Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems

Antiferromagnetic materials (AFMs) have been gaining lots of attention due to their great potential in spintronics devices and the recently discovered novel spin structure in the momentum space, i.e., C-paired spin-valley or spin-momentum locking (CSML), where spins and valleys or momenta are locked...

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Main Authors: Mengli Hu, Xingkai Cheng, Zhenqiao Huang, Junwei Liu
Format: Article
Language:English
Published: American Physical Society 2025-06-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.15.021083
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author Mengli Hu
Xingkai Cheng
Zhenqiao Huang
Junwei Liu
author_facet Mengli Hu
Xingkai Cheng
Zhenqiao Huang
Junwei Liu
author_sort Mengli Hu
collection DOAJ
description Antiferromagnetic materials (AFMs) have been gaining lots of attention due to their great potential in spintronics devices and the recently discovered novel spin structure in the momentum space, i.e., C-paired spin-valley or spin-momentum locking (CSML), where spins and valleys or momenta are locked to each other due to the crystal symmetry guaranteeing zero magnetization. Here, we systematically study CSMLs and propose a general theory and algorithm using little cogroup and coset representatives, which reveals that 12 elementary kinds of CSMLs, determined by the geometric relation of spins and valleys and the essential symmetry guaranteeing zero magnetization, are sufficient to fully represent all possible CSMLs. By combining the proposed algorithm and high-throughput first-principles calculations, we predict 38 magnetic point groups and identify 142 experimentally verified AFMs that can realize CSML. Besides predicting new materials, our theory can naturally reveal underlying mechanisms of CSMLs’ responses to external fields. As an example, two qualitatively different types of piezomagnetism via occupation imbalance or spin tilting are predicted in RbV_{2}Te_{2}O. The algorithm and conclusions can be directly extended to the locking between valley or momentum and any other pseudovector degree of freedom, e.g., Berry curvature, as exemplified in RbV_{2}Te_{2}O and the new proposed piezo-Hall effect, where a strain can induce a nonzero anomalous Hall conductance. In addition, the proposed concept and methodology can be straightforwardly applied to other symmetry groups, such as spin group.
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publishDate 2025-06-01
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series Physical Review X
spelling doaj-art-0da1a2a9e8384bc19d84d9322cd631062025-08-20T03:26:14ZengAmerican Physical SocietyPhysical Review X2160-33082025-06-0115202108310.1103/PhysRevX.15.021083Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic SystemsMengli HuXingkai ChengZhenqiao HuangJunwei LiuAntiferromagnetic materials (AFMs) have been gaining lots of attention due to their great potential in spintronics devices and the recently discovered novel spin structure in the momentum space, i.e., C-paired spin-valley or spin-momentum locking (CSML), where spins and valleys or momenta are locked to each other due to the crystal symmetry guaranteeing zero magnetization. Here, we systematically study CSMLs and propose a general theory and algorithm using little cogroup and coset representatives, which reveals that 12 elementary kinds of CSMLs, determined by the geometric relation of spins and valleys and the essential symmetry guaranteeing zero magnetization, are sufficient to fully represent all possible CSMLs. By combining the proposed algorithm and high-throughput first-principles calculations, we predict 38 magnetic point groups and identify 142 experimentally verified AFMs that can realize CSML. Besides predicting new materials, our theory can naturally reveal underlying mechanisms of CSMLs’ responses to external fields. As an example, two qualitatively different types of piezomagnetism via occupation imbalance or spin tilting are predicted in RbV_{2}Te_{2}O. The algorithm and conclusions can be directly extended to the locking between valley or momentum and any other pseudovector degree of freedom, e.g., Berry curvature, as exemplified in RbV_{2}Te_{2}O and the new proposed piezo-Hall effect, where a strain can induce a nonzero anomalous Hall conductance. In addition, the proposed concept and methodology can be straightforwardly applied to other symmetry groups, such as spin group.http://doi.org/10.1103/PhysRevX.15.021083
spellingShingle Mengli Hu
Xingkai Cheng
Zhenqiao Huang
Junwei Liu
Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems
Physical Review X
title Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems
title_full Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems
title_fullStr Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems
title_full_unstemmed Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems
title_short Catalog of C-Paired Spin-Momentum Locking in Antiferromagnetic Systems
title_sort catalog of c paired spin momentum locking in antiferromagnetic systems
url http://doi.org/10.1103/PhysRevX.15.021083
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AT zhenqiaohuang catalogofcpairedspinmomentumlockinginantiferromagneticsystems
AT junweiliu catalogofcpairedspinmomentumlockinginantiferromagneticsystems