Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques

Carminic acid is a natural pigment typically found in several insect taxa, including specific insects such as “grana cochinilla fina” in Mexico (<i>Dactylopius coccus</i> Costa). Commercially, it is also referred to as carmine, which is a more concentrated solution presenting as at least...

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Main Authors: Rogelio Reyes-Pérez, Juanita Pérez-Hernández, Minerva Rosas-Morales, Miguel Ángel Plascencia-Espinosa, Oxana Lazo-Zamalloa, Valentín López-Gayou, Pedro Antonio López, Gabriel Ríos-Cortés, Ada María Ríos-Cortés
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Molecules
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Online Access:https://www.mdpi.com/1420-3049/29/23/5568
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author Rogelio Reyes-Pérez
Juanita Pérez-Hernández
Minerva Rosas-Morales
Miguel Ángel Plascencia-Espinosa
Oxana Lazo-Zamalloa
Valentín López-Gayou
Pedro Antonio López
Gabriel Ríos-Cortés
Ada María Ríos-Cortés
author_facet Rogelio Reyes-Pérez
Juanita Pérez-Hernández
Minerva Rosas-Morales
Miguel Ángel Plascencia-Espinosa
Oxana Lazo-Zamalloa
Valentín López-Gayou
Pedro Antonio López
Gabriel Ríos-Cortés
Ada María Ríos-Cortés
author_sort Rogelio Reyes-Pérez
collection DOAJ
description Carminic acid is a natural pigment typically found in several insect taxa, including specific insects such as “grana cochinilla fina” in Mexico (<i>Dactylopius coccus</i> Costa). Commercially, it is also referred to as carmine, which is a more concentrated solution presenting as at least 50% carminic acid. To date, this dye has been used in the pharmaceutical, food and cosmetic industries. Unfortunately, one of the main limitations has to do with establishing the appropriate extraction and purification protocol. Currently, there is growing interest in developing eco-friendly and efficient pigment extraction processes for various applications. In this study, we compare the ultrasound- and microwave-assisted extraction versus with a conventional method to obtain carminic acid from cochineal. To do this, we considered three factors that influence the extraction process as independent variables: solvent volume, temperature and irradiation time. The optimization was carried out using the response surface methodology, employing a three-factor and three-level Box–Behnken experimental design. Carminic acid contents were quantified by UV–Vis spectroscopy, and extracts were evaluated by infrared spectroscopy to verify the integrity of the carminic acid molecule. The yield obtained by ultrasound-assisted extraction was 49.2 ± 3.25, with an efficiency of 31.3 mg/min, while microwave-assisted extraction showed a yield of 40.89 ± 2.96, with an efficiency of 27.3 mg/min. Both methods exceeded the extract yield (31.9 ± 3.4%) and efficiency (10.6 mg/min) obtained with the conventional method, demostrating that ultrasound- and microwave-assisted extraction are viable alternatives for obtaining carminic acid, with the potential to be scaled up to an industrial level.
