Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices

This study covers the synthesis and electrochemical characteristics of a nanocomposite solid electrolyte, AgI–Ag2CO3, including TiO2 nano-filler at various weight percentages ranging from 0 to 40 wt %. A series of compositions with various weight percentages of (1-x) AgI–Ag2CO3 -(x) TiO2 samples hav...

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Main Authors: Abjana Parbin, Shahla Imteyaz, Rafiuddin
Format: Article
Language:English
Published: Elsevier 2025-06-01
Series:Hybrid Advances
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Online Access:http://www.sciencedirect.com/science/article/pii/S2773207X25000223
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author Abjana Parbin
Shahla Imteyaz
Rafiuddin
author_facet Abjana Parbin
Shahla Imteyaz
Rafiuddin
author_sort Abjana Parbin
collection DOAJ
description This study covers the synthesis and electrochemical characteristics of a nanocomposite solid electrolyte, AgI–Ag2CO3, including TiO2 nano-filler at various weight percentages ranging from 0 to 40 wt %. A series of compositions with various weight percentages of (1-x) AgI–Ag2CO3 -(x) TiO2 samples have been fabricated by the solid-state method and characterized by FT-IR, XRD, SEM-EDX, TEM, and Impedance Spectroscopy to execute a comprehensive structural analysis of the post-synthetically modified solid electrolyte (SE). Among the various nanocomposite material compositions, 20 wt % TiO2 nanocomposite shows the highest ionic conductivity, i.e., σ = 1.159 × 10−2 Scm−1 and the lowest activation energy, 0.4789 eV at 298 K. The suggested conceptual approach was validated by the solid electrolyte's impedance, capacitance, and other structural behavior. The change in structure and morphology of the solid electrolyte has been found to be associated with the increase in conductivity, indicating that the amorphous domain is appropriate for solid-state battery applications.
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institution Kabale University
issn 2773-207X
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publishDate 2025-06-01
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series Hybrid Advances
spelling doaj-art-23c2edcd3d96481d964ddab8d66428af2025-08-20T03:25:54ZengElsevierHybrid Advances2773-207X2025-06-01910039810.1016/j.hybadv.2025.100398Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devicesAbjana Parbin0Shahla Imteyaz1 Rafiuddin2Physical Chemistry Division, Department of Chemistry, Aligarh Muslim University, Aligarh, 202002, IndiaPhysical Chemistry Division, Department of Chemistry, Aligarh Muslim University, Aligarh, 202002, IndiaCorresponding author.; Physical Chemistry Division, Department of Chemistry, Aligarh Muslim University, Aligarh, 202002, IndiaThis study covers the synthesis and electrochemical characteristics of a nanocomposite solid electrolyte, AgI–Ag2CO3, including TiO2 nano-filler at various weight percentages ranging from 0 to 40 wt %. A series of compositions with various weight percentages of (1-x) AgI–Ag2CO3 -(x) TiO2 samples have been fabricated by the solid-state method and characterized by FT-IR, XRD, SEM-EDX, TEM, and Impedance Spectroscopy to execute a comprehensive structural analysis of the post-synthetically modified solid electrolyte (SE). Among the various nanocomposite material compositions, 20 wt % TiO2 nanocomposite shows the highest ionic conductivity, i.e., σ = 1.159 × 10−2 Scm−1 and the lowest activation energy, 0.4789 eV at 298 K. The suggested conceptual approach was validated by the solid electrolyte's impedance, capacitance, and other structural behavior. The change in structure and morphology of the solid electrolyte has been found to be associated with the increase in conductivity, indicating that the amorphous domain is appropriate for solid-state battery applications.http://www.sciencedirect.com/science/article/pii/S2773207X25000223Solid electrolyteActivation energyIonic conductivityDielectric constantDielectric modulus
spellingShingle Abjana Parbin
Shahla Imteyaz
Rafiuddin
Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices
Hybrid Advances
Solid electrolyte
Activation energy
Ionic conductivity
Dielectric constant
Dielectric modulus
title Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices
title_full Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices
title_fullStr Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices
title_full_unstemmed Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices
title_short Synthesis and electrochemical characterization of titania nano-filler embedded AgI–Ag2CO3 solid electrolyte for energy storage devices
title_sort synthesis and electrochemical characterization of titania nano filler embedded agi ag2co3 solid electrolyte for energy storage devices
topic Solid electrolyte
Activation energy
Ionic conductivity
Dielectric constant
Dielectric modulus
url http://www.sciencedirect.com/science/article/pii/S2773207X25000223
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AT shahlaimteyaz synthesisandelectrochemicalcharacterizationoftitaniananofillerembeddedagiag2co3solidelectrolyteforenergystoragedevices
AT rafiuddin synthesisandelectrochemicalcharacterizationoftitaniananofillerembeddedagiag2co3solidelectrolyteforenergystoragedevices