Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating

Abstract One of the most frequently used polymers in the galvanic industry as well as for Fused Filament Fabrication (FFF) is the terpolymer of acrylonitrile butadiene styrene (ABS). Its surface is etched in chromosulfuric acid to enable the chemical deposition of a metal. The use of chromium (Cr)(V...

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Main Authors: Philipp Zimmermann, Christoph Schammel, Jürgen Nagel
Format: Article
Language:English
Published: Wiley-VCH 2025-04-01
Series:Macromolecular Materials and Engineering
Subjects:
Online Access:https://doi.org/10.1002/mame.202400367
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author Philipp Zimmermann
Christoph Schammel
Jürgen Nagel
author_facet Philipp Zimmermann
Christoph Schammel
Jürgen Nagel
author_sort Philipp Zimmermann
collection DOAJ
description Abstract One of the most frequently used polymers in the galvanic industry as well as for Fused Filament Fabrication (FFF) is the terpolymer of acrylonitrile butadiene styrene (ABS). Its surface is etched in chromosulfuric acid to enable the chemical deposition of a metal. The use of chromium (Cr)(VI) compounds is restricted in the European Union (EU) since 2017. A new plating process is proposed here that does not rely on etching. Instead, double bonds on the ABS surface are converted to epoxides, followed by grafting of a polyethylenimine (PEI) to the surface. The so modified plastic is an ideal starting point for metal plating. Printing often leads to the formation of voids between strands and layers, which hinders subsequent wet processing. The plating process introduced here requires high demands on the water tightness of parts. The proposed printing procedure reduces the degree of penetration of water from 50% to less than 0.1% at 2 bar water pressure. The combination of the new printing procedure with the new plating process results in the deposition of industrial relevant nickel (Ni) layers. The cross‐hatch test followed by a peel test exhibits values of zero, pointing to the high adhesion of Ni to ABS.
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institution OA Journals
issn 1438-7492
1439-2054
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spelling doaj-art-15a562b3020e475887deb4a04d342f762025-08-20T02:15:52ZengWiley-VCHMacromolecular Materials and Engineering1438-74921439-20542025-04-013104n/an/a10.1002/mame.202400367Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal PlatingPhilipp Zimmermann0Christoph Schammel1Jürgen Nagel2Leibniz Institute of Polymer Research Dresden e.V. Hohe Straße 6 01069 Dresden GermanyLeibniz Institute of Polymer Research Dresden e.V. Hohe Straße 6 01069 Dresden GermanyLeibniz Institute of Polymer Research Dresden e.V. Hohe Straße 6 01069 Dresden GermanyAbstract One of the most frequently used polymers in the galvanic industry as well as for Fused Filament Fabrication (FFF) is the terpolymer of acrylonitrile butadiene styrene (ABS). Its surface is etched in chromosulfuric acid to enable the chemical deposition of a metal. The use of chromium (Cr)(VI) compounds is restricted in the European Union (EU) since 2017. A new plating process is proposed here that does not rely on etching. Instead, double bonds on the ABS surface are converted to epoxides, followed by grafting of a polyethylenimine (PEI) to the surface. The so modified plastic is an ideal starting point for metal plating. Printing often leads to the formation of voids between strands and layers, which hinders subsequent wet processing. The plating process introduced here requires high demands on the water tightness of parts. The proposed printing procedure reduces the degree of penetration of water from 50% to less than 0.1% at 2 bar water pressure. The combination of the new printing procedure with the new plating process results in the deposition of industrial relevant nickel (Ni) layers. The cross‐hatch test followed by a peel test exhibits values of zero, pointing to the high adhesion of Ni to ABS.https://doi.org/10.1002/mame.202400367ABSfused filament fabricationsmetal platingssurface voidswater tightness
spellingShingle Philipp Zimmermann
Christoph Schammel
Jürgen Nagel
Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating
Macromolecular Materials and Engineering
ABS
fused filament fabrications
metal platings
surface voids
water tightness
title Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating
title_full Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating
title_fullStr Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating
title_full_unstemmed Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating
title_short Additive Manufacturing of Watertight ABS Parts and Its Use for Chemical Metal Plating
title_sort additive manufacturing of watertight abs parts and its use for chemical metal plating
topic ABS
fused filament fabrications
metal platings
surface voids
water tightness
url https://doi.org/10.1002/mame.202400367
work_keys_str_mv AT philippzimmermann additivemanufacturingofwatertightabspartsanditsuseforchemicalmetalplating
AT christophschammel additivemanufacturingofwatertightabspartsanditsuseforchemicalmetalplating
AT jurgennagel additivemanufacturingofwatertightabspartsanditsuseforchemicalmetalplating