Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics

With China's urbanization advancing, the annual volume of municipal solid waste (MSW) collection continues to rise. MSW gasification has gained significant attention due to its large processing capacity, economic benefits, and low pollutant emissions. This study systematically investigates the...

Full description

Saved in:
Bibliographic Details
Main Authors: Ruochen YANG, Lei JIANG, Can TONG, Li SONG, Jiaxin YUE, Xiong ZHANG, Wei LIAO, Jing′ai SHAO, Haiping YANG, Shihong ZHANG, Hanping CHEN
Format: Article
Language:zho
Published: Editorial Office of Energy Environmental Protection 2025-04-01
Series:能源环境保护
Subjects:
Online Access:https://doi.org/10.20078/j.eep.20240907
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849310788219568128
author Ruochen YANG
Lei JIANG
Can TONG
Li SONG
Jiaxin YUE
Xiong ZHANG
Wei LIAO
Jing′ai SHAO
Haiping YANG
Shihong ZHANG
Hanping CHEN
author_facet Ruochen YANG
Lei JIANG
Can TONG
Li SONG
Jiaxin YUE
Xiong ZHANG
Wei LIAO
Jing′ai SHAO
Haiping YANG
Shihong ZHANG
Hanping CHEN
author_sort Ruochen YANG
collection DOAJ
description With China's urbanization advancing, the annual volume of municipal solid waste (MSW) collection continues to rise. MSW gasification has gained significant attention due to its large processing capacity, economic benefits, and low pollutant emissions. This study systematically investigates the effects of reaction temperature and equivalence ratio (ER) on MSW gasification using a fixed-bed reactor, focusing on syngas composition, tar formation characteristics, and slagging behavior of gasification ash. Additionally, the transformation of tar compounds and the fusion properties of gasification ash under varying conditions are explored. Experimental results show that increasing the gasification temperature enhances MSW decomposition and tar cracking, leading to higher syngas yield and calorific value. As ER increases from 0 to 0.3, tar conversion into oxygenated compounds such as aldehydes, ketones, and acids is promoted, significantly improving syngas calorific value. However, when ER exceeds 0.3, excessive oxidation of CO and H2 reduces syngas quality and calorific value. At an optimal temperature of 700 ℃ and ER of 0.3, the highest syngas calorific value of about 23.51 MJ/Nm3 is achieved, with increased gas yield and reduced tar formation. X-ray fluorescence (XRF) spectroscopy and ash fusion analysis indicate that MSW gasification ash primarily consists of SiO2, Al2O3, and CaO. As ER increases, the hemispherical temperature (THT) and flow temperature (TFT) of the ash rise, suggesting a decrease in slagging propensity. However, slagging tendency calculations indicate a significant tendency for slagging under various conditions, posing potential risks to long-term gasifier operation. This issue is attributed to the high content of alkali metal oxides (such as Fe2O3 and K2O) in the gasification ash. These oxides react with SiO2 and Al2O3 to form low-melting eutectic compounds, reducing ash viscosity and increasing adhesion, thus exacerbating slagging at high temperatures. The study further highlights that gasification ash composition is highly sensitive to operating conditions. Slagging issues can be mitigated by adjusting the MSW feedstock composition or by adding SiO2 and Al2O3 as additives to improve reactor stability. Additionally, while increasing ER promotes syngas yield by facilitating tar cracking, excessive ER leads to undesirable oxidation of valuable syngas components, resulting in a trade-off between syngas production and calorific value. In summary, reaction temperature and ER play crucial roles in determining MSW gasification efficiency and stability. Proper optimization of these parameters enhances syngas quality while reducing tar formation and slagging risks. The findings of this study provide theoretical support for the industrial application of MSW gasification technology and offer new insights into optimizing syngas composition, improving ash behavior, and advancing sustainable waste-to-energy conversion.
format Article
id doaj-art-0c5349e877334c38a993f15900a4bf95
institution Kabale University
issn 2097-4183
language zho
publishDate 2025-04-01
publisher Editorial Office of Energy Environmental Protection
record_format Article
series 能源环境保护
