Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries

Constructing an optimal solid–electrolyte interphase (SEI) through electrolyte strategies is an effective approach to suppress lithium dendrites and improve deposition/stripping reversibility. Specifically, increasing the proportion of anion coordination in the inner Li+ solvation sheath promotes th...

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Main Authors: Pengbin Lai, Yaqi Zhang, Junhao Wang, Minghui Chen, Xinyu Li, Xiaodie Deng, Qichen Chen, Boyang Huang, Chaolun Gan, Yeguo Zou, Yu Qiao, Peng Zhang, Jinbao Zhao
Format: Article
Language:English
Published: KeAi Communications Co. Ltd. 2025-09-01
Series:eScience
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Online Access:http://www.sciencedirect.com/science/article/pii/S2667141725000291
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author Pengbin Lai
Yaqi Zhang
Junhao Wang
Minghui Chen
Xinyu Li
Xiaodie Deng
Qichen Chen
Boyang Huang
Chaolun Gan
Yeguo Zou
Yu Qiao
Peng Zhang
Jinbao Zhao
author_facet Pengbin Lai
Yaqi Zhang
Junhao Wang
Minghui Chen
Xinyu Li
Xiaodie Deng
Qichen Chen
Boyang Huang
Chaolun Gan
Yeguo Zou
Yu Qiao
Peng Zhang
Jinbao Zhao
author_sort Pengbin Lai
collection DOAJ
description Constructing an optimal solid–electrolyte interphase (SEI) through electrolyte strategies is an effective approach to suppress lithium dendrites and improve deposition/stripping reversibility. Specifically, increasing the proportion of anion coordination in the inner Li+ solvation sheath promotes the formation of an anion-derived SEI that features a high content of inorganic components favoring Li+ diffusion. However, whether this anion-rich structure can persist during cycling has not been dynamically investigated. In this work, we not only construct a favorable solvation structure but also study its evolution in both bulk and interface regions across varying temperatures. Additionally, we employ the unique “adsorption-attraction” mechanism of trifluoromethoxybenzene (PhOCF3) solvent to inhibit the undesirable transition from an “anion-rich” to “anion-deficient” structure at the anode interface, which is confirmed by 2D NMR and in situ infrared spectroscopy. In summary, this work explores the solvation structure in depth and proposes new perspectives on designing electrolytes for lithium metal batteries.
format Article
id doaj-art-1520d2e4df8945a583f8baea05a2186c
institution Kabale University
issn 2667-1417
language English
publishDate 2025-09-01
publisher KeAi Communications Co. Ltd.
record_format Article
series eScience
spelling doaj-art-1520d2e4df8945a583f8baea05a2186c2025-08-25T04:14:53ZengKeAi Communications Co. Ltd.eScience2667-14172025-09-015510039910.1016/j.esci.2025.100399Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteriesPengbin Lai0Yaqi Zhang1Junhao Wang2Minghui Chen3Xinyu Li4Xiaodie Deng5Qichen Chen6Boyang Huang7Chaolun Gan8Yeguo Zou9Yu Qiao10Peng Zhang11Jinbao Zhao12State-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaCollege of Energy, Xiamen University, Xiamen 361102, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaCollege of Energy, Xiamen University, Xiamen 361102, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaZhangjiagang Guotai Huarong Chemical New Material Co., Ltd, Zhangjiagang 215634, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaState-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, ChinaCollege of Energy, Xiamen University, Xiamen 361102, China; Corresponding author.State-Province Joint Engineering Laboratory of Power Source Technology for New Energy Vehicle, Engineering Research Center of Electrochemical Technology, Ministry of Education, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005, China; Corresponding author.Constructing an optimal solid–electrolyte interphase (SEI) through electrolyte strategies is an effective approach to suppress lithium dendrites and improve deposition/stripping reversibility. Specifically, increasing the proportion of anion coordination in the inner Li+ solvation sheath promotes the formation of an anion-derived SEI that features a high content of inorganic components favoring Li+ diffusion. However, whether this anion-rich structure can persist during cycling has not been dynamically investigated. In this work, we not only construct a favorable solvation structure but also study its evolution in both bulk and interface regions across varying temperatures. Additionally, we employ the unique “adsorption-attraction” mechanism of trifluoromethoxybenzene (PhOCF3) solvent to inhibit the undesirable transition from an “anion-rich” to “anion-deficient” structure at the anode interface, which is confirmed by 2D NMR and in situ infrared spectroscopy. In summary, this work explores the solvation structure in depth and proposes new perspectives on designing electrolytes for lithium metal batteries.http://www.sciencedirect.com/science/article/pii/S2667141725000291Solvation structureIn situ characterizationLithium metal batteryLow temperatureLocalized high-concentration electrolyte
spellingShingle Pengbin Lai
Yaqi Zhang
Junhao Wang
Minghui Chen
Xinyu Li
Xiaodie Deng
Qichen Chen
Boyang Huang
Chaolun Gan
Yeguo Zou
Yu Qiao
Peng Zhang
Jinbao Zhao
Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries
eScience
Solvation structure
In situ characterization
Lithium metal battery
Low temperature
Localized high-concentration electrolyte
title Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries
title_full Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries
title_fullStr Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries
title_full_unstemmed Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries
title_short Adsorption-attraction electrolyte addressing anion-deficient interface for lithium metal batteries
title_sort adsorption attraction electrolyte addressing anion deficient interface for lithium metal batteries
topic Solvation structure
In situ characterization
Lithium metal battery
Low temperature
Localized high-concentration electrolyte
url http://www.sciencedirect.com/science/article/pii/S2667141725000291
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