Сhromatographic methods for the study of organic extractants of transformer oil

THE PURPOSE. In order to control the technical condition of oil-filled electrical equipment, a number of new analytical methods have recently been created to determine the ultra-low concentrations of impurity compounds in transformer oil. An analysis of the literature data showed that at this stage...

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Main Authors: Ngoc Dan Vu, V. F. Novikov
Format: Article
Language:English
Published: Kazan State Power Engineering University 2021-03-01
Series:Известия высших учебных заведений: Проблемы энергетики
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Online Access:https://www.energyret.ru/jour/article/view/1627
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author Ngoc Dan Vu
V. F. Novikov
author_facet Ngoc Dan Vu
V. F. Novikov
author_sort Ngoc Dan Vu
collection DOAJ
description THE PURPOSE. In order to control the technical condition of oil-filled electrical equipment, a number of new analytical methods have recently been created to determine the ultra-low concentrations of impurity compounds in transformer oil. An analysis of the literature data showed that at this stage of the analytical procedure significant errors may occur that worsen the quality of control of the technical condition of oil-filled electrical equipment, and in some cases make its results meaningless. The published literature practically does not discuss the problem of sample preparation of transformer oil, which negatively affects the quality of analytical control, that is, the reliability of the results and, accordingly, the diagnosis of oil-filled electrical equipment. METHODS. The paper discusses a sample preparation system for transformer oil, which is based on various methods for extracting target components from it. The adsorption process is used, the preparation of chemical derivatives, various types of extraction, liquid, gas, solid phase and fluid, as well as using low temperatures, extraction in microwave, magnetic, electromagnetic and centrifugal fields. It is shown that liquid extraction with an organic solvent is widely used from all sample preparation methods, with the help of which furan compounds resulting from the destruction of paper insulation are extracted from transformer oil. The disadvantages of sample preparation using liquid-phase extraction and the possibility of using solid-phase extraction on various adsorbents for this purpose are discussed. RESULTS. The results of an experimental study of the sorption properties of various organic solvents with respect to porous materials differing in the structure of their surface are presented. We used zeolite-bearing rocks of the Tatar-Shatrashansky deposit, synthetic zeolites NaX-13A. Using the ascending variant of liquid column chromatography, the absolute retention values of standard extractants were determined and their dependence on the length of the sorption layer of the porous material was found. CONCLUSIONS. It was shown that the highest retention times for all studied adsorbents are observed for organochlorine extractants, chloroform, carbon tetrachloride, dichloroethane, trichlorethylene. For N. Hexane is a relatively small interaction. Histograms are given of the effect of the retention time of standard sorbates (extractants) on their physicochemical nature.
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spelling doaj-art-10073161e5c047febf6c7f26d46d011e2025-08-20T01:53:25ZengKazan State Power Engineering UniversityИзвестия высших учебных заведений: Проблемы энергетики1998-99032021-03-0122620221010.30724/1998-9903-2020-22-6-202-210720Сhromatographic methods for the study of organic extractants of transformer oilNgoc Dan Vu0V. F. Novikov1Kazan State Power Engineering UniversityKazan State Power Engineering UniversityTHE PURPOSE. In order to control the technical condition of oil-filled electrical equipment, a number of new analytical methods have recently been created to determine the ultra-low concentrations of impurity compounds in transformer oil. An analysis of the literature data showed that at this stage of the analytical procedure significant errors may occur that worsen the quality of control of the technical condition of oil-filled electrical equipment, and in some cases make its results meaningless. The published literature practically does not discuss the problem of sample preparation of transformer oil, which negatively affects the quality of analytical control, that is, the reliability of the results and, accordingly, the diagnosis of oil-filled electrical equipment. METHODS. The paper discusses a sample preparation system for transformer oil, which is based on various methods for extracting target components from it. The adsorption process is used, the preparation of chemical derivatives, various types of extraction, liquid, gas, solid phase and fluid, as well as using low temperatures, extraction in microwave, magnetic, electromagnetic and centrifugal fields. It is shown that liquid extraction with an organic solvent is widely used from all sample preparation methods, with the help of which furan compounds resulting from the destruction of paper insulation are extracted from transformer oil. The disadvantages of sample preparation using liquid-phase extraction and the possibility of using solid-phase extraction on various adsorbents for this purpose are discussed. RESULTS. The results of an experimental study of the sorption properties of various organic solvents with respect to porous materials differing in the structure of their surface are presented. We used zeolite-bearing rocks of the Tatar-Shatrashansky deposit, synthetic zeolites NaX-13A. Using the ascending variant of liquid column chromatography, the absolute retention values of standard extractants were determined and their dependence on the length of the sorption layer of the porous material was found. CONCLUSIONS. It was shown that the highest retention times for all studied adsorbents are observed for organochlorine extractants, chloroform, carbon tetrachloride, dichloroethane, trichlorethylene. For N. Hexane is a relatively small interaction. Histograms are given of the effect of the retention time of standard sorbates (extractants) on their physicochemical nature.https://www.energyret.ru/jour/article/view/1627electrical equipmenttransformer oilcontrolsorbentdestructionextractionchromatographyretentionsolvent
spellingShingle Ngoc Dan Vu
V. F. Novikov
Сhromatographic methods for the study of organic extractants of transformer oil
Известия высших учебных заведений: Проблемы энергетики
electrical equipment
transformer oil
control
sorbent
destruction
extraction
chromatography
retention
solvent
title Сhromatographic methods for the study of organic extractants of transformer oil
title_full Сhromatographic methods for the study of organic extractants of transformer oil
title_fullStr Сhromatographic methods for the study of organic extractants of transformer oil
title_full_unstemmed Сhromatographic methods for the study of organic extractants of transformer oil
title_short Сhromatographic methods for the study of organic extractants of transformer oil
title_sort сhromatographic methods for the study of organic extractants of transformer oil
topic electrical equipment
transformer oil
control
sorbent
destruction
extraction
chromatography
retention
solvent
url https://www.energyret.ru/jour/article/view/1627
work_keys_str_mv AT ngocdanvu shromatographicmethodsforthestudyoforganicextractantsoftransformeroil
AT vfnovikov shromatographicmethodsforthestudyoforganicextractantsoftransformeroil