Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level

Abstract The growing demand for detection and sensing in the biomedical field is placing higher demands on technology. In clinical testing, it is expected to be able to realize both rapid large‐field imaging and analysis of single particles (or single molecules or single cells), and it is expected t...

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Main Authors: Yang Shi, Lixiang Wang, Lingling Li, Chen Feng, Yue Cao
Format: Article
Language:English
Published: Wiley-VCH 2025-03-01
Series:ChemistryOpen
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Online Access:https://doi.org/10.1002/open.202400017
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author Yang Shi
Lixiang Wang
Lingling Li
Chen Feng
Yue Cao
author_facet Yang Shi
Lixiang Wang
Lingling Li
Chen Feng
Yue Cao
author_sort Yang Shi
collection DOAJ
description Abstract The growing demand for detection and sensing in the biomedical field is placing higher demands on technology. In clinical testing, it is expected to be able to realize both rapid large‐field imaging and analysis of single particles (or single molecules or single cells), and it is expected to be able to grasp both the unique individuality of single particles in time and space during the complex reaction process, as well as the regular correlation between single particles in the same population distribution. Supported and promoted by the theory of localized surface plasmon resonance (LSPR), dark‐field microscopy, as a single‐particle optical imaging technique with a very high signal‐to‐noise ratio, provides a powerful new means to address the above clinical detection needs. This review will focus on the innovative applications of dark‐field microscopy in biomedical‐related assays in the past five years, introducing the basic principles and listing the impressing works. We also summarize how dark‐field microscopy has been combined with other techniques, including surface‐enhanced Raman scattering, fluorescence, colorimetry, electrochemistry, etc., to witness the joint progress and promotion of detection methods in the future. It also provides an outlook on the current challenges and future trends in this field.
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institution Kabale University
issn 2191-1363
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spelling doaj-art-2d4f71534de04bb49b43285d168ea3882025-08-20T03:49:22ZengWiley-VCHChemistryOpen2191-13632025-03-01143n/an/a10.1002/open.202400017Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle LevelYang Shi0Lixiang Wang1Lingling Li2Chen Feng3Yue Cao4Department of Forensic Medicine Nanjing Medical University Nanjing 211166 PR ChinaDepartment of Forensic Medicine Nanjing Medical University Nanjing 211166 PR ChinaSchool of Pharmacy Nanjing Medical University Nanjing 211166 PR ChinaDepartment of Forensic Medicine Nanjing Medical University Nanjing 211166 PR ChinaDepartment of Forensic Medicine Nanjing Medical University Nanjing 211166 PR ChinaAbstract The growing demand for detection and sensing in the biomedical field is placing higher demands on technology. In clinical testing, it is expected to be able to realize both rapid large‐field imaging and analysis of single particles (or single molecules or single cells), and it is expected to be able to grasp both the unique individuality of single particles in time and space during the complex reaction process, as well as the regular correlation between single particles in the same population distribution. Supported and promoted by the theory of localized surface plasmon resonance (LSPR), dark‐field microscopy, as a single‐particle optical imaging technique with a very high signal‐to‐noise ratio, provides a powerful new means to address the above clinical detection needs. This review will focus on the innovative applications of dark‐field microscopy in biomedical‐related assays in the past five years, introducing the basic principles and listing the impressing works. We also summarize how dark‐field microscopy has been combined with other techniques, including surface‐enhanced Raman scattering, fluorescence, colorimetry, electrochemistry, etc., to witness the joint progress and promotion of detection methods in the future. It also provides an outlook on the current challenges and future trends in this field.https://doi.org/10.1002/open.202400017Dark-field microscopyScattering imagingSingle particleLocalized surface plasmon resonanceBioassay
spellingShingle Yang Shi
Lixiang Wang
Lingling Li
Chen Feng
Yue Cao
Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level
ChemistryOpen
Dark-field microscopy
Scattering imaging
Single particle
Localized surface plasmon resonance
Bioassay
title Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level
title_full Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level
title_fullStr Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level
title_full_unstemmed Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level
title_short Innovative Progress of LSPR‐Based Dark‐Field Scattering Spectral Imaging in the Biomedical Assay at the Single‐Particle Level
title_sort innovative progress of lspr based dark field scattering spectral imaging in the biomedical assay at the single particle level
topic Dark-field microscopy
Scattering imaging
Single particle
Localized surface plasmon resonance
Bioassay
url https://doi.org/10.1002/open.202400017
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AT lixiangwang innovativeprogressoflsprbaseddarkfieldscatteringspectralimaginginthebiomedicalassayatthesingleparticlelevel
AT linglingli innovativeprogressoflsprbaseddarkfieldscatteringspectralimaginginthebiomedicalassayatthesingleparticlelevel
AT chenfeng innovativeprogressoflsprbaseddarkfieldscatteringspectralimaginginthebiomedicalassayatthesingleparticlelevel
AT yuecao innovativeprogressoflsprbaseddarkfieldscatteringspectralimaginginthebiomedicalassayatthesingleparticlelevel