Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics

Composites of ferromagnetic and ferroelectric phases are of interest for studies on mechanical strain-mediated coupling between the two phases and for a variety of applications in sensors, energy harvesting, and high-frequency devices. Nanocomposites are of particular importance since their surface...

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Main Authors: Sujoy Saha, Sabita Acharya, Ying Liu, Peng Zhou, Michael R. Page, Gopalan Srinivasan
Format: Article
Language:English
Published: MDPI AG 2025-05-01
Series:Applied Sciences
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Online Access:https://www.mdpi.com/2076-3417/15/9/5162
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author Sujoy Saha
Sabita Acharya
Ying Liu
Peng Zhou
Michael R. Page
Gopalan Srinivasan
author_facet Sujoy Saha
Sabita Acharya
Ying Liu
Peng Zhou
Michael R. Page
Gopalan Srinivasan
author_sort Sujoy Saha
collection DOAJ
description Composites of ferromagnetic and ferroelectric phases are of interest for studies on mechanical strain-mediated coupling between the two phases and for a variety of applications in sensors, energy harvesting, and high-frequency devices. Nanocomposites are of particular importance since their surface area-to-volume ratio, a key factor that determines the strength of magneto-electric (ME) coupling, is much higher than for bulk or thin-film composites. Core–shell nano- and microcomposites of the ferroic phases are the preferred structures, since they are free of any clamping due to substrates that are present in nanobilayers or nanopillars on a substrate. This review concerns recent efforts on ME coupling in coaxial fibers of spinel or hexagonal ferrites for the magnetic phase and PZT or barium titanate for the ferroelectric phase. Several recent studies on the synthesis and ME measurements of fibers with nickel ferrite, nickel zinc ferrite, or cobalt ferrite for the spinel ferrite and M-, Y-, and W-types for the hexagonal ferrites were considered. Fibers synthesized by electrospinning were found to be free of impurity phases and had uniform core and shell structures. Piezo force microscopy (PFM) and scanning microwave microscopy (SMM) measurements of strengths of direct and converse ME effects on individual fibers showed evidence for strong coupling. Results of low-frequency ME voltage coefficient and magneto-dielectric effects on 2D and 3D films of the fibers assembled in a magnetic field, however, were indicative of ME couplings that were weaker than in bulk or thick-film composites. A strong ME interaction was only evident from data on magnetic field-induced variations in the remnant ferroelectric polarization in the discs of the fibers. Follow-up efforts aimed at further enhancement in the strengths of ME coupling in core–shell composites are also discussed in this review.
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spelling doaj-art-0f4a3b787f094558a1676c150da4f03c2025-08-20T02:30:46ZengMDPI AGApplied Sciences2076-34172025-05-01159516210.3390/app15095162Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and FerroelectricsSujoy Saha0Sabita Acharya1Ying Liu2Peng Zhou3Michael R. Page4Gopalan Srinivasan5Department of Physics, Oakland University, Rochester, MI 48309, USADepartment of Physics, Oakland University, Rochester, MI 48309, USADepartment of Physics, Oakland University, Rochester, MI 48309, USADepartment of Physics, Oakland University, Rochester, MI 48309, USAMaterials and Manufacturing Directorate, Air Force Research Laboratory, Wright-Patterson Air Force Base, Dayton, OH 45433, USADepartment of Physics, Oakland University, Rochester, MI 48309, USAComposites of ferromagnetic and ferroelectric phases are of interest for studies on mechanical strain-mediated coupling between the two phases and for a variety of applications in sensors, energy harvesting, and high-frequency devices. Nanocomposites are of particular importance since their surface area-to-volume ratio, a key factor that determines the strength of magneto-electric (ME) coupling, is much higher than for bulk or thin-film composites. Core–shell nano- and microcomposites of the ferroic phases are the preferred structures, since they are free of any clamping due to substrates that are present in nanobilayers or nanopillars on a substrate. This review concerns recent efforts on ME coupling in coaxial fibers of spinel or hexagonal ferrites for the magnetic phase and PZT or barium titanate for the ferroelectric phase. Several recent studies on the synthesis and ME measurements of fibers with nickel ferrite, nickel zinc ferrite, or cobalt ferrite for the spinel ferrite and M-, Y-, and W-types for the hexagonal ferrites were considered. Fibers synthesized by electrospinning were found to be free of impurity phases and had uniform core and shell structures. Piezo force microscopy (PFM) and scanning microwave microscopy (SMM) measurements of strengths of direct and converse ME effects on individual fibers showed evidence for strong coupling. Results of low-frequency ME voltage coefficient and magneto-dielectric effects on 2D and 3D films of the fibers assembled in a magnetic field, however, were indicative of ME couplings that were weaker than in bulk or thick-film composites. A strong ME interaction was only evident from data on magnetic field-induced variations in the remnant ferroelectric polarization in the discs of the fibers. Follow-up efforts aimed at further enhancement in the strengths of ME coupling in core–shell composites are also discussed in this review.https://www.mdpi.com/2076-3417/15/9/5162magnetoelectricnanofiberferrite: ferroelectricelectrospinning
spellingShingle Sujoy Saha
Sabita Acharya
Ying Liu
Peng Zhou
Michael R. Page
Gopalan Srinivasan
Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics
Applied Sciences
magnetoelectric
nanofiber
ferrite: ferroelectric
electrospinning
title Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics
title_full Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics
title_fullStr Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics
title_full_unstemmed Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics
title_short Review of Magnetoelectric Effects on Coaxial Fibers of Ferrites and Ferroelectrics
title_sort review of magnetoelectric effects on coaxial fibers of ferrites and ferroelectrics
topic magnetoelectric
nanofiber
ferrite: ferroelectric
electrospinning
url https://www.mdpi.com/2076-3417/15/9/5162
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AT pengzhou reviewofmagnetoelectriceffectsoncoaxialfibersofferritesandferroelectrics
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