Preparation and Performance Study of MXene-Regulated Ethylene Glycol-Induced WO<sub>3</sub> Film

This study introduces the development of a W-M<sub>1.0</sub> electrochromic film, characterized by a “coral”-like TiO<sub>2</sub>@WO<sub>3</sub> heterostructure, synthesized via a hydrothermal process leveraging the inherent instability of MXene. The film showcase...

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Bibliographic Details
Main Authors: Yuqi Wang, Yong Liu, Minmin Wang, Wenjun Wu, Maofei Tian, Tao Zhu
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Micromachines
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Online Access:https://www.mdpi.com/2072-666X/15/12/1486
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Summary:This study introduces the development of a W-M<sub>1.0</sub> electrochromic film, characterized by a “coral”-like TiO<sub>2</sub>@WO<sub>3</sub> heterostructure, synthesized via a hydrothermal process leveraging the inherent instability of MXene. The film showcases exceptional electrochromic performance, with a coloring response time of 2.8 s, a bleaching response time of 4.6 s, and a high coloring efficiency of 137.02 cm<sup>2</sup>C<sup>−1</sup>. It also demonstrates a superior light modulation ability of 73.83% at 1033 nm. Notably, the W-M<sub>1.0</sub> film exhibits remarkable cyclic stability, retaining over 90% of its initial light modulation capacity after 4000 cycles, outperforming many existing electrochromic materials. The film’s enhanced performance is credited to its coral-like structure, which boosts the specific surface area and promotes ion transport, and the TiO<sub>2</sub>@WO<sub>3</sub> heterojunctions, which enhance charge transfer and stabilize the material. Devices fabricated with the W-M<sub>1.0</sub> film as the cathode and a PB film as the anode exhibit a seamless transition from dark blue to colorless, underscoring their potential for smart window and dynamic glass applications.
ISSN:2072-666X