Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite

In this study, Fe-doped copper oxide nanostructures (CF8O) and their chitosan-based composites (CF8O-Cs) were synthesized via a hydrothermal method and systematically characterized for biomedical applications. Comprehensive structural and morphological analyses (XRD, EDX, FESEM) established the form...

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Main Authors: H. Khaleghi, S. Alamdari, A. Ehsani, M.H. Ehsani
Format: Article
Language:English
Published: Elsevier 2025-09-01
Series:Results in Physics
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Online Access:http://www.sciencedirect.com/science/article/pii/S2211379725002876
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author H. Khaleghi
S. Alamdari
A. Ehsani
M.H. Ehsani
author_facet H. Khaleghi
S. Alamdari
A. Ehsani
M.H. Ehsani
author_sort H. Khaleghi
collection DOAJ
description In this study, Fe-doped copper oxide nanostructures (CF8O) and their chitosan-based composites (CF8O-Cs) were synthesized via a hydrothermal method and systematically characterized for biomedical applications. Comprehensive structural and morphological analyses (XRD, EDX, FESEM) established the formation of monoclinic-phase CuO nanosheets. Brunauer–Emmett–Teller (BET) analysis revealed that Fe doping significantly increases the surface area and pore volume of CuO, favoring greater nitrogen adsorption. Antibacterial activity was assessed against representative Gram-positive (Staphylococcus aureus) and Gram-negative (Escherichia coli) bacteria using viable cell counting. Pristine CF8O nanosheets exhibited potent, broad-spectrum bactericidal effects, while the chitosan-functionalized CF8O-Cs composite showed selective and enhanced activity against S. aureus but diminished efficacy against E. coli. Cytocompatibility, evaluated via MTT assay on L929 fibroblasts, demonstrated that Fe doping reduces the cytotoxicity of CuO nanoparticles compared to undoped counterparts. These results suggest that Fe-doped CuO and its chitosan composites offer tunable antibacterial performance and improved biocompatibility, supporting their promise for future biomedical and antimicrobial applications.
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spelling doaj-art-1c715b00ffd64370a7df5daf7682c1d02025-08-20T03:41:40ZengElsevierResults in Physics2211-37972025-09-017610839310.1016/j.rinp.2025.108393Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocompositeH. Khaleghi0S. Alamdari1A. Ehsani2M.H. Ehsani3Department of Basic Sciences, Semnan Branch, Islamic Azad University, Semnan, IranDepartment of Nanotechnology, Faculty of New Sciences and Technologies, Semnan University, Semnan, IranSchool of Medicine, Semnan University of Medical Sciences, Semnan, IranFaculty of Physics, Semnan University, PO Box: 35195-363, Semnan, Iran; Corresponding author.In this study, Fe-doped copper oxide nanostructures (CF8O) and their chitosan-based composites (CF8O-Cs) were synthesized via a hydrothermal method and systematically characterized for biomedical applications. Comprehensive structural and morphological analyses (XRD, EDX, FESEM) established the formation of monoclinic-phase CuO nanosheets. Brunauer–Emmett–Teller (BET) analysis revealed that Fe doping significantly increases the surface area and pore volume of CuO, favoring greater nitrogen adsorption. Antibacterial activity was assessed against representative Gram-positive (Staphylococcus aureus) and Gram-negative (Escherichia coli) bacteria using viable cell counting. Pristine CF8O nanosheets exhibited potent, broad-spectrum bactericidal effects, while the chitosan-functionalized CF8O-Cs composite showed selective and enhanced activity against S. aureus but diminished efficacy against E. coli. Cytocompatibility, evaluated via MTT assay on L929 fibroblasts, demonstrated that Fe doping reduces the cytotoxicity of CuO nanoparticles compared to undoped counterparts. These results suggest that Fe-doped CuO and its chitosan composites offer tunable antibacterial performance and improved biocompatibility, supporting their promise for future biomedical and antimicrobial applications.http://www.sciencedirect.com/science/article/pii/S2211379725002876Fe-doped in CuO NsHydrothermal synthesisNanocompositeAntibacterial activityCytocompatibility
spellingShingle H. Khaleghi
S. Alamdari
A. Ehsani
M.H. Ehsani
Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite
Results in Physics
Fe-doped in CuO Ns
Hydrothermal synthesis
Nanocomposite
Antibacterial activity
Cytocompatibility
title Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite
title_full Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite
title_fullStr Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite
title_full_unstemmed Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite
title_short Hydrothermal synthesis, structural characterization, and biological evaluation of Fe-doped CuO nanosheets and their chitosan nanocomposite
title_sort hydrothermal synthesis structural characterization and biological evaluation of fe doped cuo nanosheets and their chitosan nanocomposite
topic Fe-doped in CuO Ns
Hydrothermal synthesis
Nanocomposite
Antibacterial activity
Cytocompatibility
url http://www.sciencedirect.com/science/article/pii/S2211379725002876
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AT salamdari hydrothermalsynthesisstructuralcharacterizationandbiologicalevaluationoffedopedcuonanosheetsandtheirchitosannanocomposite
AT aehsani hydrothermalsynthesisstructuralcharacterizationandbiologicalevaluationoffedopedcuonanosheetsandtheirchitosannanocomposite
AT mhehsani hydrothermalsynthesisstructuralcharacterizationandbiologicalevaluationoffedopedcuonanosheetsandtheirchitosannanocomposite