New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)

A number of new 5-aminomethyl-1,2,4-triazole-3-carboxamides, demonstrating high model affinity to the IGPD catalytic site comparable with that of the native substrate, were synthesized. The derivatives obtained were tested for antimicrobial potential against <i>M. smegmatis</i>, a specie...

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Main Authors: Eugenia Oleynik, Ekaterina Pyankina, Ekaterina Mitina, Ekaterina Mikhina, Andrey Matveev
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Chemistry Proceedings
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Online Access:https://www.mdpi.com/2673-4583/16/1/67
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author Eugenia Oleynik
Ekaterina Pyankina
Ekaterina Mitina
Ekaterina Mikhina
Andrey Matveev
author_facet Eugenia Oleynik
Ekaterina Pyankina
Ekaterina Mitina
Ekaterina Mikhina
Andrey Matveev
author_sort Eugenia Oleynik
collection DOAJ
description A number of new 5-aminomethyl-1,2,4-triazole-3-carboxamides, demonstrating high model affinity to the IGPD catalytic site comparable with that of the native substrate, were synthesized. The derivatives obtained were tested for antimicrobial potential against <i>M. smegmatis</i>, a species related to <i>M. tuberculosis</i>. During the initial antimicrobial activity evaluation in vitro, some compounds investigated inhibited microbial growth. Moreover, high binding energy values calculated for compounds/enzyme’s catalytic site complexes correlated with the compounds’ antimicrobial efficacy. This suggests that the probable biological action mechanism of new 5-aminomethyl-1,2,4-triazole-3-carboxamides may be based on their binding to the catalytic site of IGPD, which provides prerequisites for further study of this class of compounds as potential IGPD inhibitors.
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institution Kabale University
issn 2673-4583
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publishDate 2024-11-01
publisher MDPI AG
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series Chemistry Proceedings
spelling doaj-art-0b7c40d28ef24b95b8ef230c9eed2f3e2025-08-20T03:26:11ZengMDPI AGChemistry Proceedings2673-45832024-11-011616710.3390/ecsoc-28-20178New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)Eugenia Oleynik0Ekaterina Pyankina1Ekaterina Mitina2Ekaterina Mikhina3Andrey Matveev4Department of Biotechnology and Industrial Pharmacy, Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, Moscow 119454, RussiaDepartment of Biotechnology and Industrial Pharmacy, Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, Moscow 119454, RussiaDepartment of Biotechnology and Industrial Pharmacy, Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, Moscow 119454, RussiaDepartment of Biotechnology and Industrial Pharmacy, Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, Moscow 119454, RussiaDepartment of Biotechnology and Industrial Pharmacy, Lomonosov Institute of Fine Chemical Technologies, MIREA-Russian Technological University, Moscow 119454, RussiaA number of new 5-aminomethyl-1,2,4-triazole-3-carboxamides, demonstrating high model affinity to the IGPD catalytic site comparable with that of the native substrate, were synthesized. The derivatives obtained were tested for antimicrobial potential against <i>M. smegmatis</i>, a species related to <i>M. tuberculosis</i>. During the initial antimicrobial activity evaluation in vitro, some compounds investigated inhibited microbial growth. Moreover, high binding energy values calculated for compounds/enzyme’s catalytic site complexes correlated with the compounds’ antimicrobial efficacy. This suggests that the probable biological action mechanism of new 5-aminomethyl-1,2,4-triazole-3-carboxamides may be based on their binding to the catalytic site of IGPD, which provides prerequisites for further study of this class of compounds as potential IGPD inhibitors.https://www.mdpi.com/2673-4583/16/1/675-aminomethyl-1,2,4-triazole-3-carboxamidesimidazoleglycerol-phosphate dehydrataseIGPD inhibitorsanti-tuberculosis agents
spellingShingle Eugenia Oleynik
Ekaterina Pyankina
Ekaterina Mitina
Ekaterina Mikhina
Andrey Matveev
New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)
Chemistry Proceedings
5-aminomethyl-1,2,4-triazole-3-carboxamides
imidazoleglycerol-phosphate dehydratase
IGPD inhibitors
anti-tuberculosis agents
title New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)
title_full New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)
title_fullStr New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)
title_full_unstemmed New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)
title_short New 1,2,4-Triazole Potential Inhibitors of Mycobacterial Imidazoleglycerol-Phosphate Dehydratase (IGPD)
title_sort new 1 2 4 triazole potential inhibitors of mycobacterial imidazoleglycerol phosphate dehydratase igpd
topic 5-aminomethyl-1,2,4-triazole-3-carboxamides
imidazoleglycerol-phosphate dehydratase
IGPD inhibitors
anti-tuberculosis agents
url https://www.mdpi.com/2673-4583/16/1/67
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