Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications

Abstract Integrating conductive nanomaterials with polymer substrates in a scalable and low‐cost way is crucial for developing flexible electronics. This work presents a scalable process for integrating high‐quality nanomaterials with polymer films to fabricate flexible electrical devices by combini...

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Main Authors: Mehraneh Tavakkoli Gilavan, Oluwawemimo Igun, Md Ali Akbar, Shayan Jahangirifard, Peter Kruse, Ponnambalam Ravi Selvaganapathy
Format: Article
Language:English
Published: Wiley-VCH 2025-07-01
Series:Advanced Materials Interfaces
Subjects:
Online Access:https://doi.org/10.1002/admi.202500027
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author Mehraneh Tavakkoli Gilavan
Oluwawemimo Igun
Md Ali Akbar
Shayan Jahangirifard
Peter Kruse
Ponnambalam Ravi Selvaganapathy
author_facet Mehraneh Tavakkoli Gilavan
Oluwawemimo Igun
Md Ali Akbar
Shayan Jahangirifard
Peter Kruse
Ponnambalam Ravi Selvaganapathy
author_sort Mehraneh Tavakkoli Gilavan
collection DOAJ
description Abstract Integrating conductive nanomaterials with polymer substrates in a scalable and low‐cost way is crucial for developing flexible electronics. This work presents a scalable process for integrating high‐quality nanomaterials with polymer films to fabricate flexible electrical devices by combining simple yet effective techniques. Various conductive patterns on polymer substrates are successfully created by utilizing a combination of nanomaterial spraying, laser treatment, and adhesive delamination. The laser treatment embeds the sprayed nanoparticles onto the polymer surface by partially melting the polymer and significantly enhancing their adhesion selectively in places where it traces a path. This method incorporates single‐walled carbon nanotubes, graphene, and molybdenum disulfide onto polymers such as polypropylene, polyvinylidene fluoride, and nylon, achieving a minimum line width of 350 µm. The versatility of this technique is demonstrated by fabricating a range of devices, including microheaters, temperature sensors, chemiresistive sensors, and electrochemical sensors. The fabricated devices exhibit excellent durability and stable performance, addressing the limitations of integrating nanomaterials into polymer films. Additionally, this method allows for precise control of conductivity and pattern complexity, making it suitable for various applications. This work contributes to the advancement of flexible electronics, providing a scalable and adaptable method for creating high‐performance devices.
format Article
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institution Kabale University
issn 2196-7350
language English
publishDate 2025-07-01
publisher Wiley-VCH
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series Advanced Materials Interfaces
spelling doaj-art-10be52a204524523a30b94e992cb8af72025-08-20T03:27:29ZengWiley-VCHAdvanced Materials Interfaces2196-73502025-07-011213n/an/a10.1002/admi.202500027Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing ApplicationsMehraneh Tavakkoli Gilavan0Oluwawemimo Igun1Md Ali Akbar2Shayan Jahangirifard3Peter Kruse4Ponnambalam Ravi Selvaganapathy5School of Biomedical Engineering McMaster University 1280 Main St W Hamilton L8S 4L7 CanadaDepartment of Mechanical Engineering McMaster University 1280 Main St W Hamilton L8S 4L7 CanadaDepartment of Chemistry and Chemical Biology McMaster University 1280 Main St W Hamilton L8S 4M1 CanadaSchool of Biomedical Engineering McMaster University 1280 Main St W Hamilton L8S 4L7 CanadaDepartment of Chemistry and Chemical Biology McMaster University 1280 Main St W Hamilton L8S 4M1 CanadaSchool of Biomedical Engineering McMaster University 1280 Main St W Hamilton L8S 4L7 CanadaAbstract Integrating conductive nanomaterials with polymer substrates in a scalable and low‐cost way is crucial for developing flexible electronics. This work presents a scalable process for integrating high‐quality nanomaterials with polymer films to fabricate flexible electrical devices by combining simple yet effective techniques. Various conductive patterns on polymer substrates are successfully created by utilizing a combination of nanomaterial spraying, laser treatment, and adhesive delamination. The laser treatment embeds the sprayed nanoparticles onto the polymer surface by partially melting the polymer and significantly enhancing their adhesion selectively in places where it traces a path. This method incorporates single‐walled carbon nanotubes, graphene, and molybdenum disulfide onto polymers such as polypropylene, polyvinylidene fluoride, and nylon, achieving a minimum line width of 350 µm. The versatility of this technique is demonstrated by fabricating a range of devices, including microheaters, temperature sensors, chemiresistive sensors, and electrochemical sensors. The fabricated devices exhibit excellent durability and stable performance, addressing the limitations of integrating nanomaterials into polymer films. Additionally, this method allows for precise control of conductivity and pattern complexity, making it suitable for various applications. This work contributes to the advancement of flexible electronics, providing a scalable and adaptable method for creating high‐performance devices.https://doi.org/10.1002/admi.202500027adhesive delaminationflexible sensorslaser direct writingpatterning nanomaterials
spellingShingle Mehraneh Tavakkoli Gilavan
Oluwawemimo Igun
Md Ali Akbar
Shayan Jahangirifard
Peter Kruse
Ponnambalam Ravi Selvaganapathy
Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications
Advanced Materials Interfaces
adhesive delamination
flexible sensors
laser direct writing
patterning nanomaterials
title Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications
title_full Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications
title_fullStr Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications
title_full_unstemmed Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications
title_short Patterning of Nano and Micromaterials on Polymer Substrates Using Spraying, Selective Laser Treatment, and Adhesive Delamination for Sensing Applications
title_sort patterning of nano and micromaterials on polymer substrates using spraying selective laser treatment and adhesive delamination for sensing applications
topic adhesive delamination
flexible sensors
laser direct writing
patterning nanomaterials
url https://doi.org/10.1002/admi.202500027
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