Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations

<b>Background/Objectives:</b> Hyperlipidemia is a silent threat lurking in the bloodstream of millions worldwide. The nano-based platform has emerged as a promising drug delivery technology. Repaglinide, an anti-diabetic drug, was investigated recently as an antihyperlipidemic candidate...

Full description

Saved in:
Bibliographic Details
Main Authors: Mennatullah M. Faisal, Eman Gomaa, Mohamed S. Attia, Rana M. Abdelnaby, Adel Ehab Ibrahim, Ahmed Al-Harrasi, Sami El Deeb, Al Zahraa G. Al Ashmawy
Format: Article
Language:English
Published: MDPI AG 2025-03-01
Series:Pharmaceutics
Subjects:
Online Access:https://www.mdpi.com/1999-4923/17/3/350
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850091344003858432
author Mennatullah M. Faisal
Eman Gomaa
Mohamed S. Attia
Rana M. Abdelnaby
Adel Ehab Ibrahim
Ahmed Al-Harrasi
Sami El Deeb
Al Zahraa G. Al Ashmawy
author_facet Mennatullah M. Faisal
Eman Gomaa
Mohamed S. Attia
Rana M. Abdelnaby
Adel Ehab Ibrahim
Ahmed Al-Harrasi
Sami El Deeb
Al Zahraa G. Al Ashmawy
author_sort Mennatullah M. Faisal
collection DOAJ
description <b>Background/Objectives:</b> Hyperlipidemia is a silent threat lurking in the bloodstream of millions worldwide. The nano-based platform has emerged as a promising drug delivery technology. Repaglinide, an anti-diabetic drug, was investigated recently as an antihyperlipidemic candidate that could supersede the available antihyperlipidemic drugs. Our goal was to optimize albumin-based nanoparticles loaded with Repaglinide for parenteral delivery and conduct in silico and in vivo studies to explore the efficacy of Repaglinide for the management of hyperlipidemia along with its anti-diabetic effect. <b>Methods:</b> The impact of three independent factors, the albumin%, acetone volume, and glutaraldehyde/albumin, on the particle size, zeta potential, and entrapment efficiency was investigated. <b>Results:</b> The optimized formulation was spherical, homogenous of an average diameter (~181.86 nm) with a narrow size distribution, a zeta potential of −24.26 mV, and 76.37% as the EE%. The in vitro release of Repaglinide from nanoparticles showed a sustained release pattern for 168 h, with an initial burst release after 24 h, and was fitted to the Fickian diffusion mechanism. A molecular docking simulation showed a strong affinity to several protein targets, and the results were very promising, where Repaglinide gave a score of −7.70 Kcal/mol compared to Mevastatin (−6.71 Kcal/mol) and Atorvastatin (−8.36 Kcal/mol). On conducting in vivo studies on animal models, the optimized formula recorded a statistically significant decrease in the serum levels of total cholesterol, triglyceride, and low-density lipoproteins, with an increased high-density lipoprotein. <b>Conclusions:</b> This study suggested albumin nanoparticles as potential nanocarriers for the parenteral delivery of Repaglinide to ameliorate its antihyperlipidemic benefits, especially in diabetic patients.
format Article
id doaj-art-17d1ea17104c4aebafe2c91b3b8d678f
institution DOAJ
issn 1999-4923
language English
publishDate 2025-03-01
publisher MDPI AG
record_format Article
series Pharmaceutics
spelling doaj-art-17d1ea17104c4aebafe2c91b3b8d678f2025-08-20T02:42:24ZengMDPI AGPharmaceutics1999-49232025-03-0117335010.3390/pharmaceutics17030350Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo EvaluationsMennatullah M. Faisal0Eman Gomaa1Mohamed S. Attia2Rana M. Abdelnaby3Adel Ehab Ibrahim4Ahmed Al-Harrasi5Sami El Deeb6Al Zahraa G. Al Ashmawy7Department of Pharmaceutics, Faculty of Pharmacy, Zagazig University, Zagazig 44519, EgyptDepartment of Pharmaceutics, Faculty of Pharmacy, Zagazig University, Zagazig 44519, EgyptDepartment of Pharmaceutics, Faculty of Pharmacy, Zagazig University, Zagazig 44519, EgyptDepartment Pharmaceutical Chemistry, Faculty of Pharmacy, Heliopolis University, Cairo 11785, EgyptNatural and Medical Sciences Research Center, University of Nizwa, Birkat Al Mauz, P.O. Box 33, Nizwa 616, OmanNatural and Medical