Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties

The inherently poor flame retardancy and comparatively low tensile strength of poly(lactic acid) (PLA) have limited its wide adoption as alternative ‘green’ engineering plastic in many fields. This manuscript reports the synthesis of a new phosphorus flame retardant – phenylphosphonic 3(2-aminobenzo...

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Main Authors: B. Tawiah, B. Yu, S. Ullah, R. Wei, R. K. K. Yuen, J. H. Xin, B. Fei
Format: Article
Language:English
Published: Budapest University of Technology and Economics 2019-08-01
Series:eXPRESS Polymer Letters
Subjects:
Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0009876&mi=cd
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author B. Tawiah
B. Yu
S. Ullah
R. Wei
R. K. K. Yuen
J. H. Xin
B. Fei
author_facet B. Tawiah
B. Yu
S. Ullah
R. Wei
R. K. K. Yuen
J. H. Xin
B. Fei
author_sort B. Tawiah
collection DOAJ
description The inherently poor flame retardancy and comparatively low tensile strength of poly(lactic acid) (PLA) have limited its wide adoption as alternative ‘green’ engineering plastic in many fields. This manuscript reports the synthesis of a new phosphorus flame retardant – phenylphosphonic 3(2-aminobenzothiazole) (P-TAB) and its combination with recycled short wool fibers (WF) for improving the flame retardancy and the mechanical properties of PLA. Fourier transform infrared (FTIR), 1H, and 13C nuclear magnetic resonance (NMR) spectra proved that P-TAB was effectively synthesized. Considerable reductions in heat release rate, total heat released, CO and CO2 produced were attained with 3 wt% P-TAB and various WF loadings. The fire performance index (FPI), and fire growth index (FGI) improved by 38.2 and 48.1% respectively. The composite achieved a V-0 rating at 20 wt% WF loading and an LOI value of 28.5%. TG-IR results showed substantial reductions in evolved gaseous products. The tensile strength and Young’s modulus improved significantly with the increasing content of WF in the composite.
format Article
id doaj-art-25b6c6c4ea9544799da744610c30c652
institution Kabale University
issn 1788-618X
language English
publishDate 2019-08-01
publisher Budapest University of Technology and Economics
record_format Article
series eXPRESS Polymer Letters
spelling doaj-art-25b6c6c4ea9544799da744610c30c6522025-08-20T03:33:08ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2019-08-0113869771210.3144/expresspolymlett.2019.59Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical propertiesB. TawiahB. YuS. UllahR. WeiR. K. K. YuenJ. H. XinB. FeiThe inherently poor flame retardancy and comparatively low tensile strength of poly(lactic acid) (PLA) have limited its wide adoption as alternative ‘green’ engineering plastic in many fields. This manuscript reports the synthesis of a new phosphorus flame retardant – phenylphosphonic 3(2-aminobenzothiazole) (P-TAB) and its combination with recycled short wool fibers (WF) for improving the flame retardancy and the mechanical properties of PLA. Fourier transform infrared (FTIR), 1H, and 13C nuclear magnetic resonance (NMR) spectra proved that P-TAB was effectively synthesized. Considerable reductions in heat release rate, total heat released, CO and CO2 produced were attained with 3 wt% P-TAB and various WF loadings. The fire performance index (FPI), and fire growth index (FGI) improved by 38.2 and 48.1% respectively. The composite achieved a V-0 rating at 20 wt% WF loading and an LOI value of 28.5%. TG-IR results showed substantial reductions in evolved gaseous products. The tensile strength and Young’s modulus improved significantly with the increasing content of WF in the composite.http://www.expresspolymlett.com/letolt.php?file=EPL-0009876&mi=cdPolymer compositesFlame retardant cone calorimeter fiber reinforcement pyrolysis products
spellingShingle B. Tawiah
B. Yu
S. Ullah
R. Wei
R. K. K. Yuen
J. H. Xin
B. Fei
Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties
eXPRESS Polymer Letters
Polymer composites
Flame retardant
cone calorimeter
fiber reinforcement
pyrolysis products
title Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties
title_full Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties
title_fullStr Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties
title_full_unstemmed Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties
title_short Flame retardant poly(lactic acid) biocomposites reinforced by recycled wool fibers – Thermal and mechanical properties
title_sort flame retardant poly lactic acid biocomposites reinforced by recycled wool fibers thermal and mechanical properties
topic Polymer composites
Flame retardant
cone calorimeter
fiber reinforcement
pyrolysis products
url http://www.expresspolymlett.com/letolt.php?file=EPL-0009876&mi=cd
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