Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione

The title molecule, C25H23BrN2O2, adopts a cup shaped conformation with the distinctly ruffled imidazolidine ring as the base. In the crystal, weak C—H...O hydrogen bonds and C—H...π(ring) interactions form helical chains of molecules extending along the b-axis direction that are linked by additiona...

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Main Authors: Houda Lamssane, Amal Haoudi, Badr Eddine Kartah, Ahmed Mazzah, Joel T. Mague, Tuncer Hökelek, Youssef Kandri Rodi, Nada Kheira Sebbar
Format: Article
Language:English
Published: International Union of Crystallography 2024-11-01
Series:Acta Crystallographica Section E: Crystallographic Communications
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Online Access:https://journals.iucr.org/paper?S2056989024009228
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author Houda Lamssane
Amal Haoudi
Badr Eddine Kartah
Ahmed Mazzah
Joel T. Mague
Tuncer Hökelek
Youssef Kandri Rodi
Nada Kheira Sebbar
author_facet Houda Lamssane
Amal Haoudi
Badr Eddine Kartah
Ahmed Mazzah
Joel T. Mague
Tuncer Hökelek
Youssef Kandri Rodi
Nada Kheira Sebbar
author_sort Houda Lamssane
collection DOAJ
description The title molecule, C25H23BrN2O2, adopts a cup shaped conformation with the distinctly ruffled imidazolidine ring as the base. In the crystal, weak C—H...O hydrogen bonds and C—H...π(ring) interactions form helical chains of molecules extending along the b-axis direction that are linked by additional weak C—H...π(ring) interactions across inversion centres. The Hirshfeld surface analysis of the crystal structure indicates that the most important contributions for the crystal packing are from H...H (51.0%), C...H/H...C (21.3%), Br...H/H...Br (12.8%) and O...H/H...O (12.4%) interactions. The volume of the crystal voids and the percentage of free space were calculated to be 251.24 Å3 and 11.71%, respectively, showing that there is no large cavity in the crystal packing. Evaluation of the electrostatic, dispersion and total energy frameworks indicate that the stabilization is dominated by the dispersion energy.
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spelling doaj-art-1fad772aa4934f3aa8c6cf981dbf02fc2025-08-20T02:26:40ZengInternational Union of CrystallographyActa Crystallographica Section E: Crystallographic Communications2056-98902024-11-0180111118112410.1107/S2056989024009228jy2051Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dioneHouda Lamssane0Amal Haoudi1Badr Eddine Kartah2Ahmed Mazzah3Joel T. Mague4Tuncer Hökelek5Youssef Kandri Rodi6Nada Kheira Sebbar7Laboratory of Applied Organic Chemistry, Sidi Mohamed Ben Abdellah University, Faculty Of Science And Technology, Road Immouzer, BP 2202 Fez, MoroccoLaboratory of Applied Organic Chemistry, Sidi Mohamed Ben Abdellah University, Faculty Of Science And Technology, Road Immouzer, BP 2202 Fez, MoroccoLaboratory of Plant Chemistry, Organic and Bioorganic Synthesis, Faculty of Sciences, Mohammed V University in Rabat, 4 Avenue Ibn Battouta BP 1014 RP, MoroccoScience and Technology of Lille USR 3290, Villeneuve d'ascq cedex, FranceDepartment of Chemistry, Tulane University, New Orleans, LA 70118, USADepartment of Physics, Hacettepe University, 06800 Beytepe, Ankara, TürkiyeLaboratory of Applied Organic Chemistry, Sidi Mohamed Ben Abdellah University, Faculty Of Science And Technology, Road Immouzer, BP 2202 Fez, MoroccoLaboratory of Plant Chemistry, Organic and Bioorganic Synthesis, Faculty of Sciences, Mohammed V University in Rabat, 4 Avenue Ibn Battouta BP 1014 RP, MoroccoThe title molecule, C25H23BrN2O2, adopts a cup shaped conformation with the distinctly ruffled imidazolidine ring as the base. In the crystal, weak C—H...O hydrogen bonds and C—H...π(ring) interactions form helical chains of molecules extending along the b-axis direction that are linked by additional weak C—H...π(ring) interactions across inversion centres. The Hirshfeld surface analysis of the crystal structure indicates that the most important contributions for the crystal packing are from H...H (51.0%), C...H/H...C (21.3%), Br...H/H...Br (12.8%) and O...H/H...O (12.4%) interactions. The volume of the crystal voids and the percentage of free space were calculated to be 251.24 Å3 and 11.71%, respectively, showing that there is no large cavity in the crystal packing. Evaluation of the electrostatic, dispersion and total energy frameworks indicate that the stabilization is dominated by the dispersion energy.https://journals.iucr.org/paper?S2056989024009228crystal structureimidazolidinec—h...π(ring) interactionhydrogen bondhirshfeld surface
spellingShingle Houda Lamssane
Amal Haoudi
Badr Eddine Kartah
Ahmed Mazzah
Joel T. Mague
Tuncer Hökelek
Youssef Kandri Rodi
Nada Kheira Sebbar
Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione
Acta Crystallographica Section E: Crystallographic Communications
crystal structure
imidazolidine
c—h...π(ring) interaction
hydrogen bond
hirshfeld surface
title Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione
title_full Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione
title_fullStr Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione
title_full_unstemmed Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione
title_short Crystal structure and Hirshfeld surface analyses, crystal voids, intermolecular interaction energies and energy frameworks of 3-benzyl-1-(3-bromopropyl)-5,5-diphenylimidazolidine-2,4-dione
title_sort crystal structure and hirshfeld surface analyses crystal voids intermolecular interaction energies and energy frameworks of 3 benzyl 1 3 bromopropyl 5 5 diphenylimidazolidine 2 4 dione
topic crystal structure
imidazolidine
c—h...π(ring) interaction
hydrogen bond
hirshfeld surface
url https://journals.iucr.org/paper?S2056989024009228
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