Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles

The specific electrical conductivity and dielectric constant of aqueous solutions of ionic aminopolysaccharide chitosan in L-aspartic acid were investigated. An increase of the mobility of charge carriers in these solutions was found in comparison with solutions of an individual acid. The evaluation...

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Main Authors: T. N. Lugovitskaya, A. B. Shipovskaya, X. M. Shipenok
Format: Article
Language:English
Published: Ural Federal University 2021-11-01
Series:Chimica Techno Acta
Subjects:
Online Access:https://chimicatechnoacta.ru/article/view/5394
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author T. N. Lugovitskaya
A. B. Shipovskaya
X. M. Shipenok
author_facet T. N. Lugovitskaya
A. B. Shipovskaya
X. M. Shipenok
author_sort T. N. Lugovitskaya
collection DOAJ
description The specific electrical conductivity and dielectric constant of aqueous solutions of ionic aminopolysaccharide chitosan in L-aspartic acid were investigated. An increase of the mobility of charge carriers in these solutions was found in comparison with solutions of an individual acid. The evaluation of the kinetic stability revealed that the viscosity, electrical conductivity and dielectric constant of the chitosan – L-aspartic acid – water system decrease, while the pH value increases. It was shown that the time variation of physicochemical and electrochemical parameters is due to the effects of counterionic association with the transition of macromolecules to the ionomeric state and is accompanied by phase segregation of the polymer phase in the form of nano- and microparticles. The conducted studies carried out have shown the fundamental possibility of controlling the metastable state of this system in order to obtain nano- and microparticles.
format Article
id doaj-art-15abeb00d1cb49698eb77c448a49f2e1
institution OA Journals
issn 2411-1414
language English
publishDate 2021-11-01
publisher Ural Federal University
record_format Article
series Chimica Techno Acta
spelling doaj-art-15abeb00d1cb49698eb77c448a49f2e12025-08-20T01:58:42ZengUral Federal UniversityChimica Techno Acta2411-14142021-11-018410.15826/chimtech.2021.8.4.054113Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticlesT. N. Lugovitskaya0A. B. Shipovskaya1X. M. Shipenok2Ural Federal State University named after the first President of Russia B. N. YeltsinSaratov National Research State University named after N.G. ChernyshevskySaratov National Research State University named after N.G. ChernyshevskyThe specific electrical conductivity and dielectric constant of aqueous solutions of ionic aminopolysaccharide chitosan in L-aspartic acid were investigated. An increase of the mobility of charge carriers in these solutions was found in comparison with solutions of an individual acid. The evaluation of the kinetic stability revealed that the viscosity, electrical conductivity and dielectric constant of the chitosan – L-aspartic acid – water system decrease, while the pH value increases. It was shown that the time variation of physicochemical and electrochemical parameters is due to the effects of counterionic association with the transition of macromolecules to the ionomeric state and is accompanied by phase segregation of the polymer phase in the form of nano- and microparticles. The conducted studies carried out have shown the fundamental possibility of controlling the metastable state of this system in order to obtain nano- and microparticles.https://chimicatechnoacta.ru/article/view/5394chitosanl-aspartic acidcounterionicassociationnanoparticles
spellingShingle T. N. Lugovitskaya
A. B. Shipovskaya
X. M. Shipenok
Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles
Chimica Techno Acta
chitosan
l-aspartic acid
counterionic
association
nanoparticles
title Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles
title_full Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles
title_fullStr Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles
title_full_unstemmed Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles
title_short Kinetic instability of a chitosan – aspartic acid – water system as a method for obtaining nano- and microparticles
title_sort kinetic instability of a chitosan aspartic acid water system as a method for obtaining nano and microparticles
topic chitosan
l-aspartic acid
counterionic
association
nanoparticles
url https://chimicatechnoacta.ru/article/view/5394
work_keys_str_mv AT tnlugovitskaya kineticinstabilityofachitosanasparticacidwatersystemasamethodforobtainingnanoandmicroparticles
AT abshipovskaya kineticinstabilityofachitosanasparticacidwatersystemasamethodforobtainingnanoandmicroparticles
AT xmshipenok kineticinstabilityofachitosanasparticacidwatersystemasamethodforobtainingnanoandmicroparticles