Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue

The calcium silicate hydrate synthesized from electrolytic manganese residue was investigated as adsorbents to remove the phosphate from aqueous solutions. The effects of different experimental parameters, including contact time, initial phosphate concentration, solution pH, and temperature on the p...

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Main Authors: Changxin Li, Yuan Yu, Qiuyue Li, Hong Zhong, Shuai Wang
Format: Article
Language:English
Published: SAGE Publishing 2019-10-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1177/0263617419860620
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author Changxin Li
Yuan Yu
Qiuyue Li
Hong Zhong
Shuai Wang
author_facet Changxin Li
Yuan Yu
Qiuyue Li
Hong Zhong
Shuai Wang
author_sort Changxin Li
collection DOAJ
description The calcium silicate hydrate synthesized from electrolytic manganese residue was investigated as adsorbents to remove the phosphate from aqueous solutions. The effects of different experimental parameters, including contact time, initial phosphate concentration, solution pH, and temperature on the phosphate adsorption were investigated. The results showed that the phosphate adsorption was highly pH-dependent, with removal being more efficient under the pH range of 10.0–11.0. The Freundlich and Langmuir models were used to simulate the sorption equilibrium, and the results indicate that the adsorption data fitted well to the Langmuir model with which the maximum phosphate adsorption capacity was estimated to be 65.79–85.47 mg/g at 25–35°C. Meanwhile, the kinetic data confirmed that the sorption of phosphorus onto electrolytic manganese residue–calcium silicate hydrate can be best described by the pseudo-second-order kinetic model, suggesting that the adsorption process might be chemical sorption. Furthermore, thermodynamic studies illustrated that the adsorption process was endothermic and spontaneous in nature.
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institution DOAJ
issn 0263-6174
2048-4038
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publishDate 2019-10-01
publisher SAGE Publishing
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series Adsorption Science & Technology
spelling doaj-art-15373a68cf2c4ba58584ee347f2fff4b2025-08-20T02:43:16ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382019-10-013710.1177/0263617419860620Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residueChangxin LiYuan YuQiuyue LiHong ZhongShuai WangThe calcium silicate hydrate synthesized from electrolytic manganese residue was investigated as adsorbents to remove the phosphate from aqueous solutions. The effects of different experimental parameters, including contact time, initial phosphate concentration, solution pH, and temperature on the phosphate adsorption were investigated. The results showed that the phosphate adsorption was highly pH-dependent, with removal being more efficient under the pH range of 10.0–11.0. The Freundlich and Langmuir models were used to simulate the sorption equilibrium, and the results indicate that the adsorption data fitted well to the Langmuir model with which the maximum phosphate adsorption capacity was estimated to be 65.79–85.47 mg/g at 25–35°C. Meanwhile, the kinetic data confirmed that the sorption of phosphorus onto electrolytic manganese residue–calcium silicate hydrate can be best described by the pseudo-second-order kinetic model, suggesting that the adsorption process might be chemical sorption. Furthermore, thermodynamic studies illustrated that the adsorption process was endothermic and spontaneous in nature.https://doi.org/10.1177/0263617419860620
spellingShingle Changxin Li
Yuan Yu
Qiuyue Li
Hong Zhong
Shuai Wang
Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
Adsorption Science & Technology
title Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
title_full Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
title_fullStr Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
title_full_unstemmed Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
title_short Kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
title_sort kinetics and equilibrium studies of phosphate removal from aqueous solution by calcium silicate hydrate synthesized from electrolytic manganese residue
url https://doi.org/10.1177/0263617419860620
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AT yuanyu kineticsandequilibriumstudiesofphosphateremovalfromaqueoussolutionbycalciumsilicatehydratesynthesizedfromelectrolyticmanganeseresidue
AT qiuyueli kineticsandequilibriumstudiesofphosphateremovalfromaqueoussolutionbycalciumsilicatehydratesynthesizedfromelectrolyticmanganeseresidue
AT hongzhong kineticsandequilibriumstudiesofphosphateremovalfromaqueoussolutionbycalciumsilicatehydratesynthesizedfromelectrolyticmanganeseresidue
AT shuaiwang kineticsandequilibriumstudiesofphosphateremovalfromaqueoussolutionbycalciumsilicatehydratesynthesizedfromelectrolyticmanganeseresidue