SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION

In this study, the production of TiO2 nanoparticles from microcrystalline powder was accomplished using the high-energy ball milling (HEBM) technique. Three samples were milled for 0.5, 1, and 1.5 hours. The unmilled powder was also characterized as a comparison. The X-ray diffraction (XRD) techniqu...

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Main Authors: Ai Nurlaela, Elvan Yuniarti, Siti Ahmiatri Saptari
Format: Article
Language:English
Published: Universitas Negeri Jakarta 2023-08-01
Series:Spektra: Jurnal Fisika dan Aplikasinya
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Online Access:https://journal.unj.ac.id/unj/index.php/spektra/article/view/37094
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author Ai Nurlaela
Elvan Yuniarti
Siti Ahmiatri Saptari
author_facet Ai Nurlaela
Elvan Yuniarti
Siti Ahmiatri Saptari
author_sort Ai Nurlaela
collection DOAJ
description In this study, the production of TiO2 nanoparticles from microcrystalline powder was accomplished using the high-energy ball milling (HEBM) technique. Three samples were milled for 0.5, 1, and 1.5 hours. The unmilled powder was also characterized as a comparison. The X-ray diffraction (XRD) technique was utilized to investigate the changes in the microstructure of the milled powders over time. The XRD curve of milled samples showed the broadening of the diffraction peaks, which indicates a decrease in particle size after the milling process. Using the Debye–Scherrer relation, obtain the particle size that decreased from 138.43 nm before milled to 76.65 nm after 0.5 hours milled, 90.63 nm after 1 hour milled, and 83.05 nm after 1.5 hours milled. XRD analysis also showed that TiO2 was in an anatase phase before and after milling. Furthermore, two samples of TiO2, unmilled and after 0.5 hours milled, were used as a working photoelectrode of DSSC with dye from mustard leaves. DSSC efficiency was measured with a 1000-watt halogen lamp. The efficiency of DSSC with photoelectrodes using TiO2 after 0.5 hours milled, which is 0.1715, was higher than using TiO2 before milled, which is 0,0987. The Large surface area in TiO2 enhances the efficiency of DSSC, indicating that the HEBM technique is quite suitable for producing these nanoparticles for this aim.
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publishDate 2023-08-01
publisher Universitas Negeri Jakarta
record_format Article
series Spektra: Jurnal Fisika dan Aplikasinya
spelling doaj-art-21fd491d39944f11bbf3dcb68110bfeb2025-08-20T02:04:05ZengUniversitas Negeri JakartaSpektra: Jurnal Fisika dan Aplikasinya2541-33842541-33922023-08-0182839210.21009/SPEKTRA.082.0230617SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATIONAi Nurlaela0Elvan Yuniarti1Siti Ahmiatri Saptari2Prodi Tadris Fisika, Fakultas Ilmu Tarbiyah dan Keguruan, Universitas Islam Negeri Syarif Hidayatullah Jakarta. Jl. Ir. H. Juanda No 95. Ciputat-Tangerang Selatan, Banten 15412, IndonesiaProdi Fisika, Fakultas Sain dan Teknologi, Universitas Islam Negeri Syarif Hidayatullah Jakarta. Jl. Ir. H. Juanda No 95. Ciputat-Tangerang Selatan, Banten 15412, IndonesiaProdi Fisika, Fakultas Sain dan Teknologi, Universitas Islam Negeri Syarif Hidayatullah Jakarta. Jl. Ir. H. Juanda No 95. Ciputat-Tangerang Selatan, Banten 15412, IndonesiaIn this study, the production of TiO2 nanoparticles from microcrystalline powder was accomplished using the high-energy ball milling (HEBM) technique. Three samples were milled for 0.5, 1, and 1.5 hours. The unmilled powder was also characterized as a comparison. The X-ray diffraction (XRD) technique was utilized to investigate the changes in the microstructure of the milled powders over time. The XRD curve of milled samples showed the broadening of the diffraction peaks, which indicates a decrease in particle size after the milling process. Using the Debye–Scherrer relation, obtain the particle size that decreased from 138.43 nm before milled to 76.65 nm after 0.5 hours milled, 90.63 nm after 1 hour milled, and 83.05 nm after 1.5 hours milled. XRD analysis also showed that TiO2 was in an anatase phase before and after milling. Furthermore, two samples of TiO2, unmilled and after 0.5 hours milled, were used as a working photoelectrode of DSSC with dye from mustard leaves. DSSC efficiency was measured with a 1000-watt halogen lamp. The efficiency of DSSC with photoelectrodes using TiO2 after 0.5 hours milled, which is 0.1715, was higher than using TiO2 before milled, which is 0,0987. The Large surface area in TiO2 enhances the efficiency of DSSC, indicating that the HEBM technique is quite suitable for producing these nanoparticles for this aim.https://journal.unj.ac.id/unj/index.php/spektra/article/view/37094tio2nanoparticlesxrduv-visdssc efficiency
spellingShingle Ai Nurlaela
Elvan Yuniarti
Siti Ahmiatri Saptari
SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION
Spektra: Jurnal Fisika dan Aplikasinya
tio2
nanoparticles
xrd
uv-vis
dssc efficiency
title SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION
title_full SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION
title_fullStr SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION
title_full_unstemmed SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION
title_short SYNTHESIZE OF TiO2 NANOPARTICLES BY PLANETARY BALL MILL FOR DYE-SENSITIZED SOLAR CELLS (DSSC) PHOTOELECTRODE APPLICATION
title_sort synthesize of tio2 nanoparticles by planetary ball mill for dye sensitized solar cells dssc photoelectrode application
topic tio2
nanoparticles
xrd
uv-vis
dssc efficiency
url https://journal.unj.ac.id/unj/index.php/spektra/article/view/37094
work_keys_str_mv AT ainurlaela synthesizeoftio2nanoparticlesbyplanetaryballmillfordyesensitizedsolarcellsdsscphotoelectrodeapplication
AT elvanyuniarti synthesizeoftio2nanoparticlesbyplanetaryballmillfordyesensitizedsolarcellsdsscphotoelectrodeapplication
AT sitiahmiatrisaptari synthesizeoftio2nanoparticlesbyplanetaryballmillfordyesensitizedsolarcellsdsscphotoelectrodeapplication