Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides

A heterostructure of diamagnetic magnesium‒aluminium layered double hydroxides (Mg‒Al LDHs) and photomag‐ netic cobalt‒iron Prussian Blue analogue (Co‒Fe PBA) was designed, synthesized and then designated as LDH‒PB. The cyanide-bridged Co‒Fe PBA was two-dimensionally intercalated into the Mg‒Al LDH...

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Main Authors: Cuijuan Zhang, Takashi Yamamoto, Yasuaki Einaga
Format: Article
Language:English
Published: Wiley 2016-04-01
Series:Nanomaterials and Nanotechnology
Subjects:
Online Access:http://www.intechopen.com/journals/nanomaterials_and_nanotechnology/co-ndash-fe-prussian-blue-analogue-intercalated-into-diamagnetic-mg-ndash-al-layered-double-hydroxid
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author Cuijuan Zhang
Takashi Yamamoto
Yasuaki Einaga
author_facet Cuijuan Zhang
Takashi Yamamoto
Yasuaki Einaga
author_sort Cuijuan Zhang
collection DOAJ
description A heterostructure of diamagnetic magnesium‒aluminium layered double hydroxides (Mg‒Al LDHs) and photomag‐ netic cobalt‒iron Prussian Blue analogue (Co‒Fe PBA) was designed, synthesized and then designated as LDH‒PB. The cyanide-bridged Co‒Fe PBA was two-dimensionally intercalated into the Mg‒Al LDH template by the stepwise anion exchange method. LDH‒PB showed ferrimagnetic properties with in-plane antiferromagnetic exchange interactions, as well as small photo-induced magnetization by visible light illumination due to the low dimensional structures and the characteristic photo-induced electronic states of the mixed valence of FeIII(low spin, S = 1/2)‒CN‒ CoII(high spin, S = 3/2)‒NC‒FeII (low spin, S = 0).
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language English
publishDate 2016-04-01
publisher Wiley
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series Nanomaterials and Nanotechnology
spelling doaj-art-2575cb0219d74af38324d8a7607c2f882025-08-20T03:54:52ZengWileyNanomaterials and Nanotechnology1847-98042016-04-01626http://dx.doi.org/10.5772/6327650331Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double HydroxidesCuijuan ZhangTakashi YamamotoYasuaki EinagaA heterostructure of diamagnetic magnesium‒aluminium layered double hydroxides (Mg‒Al LDHs) and photomag‐ netic cobalt‒iron Prussian Blue analogue (Co‒Fe PBA) was designed, synthesized and then designated as LDH‒PB. The cyanide-bridged Co‒Fe PBA was two-dimensionally intercalated into the Mg‒Al LDH template by the stepwise anion exchange method. LDH‒PB showed ferrimagnetic properties with in-plane antiferromagnetic exchange interactions, as well as small photo-induced magnetization by visible light illumination due to the low dimensional structures and the characteristic photo-induced electronic states of the mixed valence of FeIII(low spin, S = 1/2)‒CN‒ CoII(high spin, S = 3/2)‒NC‒FeII (low spin, S = 0).http://www.intechopen.com/journals/nanomaterials_and_nanotechnology/co-ndash-fe-prussian-blue-analogue-intercalated-into-diamagnetic-mg-ndash-al-layered-double-hydroxidLayered Double Hydroxides (LDHs)Prussian Blue Analogue (PBA)PhotomagneticMolecule-based MagnetIntercalation
spellingShingle Cuijuan Zhang
Takashi Yamamoto
Yasuaki Einaga
Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides
Nanomaterials and Nanotechnology
Layered Double Hydroxides (LDHs)
Prussian Blue Analogue (PBA)
Photomagnetic
Molecule-based Magnet
Intercalation
title Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides
title_full Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides
title_fullStr Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides
title_full_unstemmed Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides
title_short Co–Fe Prussian Blue Analogue Intercalated into Diamagnetic Mg–Al Layered Double Hydroxides
title_sort co fe prussian blue analogue intercalated into diamagnetic mg al layered double hydroxides
topic Layered Double Hydroxides (LDHs)
Prussian Blue Analogue (PBA)
Photomagnetic
Molecule-based Magnet
Intercalation
url http://www.intechopen.com/journals/nanomaterials_and_nanotechnology/co-ndash-fe-prussian-blue-analogue-intercalated-into-diamagnetic-mg-ndash-al-layered-double-hydroxid
work_keys_str_mv AT cuijuanzhang cofeprussianblueanalogueintercalatedintodiamagneticmgallayereddoublehydroxides
AT takashiyamamoto cofeprussianblueanalogueintercalatedintodiamagneticmgallayereddoublehydroxides
AT yasuakieinaga cofeprussianblueanalogueintercalatedintodiamagneticmgallayereddoublehydroxides