Sciences Research Center, University of Nizwa, Birkat Al Mauz, P.O. Box 33, Nizwa 616, OmanInstitute of Medicinal and Pharmaceutical Chemistry, Technische Universität Braunschweig, 38106 Brunswick, GermanyDepartment of Pharmaceutics, Faculty of Pharmacy, El Saleheya El Gadida University, El Saleheya El Gadida 44813, Egypt<b>Background/Objectives:</b> Hyperlipidemia is a silent threat lurking in the bloodstream of millions worldwide. The nano-based platform has emerged as a promising drug delivery technology. Repaglinide, an anti-diabetic drug, was investigated recently as an antihyperlipidemic candidate that could supersede the available antihyperlipidemic drugs. Our goal was to optimize albumin-based nanoparticles loaded with Repaglinide for parenteral delivery and conduct in silico and in vivo studies to explore the efficacy of Repaglinide for the management of hyperlipidemia along with its anti-diabetic effect. <b>Methods:</b> The impact of three independent factors, the albumin%, acetone volume, and glutaraldehyde/albumin, on the particle size, zeta potential, and entrapment efficiency was investigated. <b>Results:</b> The optimized formulation was spherical, homogenous of an average diameter (~181.86 nm) with a narrow size distribution, a zeta potential of −24.26 mV, and 76.37% as the EE%. The in vitro release of Repaglinide from nanoparticles showed a sustained release pattern for 168 h, with an initial burst release after 24 h, and was fitted to the Fickian diffusion mechanism. A molecular docking simulation showed a strong affinity to several protein targets, and the results were very promising, where Repaglinide gave a score of −7.70 Kcal/mol compared to Mevastatin (−6.71 Kcal/mol) and Atorvastatin (−8.36 Kcal/mol). On conducting in vivo studies on animal models, the optimized formula recorded a statistically significant decrease in the serum levels of total cholesterol, triglyceride, and low-density lipoproteins, with an increased high-density lipoprotein. <b>Conclusions:</b> This study suggested albumin nanoparticles as potential nanocarriers for the parenteral delivery of Repaglinide to ameliorate its antihyperlipidemic benefits, especially in diabetic patients.https://www.mdpi.com/1999-4923/17/3/350factorial designatherosclerosisalbuminnanoparticlesin silicotriglycerides
spellingShingle Mennatullah M. Faisal
Eman Gomaa
Mohamed S. Attia
Rana M. Abdelnaby
Adel Ehab Ibrahim
Ahmed Al-Harrasi
Sami El Deeb
Al Zahraa G. Al Ashmawy
Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations
Pharmaceutics
factorial design
atherosclerosis
albumin
nanoparticles
in silico
triglycerides
title Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations
title_full Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations
title_fullStr Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations
title_full_unstemmed Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations
title_short Albumin-Based Nanoparticles with Factorial Design as a Promising Approach for Remodeled Repaglinide: Evidence from In Silico, In Vitro, and In Vivo Evaluations
title_sort albumin based nanoparticles with factorial design as a promising approach for remodeled repaglinide evidence from in silico in vitro and in vivo evaluations
topic factorial design
atherosclerosis
albumin
nanoparticles
in silico
triglycerides
url https://www.mdpi.com/1999-4923/17/3/350
work_keys_str_mv AT mennatullahmfaisal albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT emangomaa albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT mohamedsattia albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT ranamabdelnaby albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT adelehabibrahim albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT ahmedalharrasi albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT samieldeeb albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations
AT alzahraagalashmawy albuminbasednanoparticleswithfactorialdesignasapromisingapproachforremodeledrepaglinideevidencefrominsilicoinvitroandinvivoevaluations