Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies

Lithium metal batteries (LMBs) are promising candidates for electric vehicles (EVs) and next-generation energy storage systems owing to their high energy densities. The solid electrolyte interphase (SEI) on the Li metal anode plays an important role in influencing the Li deposition form and the cycl...

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Main Authors: Gyuri Youk, Jeongmin Kim, Oh B. Chae
Format: Article
Language:English
Published: MDPI AG 2025-01-01
Series:Energies
Subjects:
Online Access:https://www.mdpi.com/1996-1073/18/2/261
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author Gyuri Youk
Jeongmin Kim
Oh B. Chae
author_facet Gyuri Youk
Jeongmin Kim
Oh B. Chae
author_sort Gyuri Youk
collection DOAJ
description Lithium metal batteries (LMBs) are promising candidates for electric vehicles (EVs) and next-generation energy storage systems owing to their high energy densities. The solid electrolyte interphase (SEI) on the Li metal anode plays an important role in influencing the Li deposition form and the cycle life of the LMB. However, the SEI on Li metal differs from that for other anodes, such as graphite, owing to its instability and reactivity. In addition, dendrite growth has hindered the commercial application of Li metal batteries in regular portable electronics to EVs. This review summarizes SEI formation on Li metal, dendrite formation and growth, and their impact on battery performance. In addition, we reviewed the recent progress in pretreatment strategies using materials such as polymers, carbon materials, and inorganic compounds to suppress dendritic growth.
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series Energies
spelling doaj-art-0ae7d1f566044702977924a061a0763b2025-01-24T13:30:49ZengMDPI AGEnergies1996-10732025-01-0118226110.3390/en18020261Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment StrategiesGyuri Youk0Jeongmin Kim1Oh B. Chae2School of Chemical, Biological and Battery Engineering, Gachon University, Seongnam-si 13120, Republic of KoreaSchool of Chemical, Biological and Battery Engineering, Gachon University, Seongnam-si 13120, Republic of KoreaSchool of Chemical, Biological and Battery Engineering, Gachon University, Seongnam-si 13120, Republic of KoreaLithium metal batteries (LMBs) are promising candidates for electric vehicles (EVs) and next-generation energy storage systems owing to their high energy densities. The solid electrolyte interphase (SEI) on the Li metal anode plays an important role in influencing the Li deposition form and the cycle life of the LMB. However, the SEI on Li metal differs from that for other anodes, such as graphite, owing to its instability and reactivity. In addition, dendrite growth has hindered the commercial application of Li metal batteries in regular portable electronics to EVs. This review summarizes SEI formation on Li metal, dendrite formation and growth, and their impact on battery performance. In addition, we reviewed the recent progress in pretreatment strategies using materials such as polymers, carbon materials, and inorganic compounds to suppress dendritic growth.https://www.mdpi.com/1996-1073/18/2/261Li metal anodespretreatment materialssurface pretreatmentartificial SEILMBs
spellingShingle Gyuri Youk
Jeongmin Kim
Oh B. Chae
Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies
Energies
Li metal anodes
pretreatment materials
surface pretreatment
artificial SEI
LMBs
title Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies
title_full Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies
title_fullStr Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies
title_full_unstemmed Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies
title_short Improving Performance and Safety of Lithium Metal Batteries Through Surface Pretreatment Strategies
title_sort improving performance and safety of lithium metal batteries through surface pretreatment strategies
topic Li metal anodes
pretreatment materials
surface pretreatment
artificial SEI
LMBs
url https://www.mdpi.com/1996-1073/18/2/261
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