Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA

To assess the potential cytostatic properties of the thulium(III)-arsenazo III complex as a probe of rare earth complex antitumor drugs, the interaction information of the thulium(III)-arsenazo III complex with DNA was obtained by using spectroscopy, viscosity measurements, and voltammetric methods....

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Main Authors: Hongbo Li, Shutao Lei, Yongqiong Tang, Liyuan Zou, Hongqin Hu, Suqin Wang
Format: Article
Language:English
Published: Wiley 2018-01-01
Series:Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2018/7232793
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author Hongbo Li
Shutao Lei
Yongqiong Tang
Liyuan Zou
Hongqin Hu
Suqin Wang
author_facet Hongbo Li
Shutao Lei
Yongqiong Tang
Liyuan Zou
Hongqin Hu
Suqin Wang
author_sort Hongbo Li
collection DOAJ
description To assess the potential cytostatic properties of the thulium(III)-arsenazo III complex as a probe of rare earth complex antitumor drugs, the interaction information of the thulium(III)-arsenazo III complex with DNA was obtained by using spectroscopy, viscosity measurements, and voltammetric methods. The thermodynamic functions demonstrated that the binding constants of the thulium(III)-arsenazo III complex with DNA were Kθ298.15K = 4.84 × 106 L·mol−1 and Kθ308.15K = 4.48 × 106 L·mol−1, and the binding process was enthalpy driven. The increase in relative viscosity of DNA with the addition of the thulium(III)-arsenazo III complex and the results from Scatchard and voltammetric methods showed that the interaction mode between the thulium(III)-arsenazo III complex and DNA was groove binding along with weak intercalative binding.
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institution DOAJ
issn 2090-9063
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publisher Wiley
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series Journal of Chemistry
spelling doaj-art-1bd3be9c17894e3cb762845eb5287b862025-08-20T03:17:52ZengWileyJournal of Chemistry2090-90632090-90712018-01-01201810.1155/2018/72327937232793Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNAHongbo Li0Shutao Lei1Yongqiong Tang2Liyuan Zou3Hongqin Hu4Suqin Wang5Key Laboratory of Functional Small Organic Molecule, Ministry of Education, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, ChinaKey Laboratory of Functional Small Organic Molecule, Ministry of Education, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, ChinaKey Laboratory of Functional Small Organic Molecule, Ministry of Education, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, ChinaKey Laboratory of Functional Small Organic Molecule, Ministry of Education, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, ChinaKey Laboratory of Functional Small Organic Molecule, Ministry of Education, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, ChinaKey Laboratory of Functional Small Organic Molecule, Ministry of Education, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, ChinaTo assess the potential cytostatic properties of the thulium(III)-arsenazo III complex as a probe of rare earth complex antitumor drugs, the interaction information of the thulium(III)-arsenazo III complex with DNA was obtained by using spectroscopy, viscosity measurements, and voltammetric methods. The thermodynamic functions demonstrated that the binding constants of the thulium(III)-arsenazo III complex with DNA were Kθ298.15K = 4.84 × 106 L·mol−1 and Kθ308.15K = 4.48 × 106 L·mol−1, and the binding process was enthalpy driven. The increase in relative viscosity of DNA with the addition of the thulium(III)-arsenazo III complex and the results from Scatchard and voltammetric methods showed that the interaction mode between the thulium(III)-arsenazo III complex and DNA was groove binding along with weak intercalative binding.http://dx.doi.org/10.1155/2018/7232793
spellingShingle Hongbo Li
Shutao Lei
Yongqiong Tang
Liyuan Zou
Hongqin Hu
Suqin Wang
Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA
Journal of Chemistry
title Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA
title_full Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA
title_fullStr Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA
title_full_unstemmed Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA
title_short Drug Effect of Thulium(III)-Arsenazo III Complex on Herring Sperm DNA
title_sort drug effect of thulium iii arsenazo iii complex on herring sperm dna
url http://dx.doi.org/10.1155/2018/7232793
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AT yongqiongtang drugeffectofthuliumiiiarsenazoiiicomplexonherringspermdna
AT liyuanzou drugeffectofthuliumiiiarsenazoiiicomplexonherringspermdna
AT hongqinhu drugeffectofthuliumiiiarsenazoiiicomplexonherringspermdna
AT suqinwang drugeffectofthuliumiiiarsenazoiiicomplexonherringspermdna