Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.

The cytochrome P450 CYP168A1 from Pseudomonas aeruginosa was cloned and expressed in Escherichia coli followed by purification and characterization of function. CYP168A1 is a fatty acid hydroxylase that hydroxylates saturated fatty acids, including myristic (0.30 min-1), palmitic (1.61 min-1) and st...

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Main Authors: Claire L Price, Andrew G S Warrilow, Nicola J Rolley, Josie E Parker, Vera Thoss, Diane E Kelly, Nicolae Corcionivoschi, Steven L Kelly
Format: Article
Language:English
Published: Public Library of Science (PLoS) 2022-01-01
Series:PLoS ONE
Online Access:https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0265227&type=printable
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author Claire L Price
Andrew G S Warrilow
Nicola J Rolley
Josie E Parker
Vera Thoss
Diane E Kelly
Nicolae Corcionivoschi
Steven L Kelly
author_facet Claire L Price
Andrew G S Warrilow
Nicola J Rolley
Josie E Parker
Vera Thoss
Diane E Kelly
Nicolae Corcionivoschi
Steven L Kelly
author_sort Claire L Price
collection DOAJ
description The cytochrome P450 CYP168A1 from Pseudomonas aeruginosa was cloned and expressed in Escherichia coli followed by purification and characterization of function. CYP168A1 is a fatty acid hydroxylase that hydroxylates saturated fatty acids, including myristic (0.30 min-1), palmitic (1.61 min-1) and stearic acids (1.24 min-1), at both the ω-1- and ω-2-positions. However, CYP168A1 only hydroxylates unsaturated fatty acids, including palmitoleic (0.38 min-1), oleic (1.28 min-1) and linoleic acids (0.35 min-1), at the ω-1-position. CYP168A1 exhibited a catalytic preference for palmitic, oleic and stearic acids as substrates in keeping with the phosphatidylcholine-rich environment deep in the lung that is colonized by P. aeruginosa.
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spelling doaj-art-0c90bb703fce45e4b14eb43700b546562025-08-20T02:02:53ZengPublic Library of Science (PLoS)PLoS ONE1932-62032022-01-01173e026522710.1371/journal.pone.0265227Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.Claire L PriceAndrew G S WarrilowNicola J RolleyJosie E ParkerVera ThossDiane E KellyNicolae CorcionivoschiSteven L KellyThe cytochrome P450 CYP168A1 from Pseudomonas aeruginosa was cloned and expressed in Escherichia coli followed by purification and characterization of function. CYP168A1 is a fatty acid hydroxylase that hydroxylates saturated fatty acids, including myristic (0.30 min-1), palmitic (1.61 min-1) and stearic acids (1.24 min-1), at both the ω-1- and ω-2-positions. However, CYP168A1 only hydroxylates unsaturated fatty acids, including palmitoleic (0.38 min-1), oleic (1.28 min-1) and linoleic acids (0.35 min-1), at the ω-1-position. CYP168A1 exhibited a catalytic preference for palmitic, oleic and stearic acids as substrates in keeping with the phosphatidylcholine-rich environment deep in the lung that is colonized by P. aeruginosa.https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0265227&type=printable
spellingShingle Claire L Price
Andrew G S Warrilow
Nicola J Rolley
Josie E Parker
Vera Thoss
Diane E Kelly
Nicolae Corcionivoschi
Steven L Kelly
Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.
PLoS ONE
title Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.
title_full Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.
title_fullStr Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.
title_full_unstemmed Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.
title_short Cytochrome P450 168A1 from Pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids.
title_sort cytochrome p450 168a1 from pseudomonas aeruginosa is involved in the hydroxylation of biologically relevant fatty acids
url https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0265227&type=printable
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