Electronic superradiance mediated by nuclear dynamics

Superradiance, in which the collective behavior of emitters can generate enhanced radiative decay, was first predicted by a model, now known as the Dicke model, that contains a collection of two-level systems (the emitters) all interacting with the same photonic mode. In this article, we extend the...

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Main Authors: Xuecheng Tao, John P. Philbin, Prineha Narang
Format: Article
Language:English
Published: American Physical Society 2025-02-01
Series:Physical Review Research
Online Access:http://doi.org/10.1103/PhysRevResearch.7.013133
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author Xuecheng Tao
John P. Philbin
Prineha Narang
author_facet Xuecheng Tao
John P. Philbin
Prineha Narang
author_sort Xuecheng Tao
collection DOAJ
description Superradiance, in which the collective behavior of emitters can generate enhanced radiative decay, was first predicted by a model, now known as the Dicke model, that contains a collection of two-level systems (the emitters) all interacting with the same photonic mode. In this article, we extend the original Dicke model to elucidate the influence of nuclear motion on superradiant emission. Our dynamical simulations of the combined electronic, nuclear, and photonic system reveal a new time scale attributed to the population leakage of the dark, subradiant states. Furthermore, this dark-state emission pathway can be controlled by tuning the nuclear potential energy landscape. These findings impact how superradiant states and molecular degrees of freedom can be leveraged and utilized in quantum optical systems.
format Article
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series Physical Review Research
spelling doaj-art-132d6510212e4e1ca5d4338d3ae88db02025-02-05T15:33:50ZengAmerican Physical SocietyPhysical Review Research2643-15642025-02-017101313310.1103/PhysRevResearch.7.013133Electronic superradiance mediated by nuclear dynamicsXuecheng TaoJohn P. PhilbinPrineha NarangSuperradiance, in which the collective behavior of emitters can generate enhanced radiative decay, was first predicted by a model, now known as the Dicke model, that contains a collection of two-level systems (the emitters) all interacting with the same photonic mode. In this article, we extend the original Dicke model to elucidate the influence of nuclear motion on superradiant emission. Our dynamical simulations of the combined electronic, nuclear, and photonic system reveal a new time scale attributed to the population leakage of the dark, subradiant states. Furthermore, this dark-state emission pathway can be controlled by tuning the nuclear potential energy landscape. These findings impact how superradiant states and molecular degrees of freedom can be leveraged and utilized in quantum optical systems.http://doi.org/10.1103/PhysRevResearch.7.013133
spellingShingle Xuecheng Tao
John P. Philbin
Prineha Narang
Electronic superradiance mediated by nuclear dynamics
Physical Review Research
title Electronic superradiance mediated by nuclear dynamics
title_full Electronic superradiance mediated by nuclear dynamics
title_fullStr Electronic superradiance mediated by nuclear dynamics
title_full_unstemmed Electronic superradiance mediated by nuclear dynamics
title_short Electronic superradiance mediated by nuclear dynamics
title_sort electronic superradiance mediated by nuclear dynamics
url http://doi.org/10.1103/PhysRevResearch.7.013133
work_keys_str_mv AT xuechengtao electronicsuperradiancemediatedbynucleardynamics
AT johnpphilbin electronicsuperradiancemediatedbynucleardynamics
AT prinehanarang electronicsuperradiancemediatedbynucleardynamics