Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors

Composite-based temperature sensors utilizing the negative temperature coefficient (NTC) effect have gained significant attention across various fields, particularly in healthcare. However, the development of innovative, highly linear, and high-performance NTC-based temperature sensors remains a cha...

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Main Authors: Yeongu Choi, Minhyeok Kim, Hongyun So
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Polymer Testing
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Online Access:http://www.sciencedirect.com/science/article/pii/S0142941824003295
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author Yeongu Choi
Minhyeok Kim
Hongyun So
author_facet Yeongu Choi
Minhyeok Kim
Hongyun So
author_sort Yeongu Choi
collection DOAJ
description Composite-based temperature sensors utilizing the negative temperature coefficient (NTC) effect have gained significant attention across various fields, particularly in healthcare. However, the development of innovative, highly linear, and high-performance NTC-based temperature sensors remains a challenge. In this study, we developed a composite temperature sensor comprising thermoplastic polyurethane (TPU), single-walled carbon nanotubes (SWCNTs), and poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS). A series of performance tests demonstrated that the TPU/SWCNT/PEDOT:PSS (TSP) composite effectively monitors temperature variations with both linearity and superior performance, attributed to the synergistic NTC effects of SWCNTs and PEDOT:PSS. This flexible temperature sensor retained its sensing functionality after repeated cycles of temperature fluctuations and multiple bending tests. Moreover, due to the unique properties of CNTs, the TSP sensor exhibited photothermal responses, showing highly sensitive resistance changes upon exposure to infrared radiation. The TSP sensor proved to be effective for various practical applications, including biosignal monitoring through thermal detection, temperature tracking during phone charging, and accurate temperature sensing on curved surfaces. Additionally, non-contact heat detection can be reliably performed regardless of whether tensile stress is applied. These findings underscore the immense potential of TSP sensors for future use in wearable healthcare technologies.
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spelling doaj-art-2f52cbe0ee4c49e0972030efd3ef23aa2025-08-20T02:35:37ZengElsevierPolymer Testing1873-23482024-12-0114110865210.1016/j.polymertesting.2024.108652Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensorsYeongu Choi0Minhyeok Kim1Hongyun So2Department of Mechanical Engineering, Hanyang University, Seoul, 04763, South KoreaDepartment of Mechanical Engineering, Hanyang University, Seoul, 04763, South KoreaCorresponding author.; Department of Mechanical Engineering, Hanyang University, Seoul, 04763, South KoreaComposite-based temperature sensors utilizing the negative temperature coefficient (NTC) effect have gained significant attention across various fields, particularly in healthcare. However, the development of innovative, highly linear, and high-performance NTC-based temperature sensors remains a challenge. In this study, we developed a composite temperature sensor comprising thermoplastic polyurethane (TPU), single-walled carbon nanotubes (SWCNTs), and poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS). A series of performance tests demonstrated that the TPU/SWCNT/PEDOT:PSS (TSP) composite effectively monitors temperature variations with both linearity and superior performance, attributed to the synergistic NTC effects of SWCNTs and PEDOT:PSS. This flexible temperature sensor retained its sensing functionality after repeated cycles of temperature fluctuations and multiple bending tests. Moreover, due to the unique properties of CNTs, the TSP sensor exhibited photothermal responses, showing highly sensitive resistance changes upon exposure to infrared radiation. The TSP sensor proved to be effective for various practical applications, including biosignal monitoring through thermal detection, temperature tracking during phone charging, and accurate temperature sensing on curved surfaces. Additionally, non-contact heat detection can be reliably performed regardless of whether tensile stress is applied. These findings underscore the immense potential of TSP sensors for future use in wearable healthcare technologies.http://www.sciencedirect.com/science/article/pii/S0142941824003295Negative temperature coefficientSWCNTPEDOT:PSSPhotothermal effectFlexible and wearable sensor
spellingShingle Yeongu Choi
Minhyeok Kim
Hongyun So
Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors
Polymer Testing
Negative temperature coefficient
SWCNT
PEDOT:PSS
Photothermal effect
Flexible and wearable sensor
title Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors
title_full Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors
title_fullStr Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors
title_full_unstemmed Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors
title_short Negative temperature coefficient effect of TPU/SWCNT/PEDOT:PSS polymer matrices for wearable temperature sensors
title_sort negative temperature coefficient effect of tpu swcnt pedot pss polymer matrices for wearable temperature sensors
topic Negative temperature coefficient
SWCNT
PEDOT:PSS
Photothermal effect
Flexible and wearable sensor
url http://www.sciencedirect.com/science/article/pii/S0142941824003295
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AT minhyeokkim negativetemperaturecoefficienteffectoftpuswcntpedotpsspolymermatricesforwearabletemperaturesensors
AT hongyunso negativetemperaturecoefficienteffectoftpuswcntpedotpsspolymermatricesforwearabletemperaturesensors