Einfluss von α-Methylsubstituenten auf die Triplett-Di-π-Methan-Umlagerung von Allylbenzolen

The sensitized di-π-methane rearrangement of allylated benzene derivatives is strongly favoured by α-methyl substituents in the allyl side chain (Scheme 2). On the other hand, β- and γ-methyl substituents in the allyl moiety hinder or at least retard the triplett di-π-methane rearrangement. In the...

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Bibliographic Details
Main Authors: Jean-Pierre Fasel, Hans-Jürgen Hansen
Format: Article
Language:deu
Published: Swiss Chemical Society 1982-05-01
Series:CHIMIA
Online Access:https://www.chimia.ch/chimia/article/view/9558
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Summary:The sensitized di-π-methane rearrangement of allylated benzene derivatives is strongly favoured by α-methyl substituents in the allyl side chain (Scheme 2). On the other hand, β- and γ-methyl substituents in the allyl moiety hinder or at least retard the triplett di-π-methane rearrangement. In the presence of additional α-methyl groups the rearrangement is again facilitated (Scheme 3). The triplet di-π-methane-rearrangement of 4-allyl biphenyl is also strongly influenced by α-methyl substituents (Schema 4).
ISSN:0009-4293
2673-2424