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spelling doaj-art-29c365a14bbf45169fd92d1aee8349d92025-08-20T01:55:38ZengMDPI AGMolecules1420-30492024-11-012923556810.3390/molecules29235568Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave TechniquesRogelio Reyes-Pérez0Juanita Pérez-Hernández1Minerva Rosas-Morales2Miguel Ángel Plascencia-Espinosa3Oxana Lazo-Zamalloa4Valentín López-Gayou5Pedro Antonio López6Gabriel Ríos-Cortés7Ada María Ríos-Cortés8Centro de Desarrollo de Productos Bióticos, Instituto Politécnico Nacional, Carr Yautepec-Jojutla s/n-Km. 85, San Isidro 62739, Morelos, MexicoCentro de Investigación Biomédica del Sur, Instituto Mexicano del Seguro Social, C. Rep. Argentina 1, Xochitepec 62790, Morelos, MexicoCentro de Investigación en Biotecnología Aplicada, Instituto Politécnico Nacional, Ex-Hacienda San Juan Molino Carretera Estatal Tecuexcomac-Tepetitla Km. 1.5, Tepetitla de Lardizábal 90700, Tlaxcala, MexicoCentro de Investigación en Biotecnología Aplicada, Instituto Politécnico Nacional, Ex-Hacienda San Juan Molino Carretera Estatal Tecuexcomac-Tepetitla Km. 1.5, Tepetitla de Lardizábal 90700, Tlaxcala, MexicoCentro de Investigación en Biotecnología Aplicada, Instituto Politécnico Nacional, Ex-Hacienda San Juan Molino Carretera Estatal Tecuexcomac-Tepetitla Km. 1.5, Tepetitla de Lardizábal 90700, Tlaxcala, MexicoCentro de Investigación en Biotecnología Aplicada, Instituto Politécnico Nacional, Ex-Hacienda San Juan Molino Carretera Estatal Tecuexcomac-Tepetitla Km. 1.5, Tepetitla de Lardizábal 90700, Tlaxcala, MexicoColegio de Postgraduados, Campus Puebla, Boulevard Forjadores de Puebla No. 205, Santiago Momoxpan, Municipio de San Pedro Cholula 72760, Puebla, MexicoDepartamento de Ingeniería Química, Tecnológico Nacional de México, Instituto Tecnológico de Orizaba, Oriente 9, Orizaba 94320, Veracruz, MexicoCentro de Investigación en Biotecnología Aplicada, Instituto Politécnico Nacional, Ex-Hacienda San Juan Molino Carretera Estatal Tecuexcomac-Tepetitla Km. 1.5, Tepetitla de Lardizábal 90700, Tlaxcala, MexicoCarminic acid is a natural pigment typically found in several insect taxa, including specific insects such as “grana cochinilla fina” in Mexico (<i>Dactylopius coccus</i> Costa). Commercially, it is also referred to as carmine, which is a more concentrated solution presenting as at least 50% carminic acid. To date, this dye has been used in the pharmaceutical, food and cosmetic industries. Unfortunately, one of the main limitations has to do with establishing the appropriate extraction and purification protocol. Currently, there is growing interest in developing eco-friendly and efficient pigment extraction processes for various applications. In this study, we compare the ultrasound- and microwave-assisted extraction versus with a conventional method to obtain carminic acid from cochineal. To do this, we considered three factors that influence the extraction process as independent variables: solvent volume, temperature and irradiation time. The optimization was carried out using the response surface methodology, employing a three-factor and three-level Box–Behnken experimental design. Carminic acid contents were quantified by UV–Vis spectroscopy, and extracts were evaluated by infrared spectroscopy to verify the integrity of the carminic acid molecule. The yield obtained by ultrasound-assisted extraction was 49.2 ± 3.25, with an efficiency of 31.3 mg/min, while microwave-assisted extraction showed a yield of 40.89 ± 2.96, with an efficiency of 27.3 mg/min. Both methods exceeded the extract yield (31.9 ± 3.4%) and efficiency (10.6 mg/min) obtained with the conventional method, demostrating that ultrasound- and microwave-assisted extraction are viable alternatives for obtaining carminic acid, with the potential to be scaled up to an industrial level.https://www.mdpi.com/1420-3049/29/23/5568natural pigmentultrasoundmicrowavegreen extractionBox–Behnken design
spellingShingle Rogelio Reyes-Pérez
Juanita Pérez-Hernández
Minerva Rosas-Morales
Miguel Ángel Plascencia-Espinosa
Oxana Lazo-Zamalloa
Valentín López-Gayou
Pedro Antonio López
Gabriel Ríos-Cortés
Ada María Ríos-Cortés
Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques
Molecules
natural pigment
ultrasound
microwave
green extraction
Box–Behnken design
title Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques
title_full Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques
title_fullStr Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques
title_full_unstemmed Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques
title_short Cochineal (<i>Dactylopius coccus</i> Costa) Pigment Extraction Assisted by Ultrasound and Microwave Techniques
title_sort cochineal i dactylopius coccus i costa pigment extraction assisted by ultrasound and microwave techniques
topic natural pigment
ultrasound
microwave
green extraction
Box–Behnken design
url https://www.mdpi.com/1420-3049/29/23/5568
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