The reaction mechanism of acetanilide herbicides with urease

The binding of acetochor, pretilachor, butachlor and metolachlor to urease in aqueous solution was studied using UV difference spectrum and fluorescence spectrum methods. According to the UV difference spectrum curve obtained, the UV difference adsorption AA showed rapid change when herbicide concen...

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Main Authors: LIU Hui-jun, LIU Wei-ping
Format: Article
Language:English
Published: Zhejiang University Press 2004-03-01
Series:浙江大学学报. 农业与生命科学版
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Online Access:https://www.academax.com/doi/10.3785/1008-9209.2004.02.0210
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author LIU Hui-jun
LIU Wei-ping
author_facet LIU Hui-jun
LIU Wei-ping
author_sort LIU Hui-jun
collection DOAJ
description The binding of acetochor, pretilachor, butachlor and metolachlor to urease in aqueous solution was studied using UV difference spectrum and fluorescence spectrum methods. According to the UV difference spectrum curve obtained, the UV difference adsorption AA showed rapid change when herbicide concentrations ranged from 0.0 to 1.6 μmol/L. Red shift occurred in the UV difference spectra of urease and absorbance-peaks were lower. It was shown that the herbicides quenched the urease fluorescence mainly through a static quenching process. The binding constant K and the number of binding site n were calculated according to the fluorescence quenching results. In case of acetochor, K=1.17×10<sup>3</sup> L/mol and n was 0.81; to pretilachor, K=1.46×10<sup>2</sup> L/mol and n was 0.67; whereas for butachlor, K=29×10<sup>1</sup> L/mol and n was 0.50; and for metolachlor, K=1.49×10<sup>3</sup> L/mol and n was 0.84.
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series 浙江大学学报. 农业与生命科学版
spelling doaj-art-12d0872d71ea42d4a918b56c4a2e1ab12025-08-20T03:15:37ZengZhejiang University Press浙江大学学报. 农业与生命科学版1008-92092097-51552004-03-013021021410.3785/1008-9209.2004.02.021010089209The reaction mechanism of acetanilide herbicides with ureaseLIU Hui-junLIU Wei-pingThe binding of acetochor, pretilachor, butachlor and metolachlor to urease in aqueous solution was studied using UV difference spectrum and fluorescence spectrum methods. According to the UV difference spectrum curve obtained, the UV difference adsorption AA showed rapid change when herbicide concentrations ranged from 0.0 to 1.6 μmol/L. Red shift occurred in the UV difference spectra of urease and absorbance-peaks were lower. It was shown that the herbicides quenched the urease fluorescence mainly through a static quenching process. The binding constant K and the number of binding site n were calculated according to the fluorescence quenching results. In case of acetochor, K=1.17×10<sup>3</sup> L/mol and n was 0.81; to pretilachor, K=1.46×10<sup>2</sup> L/mol and n was 0.67; whereas for butachlor, K=29×10<sup>1</sup> L/mol and n was 0.50; and for metolachlor, K=1.49×10<sup>3</sup> L/mol and n was 0.84.https://www.academax.com/doi/10.3785/1008-9209.2004.02.0210acetanilide herbicidesureaseUV difference spectrumfluorescence spectrum
spellingShingle LIU Hui-jun
LIU Wei-ping
The reaction mechanism of acetanilide herbicides with urease
浙江大学学报. 农业与生命科学版
acetanilide herbicides
urease
UV difference spectrum
fluorescence spectrum
title The reaction mechanism of acetanilide herbicides with urease
title_full The reaction mechanism of acetanilide herbicides with urease
title_fullStr The reaction mechanism of acetanilide herbicides with urease
title_full_unstemmed The reaction mechanism of acetanilide herbicides with urease
title_short The reaction mechanism of acetanilide herbicides with urease
title_sort reaction mechanism of acetanilide herbicides with urease
topic acetanilide herbicides
urease
UV difference spectrum
fluorescence spectrum
url https://www.academax.com/doi/10.3785/1008-9209.2004.02.0210
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AT liuweiping reactionmechanismofacetanilideherbicideswithurease