Solid-electrolyte interphases for all-solid-state batteries

Interfacial engineering, particularly the design of artificial solid-electrolyte interphases (SEIs), has been successfully applied in all-solid-state batteries (ASSLBs) for industrial applications. However, a fundamental understanding of the synthesis and mechanism models of artificial SEIs in all-s...

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Main Authors: Yu Xia, Xu Han, Yue Ji, Simeng Zhang, Saiqi Wei, Yue Gong, Junyi Yue, Yueyue Wang, Xiaona Li, Zhiqiang Fang, Changtai Zhao, Jianwen Liang
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2025-01-01
Series:ChemPhysMater
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Online Access:http://www.sciencedirect.com/science/article/pii/S2772571524000597
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author Yu Xia
Xu Han
Yue Ji
Simeng Zhang
Saiqi Wei
Yue Gong
Junyi Yue
Yueyue Wang
Xiaona Li
Zhiqiang Fang
Changtai Zhao
Jianwen Liang
author_facet Yu Xia
Xu Han
Yue Ji
Simeng Zhang
Saiqi Wei
Yue Gong
Junyi Yue
Yueyue Wang
Xiaona Li
Zhiqiang Fang
Changtai Zhao
Jianwen Liang
author_sort Yu Xia
collection DOAJ
description Interfacial engineering, particularly the design of artificial solid-electrolyte interphases (SEIs), has been successfully applied in all-solid-state batteries (ASSLBs) for industrial applications. However, a fundamental understanding of the synthesis and mechanism models of artificial SEIs in all-solid-state Li-ion batteries remains limited. In this review, recent advances in designing and synthesizing artificial SEIs for ASSLBs to solve interfacial issues are thoroughly discussed, covering three main preparation methods and their technical routes: 1) atomic layer deposition, 2) sol-gel methods, and 3) mechanical ball-milling methods. Moreover, advanced ex-situ characterization techniques for artificial SEIs are comprehensively summarized. Finally, this review provides perspectives on techniques for the interface engineering of artificial SEIs for ASSLBs, with focus on promising methods for industrial applications.
format Article
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institution Kabale University
issn 2772-5715
language English
publishDate 2025-01-01
publisher KeAi Communications Co., Ltd.
record_format Article
series ChemPhysMater
spelling doaj-art-206dc89c2d52409797e2faf87a488d542025-01-22T05:44:25ZengKeAi Communications Co., Ltd.ChemPhysMater2772-57152025-01-0141929Solid-electrolyte interphases for all-solid-state batteriesYu Xia0Xu Han1Yue Ji2Simeng Zhang3Saiqi Wei4Yue Gong5Junyi Yue6Yueyue Wang7Xiaona Li8Zhiqiang Fang9Changtai Zhao10Jianwen Liang11National Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, ChinaNational Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, ChinaNational Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, ChinaSolid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; Eastern Institute for Advanced Study, Eastern Institute of Technology, Ningbo 315200, ChinaSolid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; School of Materials Science and Engineering, University of Science and Technology Beijing, Beijing 100083, ChinaSolid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; Key Laboratory of Automobile Materials of Ministry of Education & School of Materials Science and Engineering, Nanling Campus, Jilin University, Changchun 130025, China; China FAW Corporation Limited, Changchun 130013, ChinaSolid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; Eastern Institute for Advanced Study, Eastern Institute of Technology, Ningbo 315200, ChinaNational Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, ChinaEastern Institute for Advanced Study, Eastern Institute of Technology, Ningbo 315200, ChinaNational Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, China; Corresponding authors.National Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, China; Corresponding authors.National Power Battery Innovation Center, GRINM Group Co., Ltd., Beijing 100088, China; Solid State Batteries Research Center, GRINM (Guangdong) Institute for Advanced Materials and Technology, Foshan 528051, China; China Automotive Battery Research Institute Co., Ltd., Beijing 100088, China; General Research Institute for Nonferrous Metals, Beijing 100088, China; Corresponding authors.Interfacial engineering, particularly the design of artificial solid-electrolyte interphases (SEIs), has been successfully applied in all-solid-state batteries (ASSLBs) for industrial applications. However, a fundamental understanding of the synthesis and mechanism models of artificial SEIs in all-solid-state Li-ion batteries remains limited. In this review, recent advances in designing and synthesizing artificial SEIs for ASSLBs to solve interfacial issues are thoroughly discussed, covering three main preparation methods and their technical routes: 1) atomic layer deposition, 2) sol-gel methods, and 3) mechanical ball-milling methods. Moreover, advanced ex-situ characterization techniques for artificial SEIs are comprehensively summarized. Finally, this review provides perspectives on techniques for the interface engineering of artificial SEIs for ASSLBs, with focus on promising methods for industrial applications.http://www.sciencedirect.com/science/article/pii/S2772571524000597All-solid-state lithium batteriesInterfacial engineeringSolid-electrolyte interphaseAtomic layer depositionSol-gelMechanical ball-milling
spellingShingle Yu Xia
Xu Han
Yue Ji
Simeng Zhang
Saiqi Wei
Yue Gong
Junyi Yue
Yueyue Wang
Xiaona Li
Zhiqiang Fang
Changtai Zhao
Jianwen Liang
Solid-electrolyte interphases for all-solid-state batteries
ChemPhysMater
All-solid-state lithium batteries
Interfacial engineering
Solid-electrolyte interphase
Atomic layer deposition
Sol-gel
Mechanical ball-milling
title Solid-electrolyte interphases for all-solid-state batteries
title_full Solid-electrolyte interphases for all-solid-state batteries
title_fullStr Solid-electrolyte interphases for all-solid-state batteries
title_full_unstemmed Solid-electrolyte interphases for all-solid-state batteries
title_short Solid-electrolyte interphases for all-solid-state batteries
title_sort solid electrolyte interphases for all solid state batteries
topic All-solid-state lithium batteries
Interfacial engineering
Solid-electrolyte interphase
Atomic layer deposition
Sol-gel
Mechanical ball-milling
url http://www.sciencedirect.com/science/article/pii/S2772571524000597
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