Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer

Saliva has already proven to be a prospective diagnostic bioresource for both early disease detection and timely intervention due to its easy accessibility, noninvasiveness, and reproducibility. However, the in-depth identification of salivary proteins needs to be further improved. Until now, only 3...

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Main Authors: Lingling Jiao, Huilin Dong, Changjian Wu, Jing Liu, Chenhui Wang, Yi Cao, Fan Cao, Ying Zhu, Huaiyuan Zhu
Format: Article
Language:English
Published: Wiley 2025-01-01
Series:IET Nanobiotechnology
Online Access:http://dx.doi.org/10.1049/nbt2/6616433
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author Lingling Jiao
Huilin Dong
Changjian Wu
Jing Liu
Chenhui Wang
Yi Cao
Fan Cao
Ying Zhu
Huaiyuan Zhu
author_facet Lingling Jiao
Huilin Dong
Changjian Wu
Jing Liu
Chenhui Wang
Yi Cao
Fan Cao
Ying Zhu
Huaiyuan Zhu
author_sort Lingling Jiao
collection DOAJ
description Saliva has already proven to be a prospective diagnostic bioresource for both early disease detection and timely intervention due to its easy accessibility, noninvasiveness, and reproducibility. However, the in-depth identification of salivary proteins needs to be further improved. Until now, only 3427 proteins are included in the human salivary proteome (HSP), which is far from the millions of proteins that make up humans. Here, we set out to quantitatively map the HSP in rapid and in-depth Orbitrap Astral mass spectrometer (MS) and coronal nanomagnetic bead–based proteomics workflow. Our study reported 5937 salivary proteins, which was about 73% more than that recorded in HSP. Moreover, we compared the differences between the young and aged salivary proteins. The predominant functions of the upregulated proteins in the young were related to motor proteins and cardiomyopathy, whereas those of the aged were primarily upregulated with oxidation reaction, as well as neurodegenerative disorders. It is the first study to carry out salivary proteomics using a fast and deep Orbitrap Astral MS and remarkably enlarged the number of proteins with HSP, furthermore, salivary proteomics was found to be characterized in the young and aged. With the rapidly advancing MS and proteomics technologies, we believe that salivary protein biomarkers will be more promising for clinical diagnosis and prognosis of human diseases in the future.
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issn 1751-875X
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spelling doaj-art-1a3fbcb4ee304be2be9611882a1d20b32025-08-20T03:12:27ZengWileyIET Nanobiotechnology1751-875X2025-01-01202510.1049/nbt2/6616433Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass SpectrometerLingling Jiao0Huilin Dong1Changjian Wu2Jing Liu3Chenhui Wang4Yi Cao5Fan Cao6Ying Zhu7Huaiyuan Zhu8China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.China Tobacco Jiangsu Industrial Co. Ltd.Saliva has already proven to be a prospective diagnostic bioresource for both early disease detection and timely intervention due to its easy accessibility, noninvasiveness, and reproducibility. However, the in-depth identification of salivary proteins needs to be further improved. Until now, only 3427 proteins are included in the human salivary proteome (HSP), which is far from the millions of proteins that make up humans. Here, we set out to quantitatively map the HSP in rapid and in-depth Orbitrap Astral mass spectrometer (MS) and coronal nanomagnetic bead–based proteomics workflow. Our study reported 5937 salivary proteins, which was about 73% more than that recorded in HSP. Moreover, we compared the differences between the young and aged salivary proteins. The predominant functions of the upregulated proteins in the young were related to motor proteins and cardiomyopathy, whereas those of the aged were primarily upregulated with oxidation reaction, as well as neurodegenerative disorders. It is the first study to carry out salivary proteomics using a fast and deep Orbitrap Astral MS and remarkably enlarged the number of proteins with HSP, furthermore, salivary proteomics was found to be characterized in the young and aged. With the rapidly advancing MS and proteomics technologies, we believe that salivary protein biomarkers will be more promising for clinical diagnosis and prognosis of human diseases in the future.http://dx.doi.org/10.1049/nbt2/6616433
spellingShingle Lingling Jiao
Huilin Dong
Changjian Wu
Jing Liu
Chenhui Wang
Yi Cao
Fan Cao
Ying Zhu
Huaiyuan Zhu
Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer
IET Nanobiotechnology
title Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer
title_full Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer
title_fullStr Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer
title_full_unstemmed Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer
title_short Ultrafast and Deep Saliva Proteome Reveals the Dynamic of Human Saliva With Aging by Orbitrap Astral Mass Spectrometer
title_sort ultrafast and deep saliva proteome reveals the dynamic of human saliva with aging by orbitrap astral mass spectrometer
url http://dx.doi.org/10.1049/nbt2/6616433
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