Photo-Activated Carbon Dots as Catalysts in Knoevenagel Condensation: An Advance in the Synthetic Field

Photoinduced chemical reactions and the development of new materials represent a current and significant topic. We present a sustainable and eco-friendly approach to the Knoevenagel condensation reaction involving carbonyl and active methylene compounds. Our method utilizes photo-activated carbon do...

Full description

Saved in:
Bibliographic Details
Main Authors: Cinzia Michenzi, Francesca Scaramuzzo, Chiara Salvitti, Federico Pepi, Anna Troiani, Isabella Chiarotto
Format: Article
Language:English
Published: MDPI AG 2024-08-01
Series:Photochem
Subjects:
Online Access:https://www.mdpi.com/2673-7256/4/3/22
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:Photoinduced chemical reactions and the development of new materials represent a current and significant topic. We present a sustainable and eco-friendly approach to the Knoevenagel condensation reaction involving carbonyl and active methylene compounds. Our method utilizes photo-activated carbon dots (CDs) derived from 5-hydroxymethylfurfural (5HMF) within an aqueous medium and does not require acidic, basic, or thermal conditions. This protocol operates effectively with aromatic, aliphatic, and heteroaromatic aldehydes and ketones. The 5HMF-derived-CDs can be reused four times without significant loss of activity. Moreover, this methodology is suitable for scaling up reactions, thereby highlighting its potential for industrial applications.
ISSN:2673-7256