Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration

Abstract Chronic back pain and disability are primarily caused by intervertebral disc degeneration (IDD) that requires novel therapies to regenerate the nucleus pulposus (NP) and restore disc function. In this study, a bioengineered thermo-sensitive injectable hydrogel composed of co-polymeric poly-...

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Main Authors: Guangnan Chen, Chong Bian, Xiangyang Cheng, Jun Xu, Kaifeng Zhou, Yiming Zhang
Format: Article
Language:English
Published: BMC 2025-05-01
Series:Journal of Biological Engineering
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Online Access:https://doi.org/10.1186/s13036-025-00520-0
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author Guangnan Chen
Chong Bian
Xiangyang Cheng
Jun Xu
Kaifeng Zhou
Yiming Zhang
author_facet Guangnan Chen
Chong Bian
Xiangyang Cheng
Jun Xu
Kaifeng Zhou
Yiming Zhang
author_sort Guangnan Chen
collection DOAJ
description Abstract Chronic back pain and disability are primarily caused by intervertebral disc degeneration (IDD) that requires novel therapies to regenerate the nucleus pulposus (NP) and restore disc function. In this study, a bioengineered thermo-sensitive injectable hydrogel composed of co-polymeric poly-N-isopropyl acrylamide-grafted-chondroitin sulfate cross-linked with sodium alginate microspheres (PNIA-g-CS-NaA Ms: denote HMs) loaded with growth differentiation factor 5 (GDF-5), to stimulate Nucleus Pulposus cells (NPCs) activity and promote intervertebral disc (IVD) regeneration. The Low critical solution temperature (LCST) of PNIA-g-CS was 31.8 and 32.3 °C at 5% (w/v) and 15% (w/v), respectively. In the in vitro study, GDF-5-loaded hydrogel (1 mg/mL) marginally enhanced NPC proliferation and reduced inflammatory cytokines (TNF-α, IL-6, IL-1β) after 24 h. HMs-GDF-5 combined with Adipose-Derived Mesenchymal Stem Cells (ADMSCs) was delivered to NP tissue using a minimally invasive technique, promoting NP regeneration in rats. At 8 weeks, significant upregulation of COL-II and ACAN proteins and mRNA expressions was observed. X-ray imaging showed disc height recovery and increased water content, while histology revealed partial restoration of NPCs and matrix. The outcomes show that the biodegradable hydrogel could be used as a potential therapeutic agent for IVD repair.
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spelling doaj-art-26c1dda6d5e54fc28b5c08f866a0d5a02025-08-20T02:34:17ZengBMCJournal of Biological Engineering1754-16112025-05-0119111810.1186/s13036-025-00520-0Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regenerationGuangnan Chen0Chong Bian1Xiangyang Cheng2Jun Xu3Kaifeng Zhou4Yiming Zhang5Department of Orthopedics Surgery, Minhang Hospital, Fudan UniversityDepartment of Orthopedics Surgery, Minhang Hospital, Fudan UniversityDepartment of Orthopedics Surgery, Minhang Hospital, Fudan UniversityDepartment of Orthopedics Surgery, Minhang Hospital, Fudan UniversityDepartment of Orthopedics Surgery, Minhang Hospital, Fudan UniversityDepartment of Orthopedics Surgery, Minhang Hospital, Fudan UniversityAbstract Chronic back pain and disability are primarily caused by intervertebral disc degeneration (IDD) that requires novel therapies to regenerate the nucleus pulposus (NP) and restore disc function. In this study, a bioengineered thermo-sensitive injectable hydrogel composed of co-polymeric poly-N-isopropyl acrylamide-grafted-chondroitin sulfate cross-linked with sodium alginate microspheres (PNIA-g-CS-NaA Ms: denote HMs) loaded with growth differentiation factor 5 (GDF-5), to stimulate Nucleus Pulposus cells (NPCs) activity and promote intervertebral disc (IVD) regeneration. The Low critical solution temperature (LCST) of PNIA-g-CS was 31.8 and 32.3 °C at 5% (w/v) and 15% (w/v), respectively. In the in vitro study, GDF-5-loaded hydrogel (1 mg/mL) marginally enhanced NPC proliferation and reduced inflammatory cytokines (TNF-α, IL-6, IL-1β) after 24 h. HMs-GDF-5 combined with Adipose-Derived Mesenchymal Stem Cells (ADMSCs) was delivered to NP tissue using a minimally invasive technique, promoting NP regeneration in rats. At 8 weeks, significant upregulation of COL-II and ACAN proteins and mRNA expressions was observed. X-ray imaging showed disc height recovery and increased water content, while histology revealed partial restoration of NPCs and matrix. The outcomes show that the biodegradable hydrogel could be used as a potential therapeutic agent for IVD repair.https://doi.org/10.1186/s13036-025-00520-0HydrogelSodium alginateGrowth differentiation factorStem cellsNucleus pulposusIntervertebral disc regeneration
spellingShingle Guangnan Chen
Chong Bian
Xiangyang Cheng
Jun Xu
Kaifeng Zhou
Yiming Zhang
Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration
Journal of Biological Engineering
Hydrogel
Sodium alginate
Growth differentiation factor
Stem cells
Nucleus pulposus
Intervertebral disc regeneration
title Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration
title_full Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration
title_fullStr Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration
title_full_unstemmed Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration
title_short Bio-engineered thermo-sensitive alginate/PNIA-g-CS co-polymeric injectable hydrogel laden with GDF-5 to stimulate nucleus pulposus for IVD regeneration
title_sort bio engineered thermo sensitive alginate pnia g cs co polymeric injectable hydrogel laden with gdf 5 to stimulate nucleus pulposus for ivd regeneration
topic Hydrogel
Sodium alginate
Growth differentiation factor
Stem cells
Nucleus pulposus
Intervertebral disc regeneration
url https://doi.org/10.1186/s13036-025-00520-0
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