Accident-tolerant hybrid ceramics for fusion breeding blanket

In a water-cooled ceramic breeding blanket for fusion reactors, hydrogen gas generation by steam oxidation of metallic Be compounds (i.e. neutron multiplier) in a loss-of-coolant accident (LOCA) raises major safety concerns. Li–Be hybrid ceramics has a potential to reduce hydrogen generation signifi...

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Main Authors: Keisuke Mukai, Taehyun Hwang, Minoru Kusaba, Jae-Hwan Kim
Format: Article
Language:English
Published: Elsevier 2025-05-01
Series:Materials & Design
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Online Access:http://www.sciencedirect.com/science/article/pii/S0264127525003843
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author Keisuke Mukai
Taehyun Hwang
Minoru Kusaba
Jae-Hwan Kim
author_facet Keisuke Mukai
Taehyun Hwang
Minoru Kusaba
Jae-Hwan Kim
author_sort Keisuke Mukai
collection DOAJ
description In a water-cooled ceramic breeding blanket for fusion reactors, hydrogen gas generation by steam oxidation of metallic Be compounds (i.e. neutron multiplier) in a loss-of-coolant accident (LOCA) raises major safety concerns. Li–Be hybrid ceramics has a potential to reduce hydrogen generation significantly, however, the stable compositions and structures for quaternary compositions have not been comprehensively understood. Herein, we report machine-learning based prediction, synthesis, structure, and properties of chemically stabile two-phase Li–Be–X–O hybrid ceramics. The steam exposure tests demonstrated a negligibly small H2 generation from the two-phase powder of Li2BeSiO4 and 5 at.% BeO below 1200 °C. The stability is explained by the intrinsic ionic/covalent bonding characters and little capacity for further oxidation by steam. Neutronic calculations with simplified one-dimensional model show that the two-phase hybrid cermaics has a sufficient tritium breeding capability without having metallic Be-based multiplier in the blanket. The hybrid ceramics is the first example of multi-functional oxide to breed sufficient fuel tritium with no metallic neutron multiplier, which allows a novel design of ceramic breeding blanket with enhanced safety margins during in-box LOCA.
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spelling doaj-art-0a0818f129c542c4bb100ae5290329a42025-08-20T03:22:04ZengElsevierMaterials & Design0264-12752025-05-0125311396410.1016/j.matdes.2025.113964Accident-tolerant hybrid ceramics for fusion breeding blanketKeisuke Mukai0Taehyun Hwang1Minoru Kusaba2Jae-Hwan Kim3National Institute for Fusion Science, 322-6 Oroshi-cho, Toki, Gifu 509-5292, Japan; The Institute for Advanced Science, SOKENDAI, Toki 509-5292, Japan; Corresponding author at: National Institute for Fusion Science, 322-6 Oroshi-cho, Toki, Gifu 509-5292, Japan.Fusion Energy Directorate, National Institutes for Quantum Science and Technology, 2-166 Omotedate, Obuchi, Rokkasho, Aomori, 039-3212, JapanNational Institute for Fusion Science, 322-6 Oroshi-cho, Toki, Gifu 509-5292, Japan; The Institute of Statistical Mathematics, Research Organization of Information and Systems, Tachikawa, Tokyo 190-8562, JapanFusion Energy Directorate, National Institutes for Quantum Science and Technology, 2-166 Omotedate, Obuchi, Rokkasho, Aomori, 039-3212, JapanIn a water-cooled ceramic breeding blanket for fusion reactors, hydrogen gas generation by steam oxidation of metallic Be compounds (i.e. neutron multiplier) in a loss-of-coolant accident (LOCA) raises major safety concerns. Li–Be hybrid ceramics has a potential to reduce hydrogen generation significantly, however, the stable compositions and structures for quaternary compositions have not been comprehensively understood. Herein, we report machine-learning based prediction, synthesis, structure, and properties of chemically stabile two-phase Li–Be–X–O hybrid ceramics. The steam exposure tests demonstrated a negligibly small H2 generation from the two-phase powder of Li2BeSiO4 and 5 at.% BeO below 1200 °C. The stability is explained by the intrinsic ionic/covalent bonding characters and little capacity for further oxidation by steam. Neutronic calculations with simplified one-dimensional model show that the two-phase hybrid cermaics has a sufficient tritium breeding capability without having metallic Be-based multiplier in the blanket. The hybrid ceramics is the first example of multi-functional oxide to breed sufficient fuel tritium with no metallic neutron multiplier, which allows a novel design of ceramic breeding blanket with enhanced safety margins during in-box LOCA.http://www.sciencedirect.com/science/article/pii/S0264127525003843Nuclear fusionCeramicsHydrogen generationMachine learningTritium breeding
spellingShingle Keisuke Mukai
Taehyun Hwang
Minoru Kusaba
Jae-Hwan Kim
Accident-tolerant hybrid ceramics for fusion breeding blanket
Materials & Design
Nuclear fusion
Ceramics
Hydrogen generation
Machine learning
Tritium breeding
title Accident-tolerant hybrid ceramics for fusion breeding blanket
title_full Accident-tolerant hybrid ceramics for fusion breeding blanket
title_fullStr Accident-tolerant hybrid ceramics for fusion breeding blanket
title_full_unstemmed Accident-tolerant hybrid ceramics for fusion breeding blanket
title_short Accident-tolerant hybrid ceramics for fusion breeding blanket
title_sort accident tolerant hybrid ceramics for fusion breeding blanket
topic Nuclear fusion
Ceramics
Hydrogen generation
Machine learning
Tritium breeding
url http://www.sciencedirect.com/science/article/pii/S0264127525003843
work_keys_str_mv AT keisukemukai accidenttoleranthybridceramicsforfusionbreedingblanket
AT taehyunhwang accidenttoleranthybridceramicsforfusionbreedingblanket
AT minorukusaba accidenttoleranthybridceramicsforfusionbreedingblanket
AT jaehwankim accidenttoleranthybridceramicsforfusionbreedingblanket