen
author_sort Rui Cheng
collection DOAJ
description Abstract Effective heat dissipation remains a grand challenge for energy-dense devices and systems. As heterogeneous integration becomes increasingly inevitable in electronics, thermal resistance at interfaces has emerged as a critical bottleneck for thermal management. However, existing thermal interface solutions are constrained by either high thermal resistance or poor reliability. We report a strategy to create printable, high-performance liquid-infused nanostructured composites, comprising a mechanically soft and thermally conductive double-sided Cu nanowire array scaffold infused with a customized thermal-bridge liquid that suppresses contact thermal resistance. The liquid infusion concept is versatile for a broad range of thermal interface applications. Remarkably, the liquid metal infused nanostructured composite exhibits an ultra-low thermal resistance <1 mm² K W-1 at interface, outperforming state-of-the-art thermal interface materials on chip-cooling. The high reliability of the nanostructured composites enables undegraded performance through extreme temperature cycling. We envision liquid-infused nanostructured composites as a universal thermal interface solution for cooling applications in data centers, GPU/CPU systems, solid-state lasers, and LEDs.
format Article
id doaj-art-2fecd5193da8477381701d554e3c280c
institution Kabale University
issn 2041-1723
language English
publishDate 2025-01-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-2fecd5193da8477381701d554e3c280c2025-01-19T12:32:18ZengNature PortfolioNature Communications2041-17232025-01-011611810.1038/s41467-025-56163-8Liquid-infused nanostructured composite as a high-performance thermal interface material for effective coolingRui Cheng0Qixian Wang1Zexiao Wang2Lin Jing3Ana V. Garcia-Caraveo4Zhuo Li5Yibai Zhong6Xiu Liu7Xiao Luo8Tianyi Huang9Hyeong Seok Yun10Hakan Salihoglu11Loren Russell12Navid Kazem13Tianyi Chen14Sheng Shen15Department of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveCollege of Engineering, Oregon State University, 1791 SW Campus WayDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveArieca, Inc., 201 N Braddock Ave STE 334Arieca, Inc., 201 N Braddock Ave STE 334College of Engineering, Oregon State University, 1791 SW Campus WayDepartment of Mechanical Engineering, Carnegie Mellon University, 5000 Forbes AveAbstract Effective heat dissipation remains a grand challenge for energy-dense devices and systems. As heterogeneous integration becomes increasingly inevitable in electronics, thermal resistance at interfaces has emerged as a critical bottleneck for thermal management. However, existing thermal interface solutions are constrained by either high thermal resistance or poor reliability. We report a strategy to create printable, high-performance liquid-infused nanostructured composites, comprising a mechanically soft and thermally conductive double-sided Cu nanowire array scaffold infused with a customized thermal-bridge liquid that suppresses contact thermal resistance. The liquid infusion concept is versatile for a broad range of thermal interface applications. Remarkably, the liquid metal infused nanostructured composite exhibits an ultra-low thermal resistance <1 mm² K W-1 at interface, outperforming state-of-the-art thermal interface materials on chip-cooling. The high reliability of the nanostructured composites enables undegraded performance through extreme temperature cycling. We envision liquid-infused nanostructured composites as a universal thermal interface solution for cooling applications in data centers, GPU/CPU systems, solid-state lasers, and LEDs.https://doi.org/10.1038/s41467-025-56163-8
spellingShingle Rui Cheng
Qixian Wang
Zexiao Wang
Lin Jing
Ana V. Garcia-Caraveo
Zhuo Li
Yibai Zhong
Xiu Liu
Xiao Luo
Tianyi Huang
Hyeong Seok Yun
Hakan Salihoglu
Loren Russell
Navid Kazem
Tianyi Chen
Sheng Shen
Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling
Nature Communications
title Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling
title_full Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling
title_fullStr Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling
title_full_unstemmed Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling
title_short Liquid-infused nanostructured composite as a high-performance thermal interface material for effective cooling
title_sort liquid infused nanostructured composite as a high performance thermal interface material for effective cooling
url https://doi.org/10.1038/s41467-025-56163-8
work_keys_str_mv AT ruicheng liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT qixianwang liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT zexiaowang liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT linjing liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT anavgarciacaraveo liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT zhuoli liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT yibaizhong liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT xiuliu liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT xiaoluo liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT tianyihuang liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT hyeongseokyun liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT hakansalihoglu liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT lorenrussell liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT navidkazem liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT tianyichen liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling
AT shengshen liquidinfusednanostructuredcompositeasahighperformancethermalinterfacematerialforeffectivecooling