Efficient construction of a quinoline framework from alcohols, nitroarenes, and alkenes promoted by a trimetallic catalyst system

A Pd/Fe/In-trimetallic catalyst system promotes the three-component coupling reaction of primary alcohols, nitroarenes, and terminal alkenes to construct quinoline frameworks in a single operation. These consecutive coupling reactions proceed via an oxidative Povarov reaction of alkenes and aldimine...

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Bibliographic Details
Main Authors: Rikiya Horikawa, Gen Onodera, Tsutomu Fukuda, Masanari Kimura
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Tetrahedron Chem
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Online Access:http://www.sciencedirect.com/science/article/pii/S2666951X24000470
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Summary:A Pd/Fe/In-trimetallic catalyst system promotes the three-component coupling reaction of primary alcohols, nitroarenes, and terminal alkenes to construct quinoline frameworks in a single operation. These consecutive coupling reactions proceed via an oxidative Povarov reaction of alkenes and aldimines derived from primary alcohols and nitroarenes by a redox hydrogen transfer system. This reaction may contribute to the efficient development of pharmaceuticals and medicinal products.
ISSN:2666-951X