spelling doaj-art-0c5349e877334c38a993f15900a4bf952025-08-20T03:53:38ZzhoEditorial Office of Energy Environmental Protection能源环境保护2097-41832025-04-0139217018110.20078/j.eep.202409072024-07-20-0002Study on Municipal Solid Waste Gasification and Ash Residue Slagging CharacteristicsRuochen YANG0Lei JIANG1Can TONG2Li SONG3Jiaxin YUE4Xiong ZHANG5Wei LIAO6Jing′ai SHAO7Haiping YANG8Shihong ZHANG9Hanping CHEN10State Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaBeijing Huayuhuihuang Eco-Environmental Protection Technology Co., Ltd., Beijing 100000, ChinaBeijing Huayuhuihuang Eco-Environmental Protection Technology Co., Ltd., Beijing 100000, ChinaBeijing Huayuhuihuang Eco-Environmental Protection Technology Co., Ltd., Beijing 100000, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Coal Combustion, School of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaWith China's urbanization advancing, the annual volume of municipal solid waste (MSW) collection continues to rise. MSW gasification has gained significant attention due to its large processing capacity, economic benefits, and low pollutant emissions. This study systematically investigates the effects of reaction temperature and equivalence ratio (ER) on MSW gasification using a fixed-bed reactor, focusing on syngas composition, tar formation characteristics, and slagging behavior of gasification ash. Additionally, the transformation of tar compounds and the fusion properties of gasification ash under varying conditions are explored. Experimental results show that increasing the gasification temperature enhances MSW decomposition and tar cracking, leading to higher syngas yield and calorific value. As ER increases from 0 to 0.3, tar conversion into oxygenated compounds such as aldehydes, ketones, and acids is promoted, significantly improving syngas calorific value. However, when ER exceeds 0.3, excessive oxidation of CO and H2 reduces syngas quality and calorific value. At an optimal temperature of 700 ℃ and ER of 0.3, the highest syngas calorific value of about 23.51 MJ/Nm3 is achieved, with increased gas yield and reduced tar formation. X-ray fluorescence (XRF) spectroscopy and ash fusion analysis indicate that MSW gasification ash primarily consists of SiO2, Al2O3, and CaO. As ER increases, the hemispherical temperature (THT) and flow temperature (TFT) of the ash rise, suggesting a decrease in slagging propensity. However, slagging tendency calculations indicate a significant tendency for slagging under various conditions, posing potential risks to long-term gasifier operation. This issue is attributed to the high content of alkali metal oxides (such as Fe2O3 and K2O) in the gasification ash. These oxides react with SiO2 and Al2O3 to form low-melting eutectic compounds, reducing ash viscosity and increasing adhesion, thus exacerbating slagging at high temperatures. The study further highlights that gasification ash composition is highly sensitive to operating conditions. Slagging issues can be mitigated by adjusting the MSW feedstock composition or by adding SiO2 and Al2O3 as additives to improve reactor stability. Additionally, while increasing ER promotes syngas yield by facilitating tar cracking, excessive ER leads to undesirable oxidation of valuable syngas components, resulting in a trade-off between syngas production and calorific value. In summary, reaction temperature and ER play crucial roles in determining MSW gasification efficiency and stability. Proper optimization of these parameters enhances syngas quality while reducing tar formation and slagging risks. The findings of this study provide theoretical support for the industrial application of MSW gasification technology and offer new insights into optimizing syngas composition, improving ash behavior, and advancing sustainable waste-to-energy conversion.https://doi.org/10.20078/j.eep.20240907municipal solid wastegasificationash residuemelting characteristicsreaction temperature
spellingShingle Ruochen YANG
Lei JIANG
Can TONG
Li SONG
Jiaxin YUE
Xiong ZHANG
Wei LIAO
Jing′ai SHAO
Haiping YANG
Shihong ZHANG
Hanping CHEN
Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics
能源环境保护
municipal solid waste
gasification
ash residue
melting characteristics
reaction temperature
title Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics
title_full Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics
title_fullStr Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics
title_full_unstemmed Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics
title_short Study on Municipal Solid Waste Gasification and Ash Residue Slagging Characteristics
title_sort study on municipal solid waste gasification and ash residue slagging characteristics
topic municipal solid waste
gasification
ash residue
melting characteristics
reaction temperature
url https://doi.org/10.20078/j.eep.20240907
work_keys_str_mv AT ruochenyang studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT leijiang studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT cantong studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT lisong studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT jiaxinyue studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT xiongzhang studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT weiliao studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT jingaishao studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT haipingyang studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT shihongzhang studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics
AT hanpingchen studyonmunicipalsolidwastegasificationandashresidueslaggingcharacteristics