Spin detector for panchromatic circularly polarized light detection
Abstract Circularly polarized light (CPL) detection is crucial for optical communication, bioimaging and quantum computing. However, CPL detectors based on chiral low-dimensional perovskites face a trade-off between optoelectronic performance and CPL discrimination, and typically exhibit a CPL respo...
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| Main Authors: | , , , , |
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| Format: | Article |
| Language: | English |
| Published: |
Nature Portfolio
2025-05-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-025-59287-z |
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| Summary: | Abstract Circularly polarized light (CPL) detection is crucial for optical communication, bioimaging and quantum computing. However, CPL detectors based on chiral low-dimensional perovskites face a trade-off between optoelectronic performance and CPL discrimination, and typically exhibit a CPL response within a narrow spectral range. Here, we overcome these limitations by integrating three-dimensional (3D) and chiral-two-dimensional (2D) perovskites. The 3D perovskite serving as the photoabsorption layer extends the detection range to 760 nm and enhances optoelectronic responses, while also generating spin-polarized carriers through large Rashba splitting. The chiral-2D perovskite achieves spin filtering efficiency up to 80%. The synergy between spin polarization and chiral-induced spin selectivity processes enables a panchromatic CPL response, with a photocurrent asymmetry factor exceeding 0.28 across the visible spectrum and peaking at 0.35. Furthermore, our detector achieves a detectivity of 3.7×1011 Jones. Our work introduces a spin manipulation strategy for panchromatic CPL detection, expanding the scope of spintronics applications. |
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| ISSN: | 2041-1723 |