Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals

Abstract Mechanical properties and integrity of biodegradable Zn alloys during degradation holds significant importance. In this study, a Zn-Mg-Mn alloy with tensile strength of 414 MPa and an elongation of 26% was developed. The strength contributions of as-extruded Zn alloy from grain boundary str...

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Main Authors: Chengwu Lu, Chao Song, Yunlong Yu, Linhai Yang, Wu Zheng, Fenqi Luo, Yuhua Xiao, Jun Luo, Jie Xu
Format: Article
Language:English
Published: Nature Portfolio 2024-12-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-024-78842-0
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author Chengwu Lu
Chao Song
Yunlong Yu
Linhai Yang
Wu Zheng
Fenqi Luo
Yuhua Xiao
Jun Luo
Jie Xu
author_facet Chengwu Lu
Chao Song
Yunlong Yu
Linhai Yang
Wu Zheng
Fenqi Luo
Yuhua Xiao
Jun Luo
Jie Xu
author_sort Chengwu Lu
collection DOAJ
description Abstract Mechanical properties and integrity of biodegradable Zn alloys during degradation holds significant importance. In this study, a Zn-Mg-Mn alloy with tensile strength of 414 MPa and an elongation of 26% was developed. The strength contributions of as-extruded Zn alloy from grain boundary strengthening, precipitation strengthening, and second phase strengthening. Degradation of the Zn alloy in Hank’s solution exhibited a decreasing trend with prolonged immersion, eventually stabilizing at 16 μm/year. Corrosion morphology analysis revealed that the corrosion modes transformed from pitting corrosion to severely localized corrosion with prolonged immersion time, eventually lead to formation of large holes. Although the tensile strength of the Zn alloys remained relatively unchanged following varied immersion time, a substantial decrease in elongation was observed. The decreased elongation primarily attributed to the formation of surface corrosion pits or holes, exacerbating crack propagation during tension. Biocompatibility assessments of Zn alloys demonstrated that a 50% concentration of Zn alloy leach solution cultured with C3H10 and RMSC cells yielded cellular activity exceeding 80%, indicating excellent cytocompatibility. Alkaline phosphatase (ALP) and alizarin red staining results further underscored the remarkable early and late osteogenic properties exhibited by Zn-Mg-Mn alloy.
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issn 2045-2322
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spelling doaj-art-1515ac29f51c4f76a32d5163953df3aa2025-08-20T02:39:40ZengNature PortfolioScientific Reports2045-23222024-12-0114111410.1038/s41598-024-78842-0Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metalsChengwu Lu0Chao Song1Yunlong Yu2Linhai Yang3Wu Zheng4Fenqi Luo5Yuhua Xiao6Jun Luo7Jie Xu8Shengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityShengli Clinical Medical College of Fujian Medical UniversityAbstract Mechanical properties and integrity of biodegradable Zn alloys during degradation holds significant importance. In this study, a Zn-Mg-Mn alloy with tensile strength of 414 MPa and an elongation of 26% was developed. The strength contributions of as-extruded Zn alloy from grain boundary strengthening, precipitation strengthening, and second phase strengthening. Degradation of the Zn alloy in Hank’s solution exhibited a decreasing trend with prolonged immersion, eventually stabilizing at 16 μm/year. Corrosion morphology analysis revealed that the corrosion modes transformed from pitting corrosion to severely localized corrosion with prolonged immersion time, eventually lead to formation of large holes. Although the tensile strength of the Zn alloys remained relatively unchanged following varied immersion time, a substantial decrease in elongation was observed. The decreased elongation primarily attributed to the formation of surface corrosion pits or holes, exacerbating crack propagation during tension. Biocompatibility assessments of Zn alloys demonstrated that a 50% concentration of Zn alloy leach solution cultured with C3H10 and RMSC cells yielded cellular activity exceeding 80%, indicating excellent cytocompatibility. Alkaline phosphatase (ALP) and alizarin red staining results further underscored the remarkable early and late osteogenic properties exhibited by Zn-Mg-Mn alloy.https://doi.org/10.1038/s41598-024-78842-0Biodegradable zn alloysMechanical propertiesMechanical integrityBiocompatibility
spellingShingle Chengwu Lu
Chao Song
Yunlong Yu
Linhai Yang
Wu Zheng
Fenqi Luo
Yuhua Xiao
Jun Luo
Jie Xu
Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
Scientific Reports
Biodegradable zn alloys
Mechanical properties
Mechanical integrity
Biocompatibility
title Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
title_full Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
title_fullStr Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
title_full_unstemmed Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
title_short Biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
title_sort biodegradable zinc alloys with high strength and suitable mechanical integrity as bone repair metals
topic Biodegradable zn alloys
Mechanical properties
Mechanical integrity
Biocompatibility
url https://doi.org/10.1038/s41598-024-78842-0
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AT yunlongyu biodegradablezincalloyswithhighstrengthandsuitablemechanicalintegrityasbonerepairmetals
AT linhaiyang biodegradablezincalloyswithhighstrengthandsuitablemechanicalintegrityasbonerepairmetals
AT wuzheng biodegradablezincalloyswithhighstrengthandsuitablemechanicalintegrityasbonerepairmetals
AT fenqiluo biodegradablezincalloyswithhighstrengthandsuitablemechanicalintegrityasbonerepairmetals
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