COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents

In this work, absorption refrigerant working pairs consisting of four HFO refrigerants, R1234ze(E), R1234yf, R1233zd, and R1243zf, and ionic liquids were studied. The different ionic liquids contained 20 cations and 16 anions. The Henry′s law constant and solubility data of working pairs were simula...

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Main Authors: Sun Yanjun, Zheng Haiqi, Wang Shibiao, Wang Xiaopo, He Maogang
Format: Article
Language:zho
Published: Journal of Refrigeration Magazines Agency Co., Ltd. 2024-12-01
Series:Zhileng xuebao
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Online Access:http://www.zhilengxuebao.com/thesisDetails#10.12465/j.issn.0253-4339.2024.06.091
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author Sun Yanjun
Zheng Haiqi
Wang Shibiao
Wang Xiaopo
He Maogang
author_facet Sun Yanjun
Zheng Haiqi
Wang Shibiao
Wang Xiaopo
He Maogang
author_sort Sun Yanjun
collection DOAJ
description In this work, absorption refrigerant working pairs consisting of four HFO refrigerants, R1234ze(E), R1234yf, R1233zd, and R1243zf, and ionic liquids were studied. The different ionic liquids contained 20 cations and 16 anions. The Henry′s law constant and solubility data of working pairs were simulated by the COSMO-RS method. The differences in Henry′s law constant and solubility between the different working pairs are discussed from the perspective of polarized charge density on the molecular surface. The polarized surface charge density curve of the R1234ze(E) refrigerant has a peak in the negative region. It is compatible with anions with a peak in the positive region. However, the compatibility with the peak in the negative region is poor. Ionic liquids with low Henry′s law constants and high solubilities were screened out when they were paired with HFO refrigerants.
format Article
id doaj-art-0ec90072ef2041a6aa2d3bf7302db307
institution OA Journals
issn 0253-4339
language zho
publishDate 2024-12-01
publisher Journal of Refrigeration Magazines Agency Co., Ltd.
record_format Article
series Zhileng xuebao
spelling doaj-art-0ec90072ef2041a6aa2d3bf7302db3072025-08-20T02:02:58ZzhoJournal of Refrigeration Magazines Agency Co., Ltd.Zhileng xuebao0253-43392024-12-0145919878553316COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as AbsorbentsSun YanjunZheng HaiqiWang ShibiaoWang XiaopoHe MaogangIn this work, absorption refrigerant working pairs consisting of four HFO refrigerants, R1234ze(E), R1234yf, R1233zd, and R1243zf, and ionic liquids were studied. The different ionic liquids contained 20 cations and 16 anions. The Henry′s law constant and solubility data of working pairs were simulated by the COSMO-RS method. The differences in Henry′s law constant and solubility between the different working pairs are discussed from the perspective of polarized charge density on the molecular surface. The polarized surface charge density curve of the R1234ze(E) refrigerant has a peak in the negative region. It is compatible with anions with a peak in the positive region. However, the compatibility with the peak in the negative region is poor. Ionic liquids with low Henry′s law constants and high solubilities were screened out when they were paired with HFO refrigerants.http://www.zhilengxuebao.com/thesisDetails#10.12465/j.issn.0253-4339.2024.06.091COSMO-RSionic liquidsHFO refrigerantsabsorption refrigeration
spellingShingle Sun Yanjun
Zheng Haiqi
Wang Shibiao
Wang Xiaopo
He Maogang
COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents
Zhileng xuebao
COSMO-RS
ionic liquids
HFO refrigerants
absorption refrigeration
title COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents
title_full COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents
title_fullStr COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents
title_full_unstemmed COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents
title_short COSMO-RS Method for Screening Absorption Refrigerant Working Pairs Using Ionic Liquids as Absorbents
title_sort cosmo rs method for screening absorption refrigerant working pairs using ionic liquids as absorbents
topic COSMO-RS
ionic liquids
HFO refrigerants
absorption refrigeration
url http://www.zhilengxuebao.com/thesisDetails#10.12465/j.issn.0253-4339.2024.06.091
work_keys_str_mv AT sunyanjun cosmorsmethodforscreeningabsorptionrefrigerantworkingpairsusingionicliquidsasabsorbents
AT zhenghaiqi cosmorsmethodforscreeningabsorptionrefrigerantworkingpairsusingionicliquidsasabsorbents
AT wangshibiao cosmorsmethodforscreeningabsorptionrefrigerantworkingpairsusingionicliquidsasabsorbents
AT wangxiaopo cosmorsmethodforscreeningabsorptionrefrigerantworkingpairsusingionicliquidsasabsorbents
AT hemaogang cosmorsmethodforscreeningabsorptionrefrigerantworkingpairsusingionicliquidsasabsorbents