Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor

Abstract Perfluorinated compounds (PFCs) are emerging environmental pollutants characterized by their extreme stability and resistance to degradation. Among them, tetrafluoromethane (CF4) is the simplest and most abundant PFC in the atmosphere. However, the highest C─F bond energy and its highly sym...

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Main Authors: Jialin Zheng, Xiaojian Wang, Xin Zi, Hang Zhang, Heping Chen, Evangelina Pensa, Kang Liu, Junwei Fu, Zhang Lin, Liyuan Chai, Emiliano Cortés, Min Liu
Format: Article
Language:English
Published: Wiley 2025-03-01
Series:Advanced Science
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Online Access:https://doi.org/10.1002/advs.202413203
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author Jialin Zheng
Xiaojian Wang
Xin Zi
Hang Zhang
Heping Chen
Evangelina Pensa
Kang Liu
Junwei Fu
Zhang Lin
Liyuan Chai
Emiliano Cortés
Min Liu
author_facet Jialin Zheng
Xiaojian Wang
Xin Zi
Hang Zhang
Heping Chen
Evangelina Pensa
Kang Liu
Junwei Fu
Zhang Lin
Liyuan Chai
Emiliano Cortés
Min Liu
author_sort Jialin Zheng
collection DOAJ
description Abstract Perfluorinated compounds (PFCs) are emerging environmental pollutants characterized by their extreme stability and resistance to degradation. Among them, tetrafluoromethane (CF4) is the simplest and most abundant PFC in the atmosphere. However, the highest C─F bond energy and its highly symmetrical structure make it particularly challenging to decompose. In this work, a yolk–shell Al2O3 micro‐reactor is developed to enhance the catalytic hydrolysis performance of CF4 by creating a local autothermic environment. Finite element simulations predict that the yolk–shell Al2O3 micro‐reactor captures the heat released during the catalytic hydrolysis of CF4, resulting in a local autothermic environment within the yolk–shell structure that is 50 °C higher than the set temperature. The effectiveness of this local autothermic environment is experimentally confirmed by in situ Raman spectroscopy. As a result, the obtained yolk–shell Al2O3 micro‐reactor achieves 100% CF4 conversion at a considerably low temperature of 580 °C for over 150 h, while hollow and solid Al2O3 structures required higher temperatures of 610 and 630 °C, respectively, to achieve the same conversion rate, demonstrating the potential of yolk–shell Al2O3 micro‐reactor to significantly reduce the energy requirements for PFCs degradation and contribute to more sustainable and effective environmental remediation strategies.
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institution Kabale University
issn 2198-3844
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spelling doaj-art-202e5da76b444509bb02d831751becfe2025-08-20T03:32:24ZengWileyAdvanced Science2198-38442025-03-01129n/an/a10.1002/advs.202413203Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐ReactorJialin Zheng0Xiaojian Wang1Xin Zi2Hang Zhang3Heping Chen4Evangelina Pensa5Kang Liu6Junwei Fu7Zhang Lin8Liyuan Chai9Emiliano Cortés10Min Liu11Hunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaHunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaHunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaHunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaSchool of Resource Environment and Safety Engineering University of South China Hengyang Hunan 421001 P. R. ChinaNanoinstitute Munich Faculty of Physics Ludwig‐Maximilians‐Universität München 80539 München GermanyHunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaHunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaSchool of Metallurgy and Environment Central South University Changsha Hunan 410083 P. R. ChinaSchool of Metallurgy and Environment Central South University Changsha Hunan 410083 P. R. ChinaNanoinstitute Munich Faculty of Physics Ludwig‐Maximilians‐Universität München 80539 München GermanyHunan Joint International Research Center for Carbon Dioxide Resource Utilization School of Physics Central South University Changsha Hunan 410083 P. R. ChinaAbstract Perfluorinated compounds (PFCs) are emerging environmental pollutants characterized by their extreme stability and resistance to degradation. Among them, tetrafluoromethane (CF4) is the simplest and most abundant PFC in the atmosphere. However, the highest C─F bond energy and its highly symmetrical structure make it particularly challenging to decompose. In this work, a yolk–shell Al2O3 micro‐reactor is developed to enhance the catalytic hydrolysis performance of CF4 by creating a local autothermic environment. Finite element simulations predict that the yolk–shell Al2O3 micro‐reactor captures the heat released during the catalytic hydrolysis of CF4, resulting in a local autothermic environment within the yolk–shell structure that is 50 °C higher than the set temperature. The effectiveness of this local autothermic environment is experimentally confirmed by in situ Raman spectroscopy. As a result, the obtained yolk–shell Al2O3 micro‐reactor achieves 100% CF4 conversion at a considerably low temperature of 580 °C for over 150 h, while hollow and solid Al2O3 structures required higher temperatures of 610 and 630 °C, respectively, to achieve the same conversion rate, demonstrating the potential of yolk–shell Al2O3 micro‐reactor to significantly reduce the energy requirements for PFCs degradation and contribute to more sustainable and effective environmental remediation strategies.https://doi.org/10.1002/advs.202413203catalytic hydrolysisenvironmental chemistryperfluorocarbonsthermal effectsyolk–shell
spellingShingle Jialin Zheng
Xiaojian Wang
Xin Zi
Hang Zhang
Heping Chen
Evangelina Pensa
Kang Liu
Junwei Fu
Zhang Lin
Liyuan Chai
Emiliano Cortés
Min Liu
Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor
Advanced Science
catalytic hydrolysis
environmental chemistry
perfluorocarbons
thermal effects
yolk–shell
title Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor
title_full Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor
title_fullStr Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor
title_full_unstemmed Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor
title_short Catalytic Hydrolysis of Perfluorinated Compounds in a Yolk–Shell Micro‐Reactor
title_sort catalytic hydrolysis of perfluorinated compounds in a yolk shell micro reactor
topic catalytic hydrolysis
environmental chemistry
perfluorocarbons
thermal effects
yolk–shell
url https://doi.org/10.1002/advs.202413203
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