Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system

A polymer brush system of a neutral polymer poly (ethylene glycol) with a molecular weight of Mw = 20 kDa on silicon substrates in an aqueous medium was studied by the specular neutron reflectometry. Structural changes in the density profile of a polymer brush caused by the interaction of polymer ch...

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Main Authors: O. P. Artykulnyi, M. M. Avdeev, Ye. M. Kosiachkin, V. I. Petrenko, I. Safarik, L. A. Bulavin
Format: Article
Language:English
Published: Institute for Nuclear Research, National Academy of Sciences of Ukraine 2021-06-01
Series:Ядерна фізика та енергетика
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Online Access:http://jnpae.kinr.kiev.ua/22.2/Articles_PDF/jnpae-2021-22-0149-Artykulnyi.pdf
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author O. P. Artykulnyi
M. M. Avdeev
Ye. M. Kosiachkin
V. I. Petrenko
I. Safarik
L. A. Bulavin
author_facet O. P. Artykulnyi
M. M. Avdeev
Ye. M. Kosiachkin
V. I. Petrenko
I. Safarik
L. A. Bulavin
author_sort O. P. Artykulnyi
collection DOAJ
description A polymer brush system of a neutral polymer poly (ethylene glycol) with a molecular weight of Mw = 20 kDa on silicon substrates in an aqueous medium was studied by the specular neutron reflectometry. Structural changes in the density profile of a polymer brush caused by the interaction of polymer chains with micelles of the anionic surfactant dodecylbenzenesulfonate acid were observed. The effect is shown to be related to the formation of molecular polymer-micelle associates in the bulk of the solution, which was previously studied by small-angle neutron scattering in a wide range of surfactant concentrations at various molecular weights of the polymer. The density of the dry polymer layer on the silicon substrate was additionally characterized by X-ray reflectometry and scanning atomic force microscopy.
format Article
id doaj-art-2b8a00764e374be5bab8dfd9c38644fa
institution DOAJ
issn 1818-331X
2074-0565
language English
publishDate 2021-06-01
publisher Institute for Nuclear Research, National Academy of Sciences of Ukraine
record_format Article
series Ядерна фізика та енергетика
spelling doaj-art-2b8a00764e374be5bab8dfd9c38644fa2025-08-20T03:17:52ZengInstitute for Nuclear Research, National Academy of Sciences of UkraineЯдерна фізика та енергетика1818-331X2074-05652021-06-01222149156https://doi.org/10.15407/jnpae2021.02.149Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush systemO. P. Artykulnyi0M. M. Avdeev1Ye. M. Kosiachkin2V. I. Petrenko3I. Safarik4L. A. Bulavin5Taras Shevchenko National University of Kyiv, Kyiv, Ukraine; Joint Institute for Nuclear Research, Dubna, Russia;Joint Institute for Nuclear Research, Dubna, RussiaTaras Shevchenko National University of Kyiv, Kyiv, Ukraine; Joint Institute for Nuclear Research, Dubna, Russia; Institute for Scintillation Materials, National Academy of Sciences of Ukraine, Kharkiv, UkraineBCMaterials, Basque Center for Materials, Applications and Nanostructures, 48940 Leioa, Spain; Ikerbasque, Basque Foundation for Science, 48009 Bilbao, SpainDepartment of Nanobiotechnology, Biology Centre, ISB, CAS, Ceske Budejovice, Czech RepublicTaras Shevchenko National University of Kyiv, Kyiv, UkraineA polymer brush system of a neutral polymer poly (ethylene glycol) with a molecular weight of Mw = 20 kDa on silicon substrates in an aqueous medium was studied by the specular neutron reflectometry. Structural changes in the density profile of a polymer brush caused by the interaction of polymer chains with micelles of the anionic surfactant dodecylbenzenesulfonate acid were observed. The effect is shown to be related to the formation of molecular polymer-micelle associates in the bulk of the solution, which was previously studied by small-angle neutron scattering in a wide range of surfactant concentrations at various molecular weights of the polymer. The density of the dry polymer layer on the silicon substrate was additionally characterized by X-ray reflectometry and scanning atomic force microscopy.http://jnpae.kinr.kiev.ua/22.2/Articles_PDF/jnpae-2021-22-0149-Artykulnyi.pdfmicellesanionic surfactantspoly (ethylene glycol)neutron reflectometrypolymer brushsmall-angle neutron scattering.
spellingShingle O. P. Artykulnyi
M. M. Avdeev
Ye. M. Kosiachkin
V. I. Petrenko
I. Safarik
L. A. Bulavin
Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system
Ядерна фізика та енергетика
micelles
anionic surfactants
poly (ethylene glycol)
neutron reflectometry
polymer brush
small-angle neutron scattering.
title Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system
title_full Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system
title_fullStr Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system
title_full_unstemmed Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system
title_short Neutron investigation of interaction between anionic surfactant micelles and poly (ethylene glycol) polymer brush system
title_sort neutron investigation of interaction between anionic surfactant micelles and poly ethylene glycol polymer brush system
topic micelles
anionic surfactants
poly (ethylene glycol)
neutron reflectometry
polymer brush
small-angle neutron scattering.
url http://jnpae.kinr.kiev.ua/22.2/Articles_PDF/jnpae-2021-22-0149-Artykulnyi.pdf
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AT mmavdeev neutroninvestigationofinteractionbetweenanionicsurfactantmicellesandpolyethyleneglycolpolymerbrushsystem
AT yemkosiachkin neutroninvestigationofinteractionbetweenanionicsurfactantmicellesandpolyethyleneglycolpolymerbrushsystem
AT vipetrenko neutroninvestigationofinteractionbetweenanionicsurfactantmicellesandpolyethyleneglycolpolymerbrushsystem
AT isafarik neutroninvestigationofinteractionbetweenanionicsurfactantmicellesandpolyethyleneglycolpolymerbrushsystem
AT labulavin neutroninvestigationofinteractionbetweenanionicsurfactantmicellesandpolyethyleneglycolpolymerbrushsystem