Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction

Increased levels of reactive oxygen species (ROS) are a hallmark of cardiovascular disease. ROS impact the function of proteins largely through thiol modification leading to redox signalling. Acute, targeted interference with local ROS levels has been difficult. Therefore, how dynamics in redox sign...

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Main Authors: Melina Lopez, Niklas Herrle, Bardia Amirmiran, Pedro F. Malacarne, Julia Werkhäuser, Souradeep Chatterjee, Carine Kader, Victoria Jurisch, Xin Wen, Maedeh Gheisari, Katrin Schäfer, Christian Münch, Florian Leuschner, Ralf Gilsbach, Flávia Rezende, Ralf P. Brandes
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Antioxidants
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Online Access:https://www.mdpi.com/2076-3921/14/6/705
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author Melina Lopez
Niklas Herrle
Bardia Amirmiran
Pedro F. Malacarne
Julia Werkhäuser
Souradeep Chatterjee
Carine Kader
Victoria Jurisch
Xin Wen
Maedeh Gheisari
Katrin Schäfer
Christian Münch
Florian Leuschner
Ralf Gilsbach
Flávia Rezende
Ralf P. Brandes
author_facet Melina Lopez
Niklas Herrle
Bardia Amirmiran
Pedro F. Malacarne
Julia Werkhäuser
Souradeep Chatterjee
Carine Kader
Victoria Jurisch
Xin Wen
Maedeh Gheisari
Katrin Schäfer
Christian Münch
Florian Leuschner
Ralf Gilsbach
Flávia Rezende
Ralf P. Brandes
author_sort Melina Lopez
collection DOAJ
description Increased levels of reactive oxygen species (ROS) are a hallmark of cardiovascular disease. ROS impact the function of proteins largely through thiol modification leading to redox signalling. Acute, targeted interference with local ROS levels has been difficult. Therefore, how dynamics in redox signalling impact cardiovascular health is still a matter of current research. An inducible, endothelial cell-specific knock-in mouse model expressing a yeast D-amino acid oxidase enzyme was generated (Hipp11-Flox-Stop-Flox-yDAO-Cdh5-CreERT2<sup>+/0</sup> referred to as ecDAO). DAO releases H<sub>2</sub>O<sub>2</sub> as a by-product of the conversion of D-amino acids into imino acids. The D-amino acid treatment of DAO-expressing cells therefore increases their intracellular H<sub>2</sub>O<sub>2</sub> production. The induction of yDAO in the ecDAO mice was performed with tamoxifen. Subsequently, the mice received D-Alanine (D-Ala, 0.5 M) through drinking water, and the effects on ROS production and vascular and cardiac function were determined. ecDAO induction increased endothelial ROS production as well as ROS production in the lung, which is rich in endothelial cells. The functional consequences of this were, however limited: After minimally invasive myocardial infarction, there was no difference in the outcome between the control (CTL) and ecDAO mice. With respect to vascular function, three days of D-Ala slightly improved vascular function as demonstrated by an increase in the diameter of the carotid artery in vivo and decreased vessel constriction to phenylephrine. Fifty-two days of D-Ala induced cardiac remodelling, increased peripheral resistance, and overoxidation of peroxiredoxins. In conclusion, acute stimulation of endothelial ROS improves cardiovascular function, whereas prolonged ROS exposure deteriorates it.
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spelling doaj-art-1e052c8a687e4004a23d01aef311c09c2025-08-20T02:24:17ZengMDPI AGAntioxidants2076-39212025-06-0114670510.3390/antiox14060705Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular DysfunctionMelina Lopez0Niklas Herrle1Bardia Amirmiran2Pedro F. Malacarne3Julia Werkhäuser4Souradeep Chatterjee5Carine Kader6Victoria Jurisch7Xin Wen8Maedeh Gheisari9Katrin Schäfer10Christian Münch11Florian Leuschner12Ralf Gilsbach13Flávia Rezende14Ralf P. Brandes15Institute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyDepartment of Cardiology, University Medical Center Mainz, 55131 Mainz, GermanyInstitute of Molecular Systems Medicine, Goethe University, 60438 Frankfurt am Main, GermanyDepartment of Cardiology, Angiology and Pulmonology, University Hospital Heidelberg, 69118 Heidelberg, GermanyGerman Centre of Cardiovascular Research (DZHK), Partner Site Heidelberg/Mannheim, 69120 Heidelberg, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyInstitute for Cardiovascular Physiology, Goethe University, 60590 Frankfurt am Main, GermanyIncreased levels of reactive oxygen species (ROS) are a hallmark of cardiovascular disease. ROS impact the function of proteins largely through thiol modification leading to redox signalling. Acute, targeted interference with local ROS levels has been difficult. Therefore, how dynamics in redox signalling impact cardiovascular health is still a matter of current research. An inducible, endothelial cell-specific knock-in mouse model expressing a yeast D-amino acid oxidase enzyme was generated (Hipp11-Flox-Stop-Flox-yDAO-Cdh5-CreERT2<sup>+/0</sup> referred to as ecDAO). DAO releases H<sub>2</sub>O<sub>2</sub> as a by-product of the conversion of D-amino acids into imino acids. The D-amino acid treatment of DAO-expressing cells therefore increases their intracellular H<sub>2</sub>O<sub>2</sub> production. The induction of yDAO in the ecDAO mice was performed with tamoxifen. Subsequently, the mice received D-Alanine (D-Ala, 0.5 M) through drinking water, and the effects on ROS production and vascular and cardiac function were determined. ecDAO induction increased endothelial ROS production as well as ROS production in the lung, which is rich in endothelial cells. The functional consequences of this were, however limited: After minimally invasive myocardial infarction, there was no difference in the outcome between the control (CTL) and ecDAO mice. With respect to vascular function, three days of D-Ala slightly improved vascular function as demonstrated by an increase in the diameter of the carotid artery in vivo and decreased vessel constriction to phenylephrine. Fifty-two days of D-Ala induced cardiac remodelling, increased peripheral resistance, and overoxidation of peroxiredoxins. In conclusion, acute stimulation of endothelial ROS improves cardiovascular function, whereas prolonged ROS exposure deteriorates it.https://www.mdpi.com/2076-3921/14/6/705D-amino acid oxidasechemogeneticoxidative stressreactive oxygen speciesendothelial cellsmyocardial infarction
spellingShingle Melina Lopez
Niklas Herrle
Bardia Amirmiran
Pedro F. Malacarne
Julia Werkhäuser
Souradeep Chatterjee
Carine Kader
Victoria Jurisch
Xin Wen
Maedeh Gheisari
Katrin Schäfer
Christian Münch
Florian Leuschner
Ralf Gilsbach
Flávia Rezende
Ralf P. Brandes
Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction
Antioxidants
D-amino acid oxidase
chemogenetic
oxidative stress
reactive oxygen species
endothelial cells
myocardial infarction
title Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction
title_full Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction
title_fullStr Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction
title_full_unstemmed Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction
title_short Prolonged In Vivo Chemogenetic Generation of Hydrogen Peroxide by Endothelial Cells Induces Cardiac Remodelling and Vascular Dysfunction
title_sort prolonged in vivo chemogenetic generation of hydrogen peroxide by endothelial cells induces cardiac remodelling and vascular dysfunction
topic D-amino acid oxidase
chemogenetic
oxidative stress
reactive oxygen species
endothelial cells
myocardial infarction
url https://www.mdpi.com/2076-3921/14/6/705
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