Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis

Spinel oxide Sr0.5Zn0.5Mn2O4 powder was successfully synthesized using the ultrasonic process. A comprehensive characterization was conducted employing various analytical techniques, including X-ray diffraction (XRD), infrared spectroscopy (IR), UV-Vis spectroscopy, scanning electron microscopy (SEM...

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Main Authors: Benyahia Khawla, Badaoui Mohamed, Sehil Hafida, Chougui Abdelkader, Mourad Abdel-Hamid I., Grira Soumaya, Dehbi Abdelkader
Format: Article
Language:English
Published: University of Novi Sad 2025-06-01
Series:Processing and Application of Ceramics
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Online Access:https://doiserbia.nb.rs/img/doi/1820-6131/2025/1820-61312502179B.pdf
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author Benyahia Khawla
Badaoui Mohamed
Sehil Hafida
Chougui Abdelkader
Mourad Abdel-Hamid I.
Grira Soumaya
Dehbi Abdelkader
author_facet Benyahia Khawla
Badaoui Mohamed
Sehil Hafida
Chougui Abdelkader
Mourad Abdel-Hamid I.
Grira Soumaya
Dehbi Abdelkader
author_sort Benyahia Khawla
collection DOAJ
description Spinel oxide Sr0.5Zn0.5Mn2O4 powder was successfully synthesized using the ultrasonic process. A comprehensive characterization was conducted employing various analytical techniques, including X-ray diffraction (XRD), infrared spectroscopy (IR), UV-Vis spectroscopy, scanning electron microscopy (SEM), thermogravimetric analysis, energy-dispersive X-ray spectroscopy and point of zero charge measurements. The results of IR analysis confirmed the presence of Zn-O, Sr-O and Mn-O bonds, which are crucial for the structural integrity of the material. The XRD patterns showed enhanced crystallinity, while the band gap energy was determined to be 2.5 eV, as corroborated by UV-Vis spectroscopy. Additionally, the SEM analysis revealed that the particles exhibited uniformity in both size and shape, which is essential for consistent photocatalytic performance. Furthermore, the Sr0.5Zn0.5Mn2O4 was evaluated for its photocatalytic activity, specifically targeting the degradation of Congo red dye under visible light irradiation. The findings of the photocatalytic study demonstrated a significant improvement in degradation efficiency (99.37%), highlighting the potential application of Sr0.5Zn0.5Mn2O4 in environmental remediation. A detailed study on the influence of various parameters, including pH, the amount of catalyst and the initial concentration of dye was also conducted to optimize the photocatalytic process.
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spelling doaj-art-1e8e664833e44740a2d7fe9cc6e2919e2025-08-20T03:14:10ZengUniversity of Novi SadProcessing and Application of Ceramics1820-61312406-10342025-06-0119217918910.2298/PAC2502179BSynthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysisBenyahia Khawla0https://orcid.org/0009-0009-8800-6282Badaoui Mohamed1https://orcid.org/0000-0001-7455-7184Sehil Hafida2https://orcid.org/0009-0002-5773-8295Chougui Abdelkader3Mourad Abdel-Hamid I.4https://orcid.org/0000-0002-8356-0542Grira Soumaya5https://orcid.org/0000-0002-9989-8361Dehbi Abdelkader6Synthesis and Catalysis Laboratory, University of Tiaret, Zaaroura, Tiaret, AlgeriaSynthesis and Catalysis Laboratory, University of Tiaret, Zaaroura, Tiaret, AlgeriaDepartment of Chemistry, Faculty of Sciences of the Matter, University of Tiaret, Zaaroura, Tiaret, AlgeriaDepartment of Sciences and Technologies, Faculty of Applied Science, University of Tiaret, AlgeriaMechanical and Aerospace Engineering Department, United Arab Emirates University, Al-Ain, UAE + National Water and Energy Center, United Arab Emirates University, Al-Ain, UAEChemical and Petroleum Engineering Department, United Arab Emirates University, Al-Ain, UAEEngineering Physics Laboratory, University of Tiaret, Tiaret, AlgeriaSpinel oxide Sr0.5Zn0.5Mn2O4 powder was successfully synthesized using the ultrasonic process. A comprehensive characterization was conducted employing various analytical techniques, including X-ray diffraction (XRD), infrared spectroscopy (IR), UV-Vis spectroscopy, scanning electron microscopy (SEM), thermogravimetric analysis, energy-dispersive X-ray spectroscopy and point of zero charge measurements. The results of IR analysis confirmed the presence of Zn-O, Sr-O and Mn-O bonds, which are crucial for the structural integrity of the material. The XRD patterns showed enhanced crystallinity, while the band gap energy was determined to be 2.5 eV, as corroborated by UV-Vis spectroscopy. Additionally, the SEM analysis revealed that the particles exhibited uniformity in both size and shape, which is essential for consistent photocatalytic performance. Furthermore, the Sr0.5Zn0.5Mn2O4 was evaluated for its photocatalytic activity, specifically targeting the degradation of Congo red dye under visible light irradiation. The findings of the photocatalytic study demonstrated a significant improvement in degradation efficiency (99.37%), highlighting the potential application of Sr0.5Zn0.5Mn2O4 in environmental remediation. A detailed study on the influence of various parameters, including pH, the amount of catalyst and the initial concentration of dye was also conducted to optimize the photocatalytic process.https://doiserbia.nb.rs/img/doi/1820-6131/2025/1820-61312502179B.pdfsr0.5zn0.5mn2o4 powderultrasonic methodstructurephotocatalysisdegradationcongo red
spellingShingle Benyahia Khawla
Badaoui Mohamed
Sehil Hafida
Chougui Abdelkader
Mourad Abdel-Hamid I.
Grira Soumaya
Dehbi Abdelkader
Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis
Processing and Application of Ceramics
sr0.5zn0.5mn2o4 powder
ultrasonic method
structure
photocatalysis
degradation
congo red
title Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis
title_full Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis
title_fullStr Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis
title_full_unstemmed Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis
title_short Synthesis and characterization of Sr0.5Zn0.5Mn2O4 powder for highly efficient visible light photocatalysis
title_sort synthesis and characterization of sr0 5zn0 5mn2o4 powder for highly efficient visible light photocatalysis
topic sr0.5zn0.5mn2o4 powder
ultrasonic method
structure
photocatalysis
degradation
congo red
url https://doiserbia.nb.rs/img/doi/1820-6131/2025/1820-61312502179B.pdf
work_keys_str_mv AT benyahiakhawla synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis
AT badaouimohamed synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis
AT sehilhafida synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis
AT chouguiabdelkader synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis
AT mouradabdelhamidi synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis
AT grirasoumaya synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis
AT dehbiabdelkader synthesisandcharacterizationofsr05zn05mn2o4powderforhighlyefficientvisiblelightphotocatalysis