Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor

This study examined the photocatalytic degradation of wastewater containing methyl violet dye in a recirculating slurry-type reactor using commercial TiO2 as the photocatalyst under ultraviolet irradiation. The effects of initial dye concentration (10 – 80 ppm), photocatalyst dosage (0.2 – 1 g/L), s...

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Main Authors: F. Shokry, M. El-Gedawy, S.A. Nosier, M.H. Abdel-Aziz
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Results in Chemistry
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Online Access:http://www.sciencedirect.com/science/article/pii/S2211715624006763
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author F. Shokry
M. El-Gedawy
S.A. Nosier
M.H. Abdel-Aziz
author_facet F. Shokry
M. El-Gedawy
S.A. Nosier
M.H. Abdel-Aziz
author_sort F. Shokry
collection DOAJ
description This study examined the photocatalytic degradation of wastewater containing methyl violet dye in a recirculating slurry-type reactor using commercial TiO2 as the photocatalyst under ultraviolet irradiation. The effects of initial dye concentration (10 – 80 ppm), photocatalyst dosage (0.2 – 1 g/L), solution pH (2 – 11), and flow rate (2 – 4 L/min) on degradation efficiency were thoroughly assessed. Results showed that degradation efficiency increased with pH, peaking at neutral pH (7), before declining at higher values. Similarly, catalyst loading up to 1 g/L enhanced efficiency, but further increases caused a decline. Higher solution flow rates improved mass transfer by increasing turbulence, leading to enhanced degradation efficiency. Optimal conditions (neutral pH, 1 g/L catalyst loading, and 4 L/min flow rate) achieved complete decolorization of a 10-ppm dye solution. These findings highlight the feasibility of achieving high degradation efficiencies under practical conditions, supporting the potential for industrial-scale application in effluent treatment.
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institution Kabale University
issn 2211-7156
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publishDate 2025-01-01
publisher Elsevier
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series Results in Chemistry
spelling doaj-art-26f00903fa734d12890d2cf9647087f22025-01-29T05:00:47ZengElsevierResults in Chemistry2211-71562025-01-0113101980Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactorF. Shokry0M. El-Gedawy1S.A. Nosier2M.H. Abdel-Aziz3Chemical Engineering Department, Faculty of Engineering Port Said University, Port Said 42526, EgyptChemical Engineering Department, Faculty of Engineering, Alexandria University, Alexandria 21544, EgyptChemical Engineering Department, Faculty of Engineering, Alexandria University, Alexandria 21544, EgyptChemical Engineering Department, Faculty of Engineering, Alexandria University, Alexandria 21544, Egypt; Chemical and Materials Engineering Department, King Abdulaziz University, Rabigh 21911, Saudi Arabia; Corresponding author at: Chemical Engineering Department, Faculty of Engineering, Alexandria University, Alexandria 21544, Egypt.This study examined the photocatalytic degradation of wastewater containing methyl violet dye in a recirculating slurry-type reactor using commercial TiO2 as the photocatalyst under ultraviolet irradiation. The effects of initial dye concentration (10 – 80 ppm), photocatalyst dosage (0.2 – 1 g/L), solution pH (2 – 11), and flow rate (2 – 4 L/min) on degradation efficiency were thoroughly assessed. Results showed that degradation efficiency increased with pH, peaking at neutral pH (7), before declining at higher values. Similarly, catalyst loading up to 1 g/L enhanced efficiency, but further increases caused a decline. Higher solution flow rates improved mass transfer by increasing turbulence, leading to enhanced degradation efficiency. Optimal conditions (neutral pH, 1 g/L catalyst loading, and 4 L/min flow rate) achieved complete decolorization of a 10-ppm dye solution. These findings highlight the feasibility of achieving high degradation efficiencies under practical conditions, supporting the potential for industrial-scale application in effluent treatment.http://www.sciencedirect.com/science/article/pii/S2211715624006763Photocatalytic degradationMethyl violet dyeSlurry-type reactorRecirculationTiO2 photocatalystWastewater treatment
spellingShingle F. Shokry
M. El-Gedawy
S.A. Nosier
M.H. Abdel-Aziz
Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor
Results in Chemistry
Photocatalytic degradation
Methyl violet dye
Slurry-type reactor
Recirculation
TiO2 photocatalyst
Wastewater treatment
title Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor
title_full Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor
title_fullStr Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor
title_full_unstemmed Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor
title_short Optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry-type reactor
title_sort optimizing photocatalytic degradation of methyl violet dye in a recirculating slurry type reactor
topic Photocatalytic degradation
Methyl violet dye
Slurry-type reactor
Recirculation
TiO2 photocatalyst
Wastewater treatment
url http://www.sciencedirect.com/science/article/pii/S2211715624006763
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AT melgedawy optimizingphotocatalyticdegradationofmethylvioletdyeinarecirculatingslurrytypereactor
AT sanosier optimizingphotocatalyticdegradationofmethylvioletdyeinarecirculatingslurrytypereactor
AT mhabdelaziz optimizingphotocatalyticdegradationofmethylvioletdyeinarecirculatingslurrytypereactor