Tip-enhanced Raman scattering of glucose molecules

Glucose molecules are of great significance being one of the most important molecules in metabolic chain. However, due to the small Raman scattering cross-section and weak/non-adsorption on bare metals, accurately obtaining their "fingerprint information" remains a huge obstacle. Herein, w...

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Bibliographic Details
Main Authors: Zhonglin Xie, Chao Meng, Donghua Yue, Lei Xu, Ting Mei, Wending Zhang
Format: Article
Language:English
Published: Editorial Office of Opto-Electronic Journals, Institute of Optics and Electronics, CAS, China 2025-05-01
Series:Opto-Electronic Science
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Online Access:https://www.oejournal.org/article/doi/10.29026/oes.2025.240027
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Summary:Glucose molecules are of great significance being one of the most important molecules in metabolic chain. However, due to the small Raman scattering cross-section and weak/non-adsorption on bare metals, accurately obtaining their "fingerprint information" remains a huge obstacle. Herein, we developed a tip-enhanced Raman scattering (TERS) technique to address this challenge. Adopting an optical fiber radial vector mode internally illuminates the plasmonic fiber tip to effectively suppress the background noise while generating a strong electric-field enhanced tip hotspot. Furthermore, the tip hotspot approaching the glucose molecules was manipulated via the shear-force feedback to provide more freedom for selecting substrates. Consequently, our TERS technique achieves the visualization of all Raman modes of glucose molecules within spectral window of 400–3200 cm−1, which is not achievable through the far-field/surface-enhanced Raman, or the existing TERS techniques. Our TERS technique offers a powerful tool for accurately identifying Raman scattering of molecules, paving the way for biomolecular analysis.
ISSN:2097-0382