Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt

A molten salt reactor is one of the fourth-generation reactors and is considered to be a feasible replacement for current reactors due to their many advantages. However, there are a number of issues that remain; one of which is the corrosion of the materials. Corrosion problems in molten salt reacto...

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Main Authors: Maehyun Cho, Michael R. Tonks, Kunok Chang
Format: Article
Language:English
Published: MDPI AG 2024-09-01
Series:Metals
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Online Access:https://www.mdpi.com/2075-4701/14/9/1088
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author Maehyun Cho
Michael R. Tonks
Kunok Chang
author_facet Maehyun Cho
Michael R. Tonks
Kunok Chang
author_sort Maehyun Cho
collection DOAJ
description A molten salt reactor is one of the fourth-generation reactors and is considered to be a feasible replacement for current reactors due to their many advantages. However, there are a number of issues that remain; one of which is the corrosion of the materials. Corrosion problems in molten salt reactors have been reported since The Molten Salt Reactor Experiment at Oak Ridge National Laboratory in the 1960s. There have been many attempts to mitigate the corrosion problem, but a fundamental solution has not yet been achived. In this study, surface reaction-diffusion-coupled simulations were performed to simulate the corrosion of a Ni–Cr–Fe material, a prototype of Hastelloy N, which is being promoted as a structural material for molten salt reactors in F–Li–Na–K eutectic salts. This surface reaction-diffusion-coupled simulation framework was developed to study which corrosion reactions are dominant in molten salt environment corrosion where a large number of oxidation–reduction reactions exist, the correlation between composition of alloy and corrosion rate, and the effect of Cr depletion on corrosion.
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spelling doaj-art-2a9d0e571d1f4c4fa9cf2363a97730772025-08-20T01:55:41ZengMDPI AGMetals2075-47012024-09-01149108810.3390/met14091088Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten SaltMaehyun Cho0Michael R. Tonks1Kunok Chang2Department of Nuclear Engineering, Kyung Hee University, Yongin-si 17104, Republic of KoreaDepartment of Materials Science and Engineering, University of Florida, Gainesville, FL 32603, USADepartment of Nuclear Engineering, Kyung Hee University, Yongin-si 17104, Republic of KoreaA molten salt reactor is one of the fourth-generation reactors and is considered to be a feasible replacement for current reactors due to their many advantages. However, there are a number of issues that remain; one of which is the corrosion of the materials. Corrosion problems in molten salt reactors have been reported since The Molten Salt Reactor Experiment at Oak Ridge National Laboratory in the 1960s. There have been many attempts to mitigate the corrosion problem, but a fundamental solution has not yet been achived. In this study, surface reaction-diffusion-coupled simulations were performed to simulate the corrosion of a Ni–Cr–Fe material, a prototype of Hastelloy N, which is being promoted as a structural material for molten salt reactors in F–Li–Na–K eutectic salts. This surface reaction-diffusion-coupled simulation framework was developed to study which corrosion reactions are dominant in molten salt environment corrosion where a large number of oxidation–reduction reactions exist, the correlation between composition of alloy and corrosion rate, and the effect of Cr depletion on corrosion.https://www.mdpi.com/2075-4701/14/9/1088molten salt reactorcorrosionsurface reaction-diffusion-coupled simulation
spellingShingle Maehyun Cho
Michael R. Tonks
Kunok Chang
Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt
Metals
molten salt reactor
corrosion
surface reaction-diffusion-coupled simulation
title Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt
title_full Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt
title_fullStr Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt
title_full_unstemmed Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt
title_short Surface Reaction-Diffusion-Coupled Simulation of Ni–Fe–Cr Alloy under FLiNaK Molten Salt
title_sort surface reaction diffusion coupled simulation of ni fe cr alloy under flinak molten salt
topic molten salt reactor
corrosion
surface reaction-diffusion-coupled simulation
url https://www.mdpi.com/2075-4701/14/9/1088
work_keys_str_mv AT maehyuncho surfacereactiondiffusioncoupledsimulationofnifecralloyunderflinakmoltensalt
AT michaelrtonks surfacereactiondiffusioncoupledsimulationofnifecralloyunderflinakmoltensalt
AT kunokchang surfacereactiondiffusioncoupledsimulationofnifecralloyunderflinakmoltensalt