Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon

The flue gas mercury removal experiment was carried out on a 0.3MW pilot scale circulating fluidized bed test facility by injecting biomass based activated carbon which is originally derived from rice husk and then modified by halogenated ammonium. Effects of exit temperature of the SCR and flue gas...

Full description

Saved in:
Bibliographic Details
Main Authors: Jun TAO, Xiaobing GU, Tianfang HUANG, Shuai LIU, Peng HU, Lu DONG, Yaji HUANG, Yufeng DUAN
Format: Article
Language:zho
Published: State Grid Energy Research Institute 2019-10-01
Series:Zhongguo dianli
Subjects:
Online Access:https://www.electricpower.com.cn/CN/10.11930/j.issn.1004-9649.201901022
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850053390918221824
author Jun TAO
Xiaobing GU
Tianfang HUANG
Shuai LIU
Peng HU
Lu DONG
Yaji HUANG
Yufeng DUAN
author_facet Jun TAO
Xiaobing GU
Tianfang HUANG
Shuai LIU
Peng HU
Lu DONG
Yaji HUANG
Yufeng DUAN
author_sort Jun TAO
collection DOAJ
description The flue gas mercury removal experiment was carried out on a 0.3MW pilot scale circulating fluidized bed test facility by injecting biomass based activated carbon which is originally derived from rice husk and then modified by halogenated ammonium. Effects of exit temperature of the SCR and flue gas, concentration of SO2 and NO on the injection demercuration efficiency were discussed. The ASTM Standard D 6784-02 (OHM Ontario Method) was applied to measure the concentration of mercury from the coal-fired flue gas. The results showed that both the mercury removal efficiency and elemental mercury conversion efficiency go up with the elevated flue gas temperature; The existence of NO can enhance the mercury removal effect but SO2 will inhibit it on the other way. The mercury removal efficiency could reach about 90% with this modified type of activated carbon sprayed into flue gas under the conditions of SCR inlet temperature in the range of 351~370 °C , flue gas temperature in the range of 191~210 °C, SO2 volume fraction of (293~602)×10–6, NO volume fraction of (588~893)×10–6, activated carbon injection quantity of 0.5 kg/h, reaction space velocity of 4 000 h–1, and flue gas flow rate of 400~500 m3/h.
format Article
id doaj-art-28dce83ad8e24641b17b099a56b8cd5b
institution DOAJ
issn 1004-9649
language zho
publishDate 2019-10-01
publisher State Grid Energy Research Institute
record_format Article
series Zhongguo dianli
spelling doaj-art-28dce83ad8e24641b17b099a56b8cd5b2025-08-20T02:52:34ZzhoState Grid Energy Research InstituteZhongguo dianli1004-96492019-10-01521015015410.11930/j.issn.1004-9649.201901022zgdl-52-8-taojunEffect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated CarbonJun TAO0Xiaobing GU1Tianfang HUANG2Shuai LIU3Peng HU4Lu DONG5Yaji HUANG6Yufeng DUAN7Datang Environment Industry Group Co., Ltd., Beijing 100097, ChinaDatang Environment Industry Group Co., Ltd., Beijing 100097, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, ChinaKey Laboratory of Energy Thermal Conversion and Control of Ministry of Education, School of Energy and Environment, Southeast University, Nanjing 210096, ChinaThe flue gas mercury removal experiment was carried out on a 0.3MW pilot scale circulating fluidized bed test facility by injecting biomass based activated carbon which is originally derived from rice husk and then modified by halogenated ammonium. Effects of exit temperature of the SCR and flue gas, concentration of SO2 and NO on the injection demercuration efficiency were discussed. The ASTM Standard D 6784-02 (OHM Ontario Method) was applied to measure the concentration of mercury from the coal-fired flue gas. The results showed that both the mercury removal efficiency and elemental mercury conversion efficiency go up with the elevated flue gas temperature; The existence of NO can enhance the mercury removal effect but SO2 will inhibit it on the other way. The mercury removal efficiency could reach about 90% with this modified type of activated carbon sprayed into flue gas under the conditions of SCR inlet temperature in the range of 351~370 °C , flue gas temperature in the range of 191~210 °C, SO2 volume fraction of (293~602)×10–6, NO volume fraction of (588~893)×10–6, activated carbon injection quantity of 0.5 kg/h, reaction space velocity of 4 000 h–1, and flue gas flow rate of 400~500 m3/h.https://www.electricpower.com.cn/CN/10.11930/j.issn.1004-9649.201901022coal fired flue gasinjection demercurationnh4br modificationrice husk-derived activated carbonflue gas composition
spellingShingle Jun TAO
Xiaobing GU
Tianfang HUANG
Shuai LIU
Peng HU
Lu DONG
Yaji HUANG
Yufeng DUAN
Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon
Zhongguo dianli
coal fired flue gas
injection demercuration
nh4br modification
rice husk-derived activated carbon
flue gas composition
title Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon
title_full Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon
title_fullStr Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon
title_full_unstemmed Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon
title_short Effect of Flue Gas Composition on Mercury Removal by Injecting Rice Husk-Derived Activated Carbon
title_sort effect of flue gas composition on mercury removal by injecting rice husk derived activated carbon
topic coal fired flue gas
injection demercuration
nh4br modification
rice husk-derived activated carbon
flue gas composition
url https://www.electricpower.com.cn/CN/10.11930/j.issn.1004-9649.201901022
work_keys_str_mv AT juntao effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT xiaobinggu effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT tianfanghuang effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT shuailiu effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT penghu effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT ludong effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT yajihuang effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon
AT yufengduan effectoffluegascompositiononmercuryremovalbyinjectingricehuskderivedactivatedcarbon