A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing

Abstract The rising flexible and intelligent electronics greatly facilitate the noninvasive and timely tracking of physiological information in telemedicine healthcare. Meticulously building bionic-sensitive moieties is vital for designing efficient electronic skin with advanced cognitive functional...

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Main Authors: Qingqing Zhou, Qihang Ding, Zixun Geng, Chencheng Hu, Long Yang, Zitong Kan, Biao Dong, Miae Won, Hongwei Song, Lin Xu, Jong Seung Kim
Format: Article
Language:English
Published: SpringerOpen 2024-10-01
Series:Nano-Micro Letters
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Online Access:https://doi.org/10.1007/s40820-024-01548-5
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author Qingqing Zhou
Qihang Ding
Zixun Geng
Chencheng Hu
Long Yang
Zitong Kan
Biao Dong
Miae Won
Hongwei Song
Lin Xu
Jong Seung Kim
author_facet Qingqing Zhou
Qihang Ding
Zixun Geng
Chencheng Hu
Long Yang
Zitong Kan
Biao Dong
Miae Won
Hongwei Song
Lin Xu
Jong Seung Kim
author_sort Qingqing Zhou
collection DOAJ
description Abstract The rising flexible and intelligent electronics greatly facilitate the noninvasive and timely tracking of physiological information in telemedicine healthcare. Meticulously building bionic-sensitive moieties is vital for designing efficient electronic skin with advanced cognitive functionalities to pluralistically capture external stimuli. However, realistic mimesis, both in the skin’s three-dimensional interlocked hierarchical structures and synchronous encoding multistimuli information capacities, remains a challenging yet vital need for simplifying the design of flexible logic circuits. Herein, we construct an artificial epidermal device by in situ growing Cu3(HHTP)2 particles onto the hollow spherical Ti3C2T x surface, aiming to concurrently emulate the spinous and granular layers of the skin’s epidermis. The bionic Ti3C2T x @Cu3(HHTP)2 exhibits independent NO2 and pressure response, as well as novel functionalities such as acoustic signature perception and Morse code-encrypted message communication. Ultimately, a wearable alarming system with a mobile application terminal is self-developed by integrating the bimodular senor into flexible printed circuits. This system can assess risk factors related with asthmatic, such as stimulation of external NO2 gas, abnormal expiratory behavior and exertion degrees of fingers, achieving a recognition accuracy of 97.6% as assisted by a machine learning algorithm. Our work provides a feasible routine to develop intelligent multifunctional healthcare equipment for burgeoning transformative telemedicine diagnosis.
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spelling doaj-art-08e8ccc592aa4d71aa1e4804a2bb60c82025-08-20T04:02:55ZengSpringerOpenNano-Micro Letters2311-67062150-55512024-10-0117112010.1007/s40820-024-01548-5A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure SensingQingqing Zhou0Qihang Ding1Zixun Geng2Chencheng Hu3Long Yang4Zitong Kan5Biao Dong6Miae Won7Hongwei Song8Lin Xu9Jong Seung Kim10State Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityDepartment of Chemistry, Korea UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityDepartment of Chemistry, Korea UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityState Key Laboratory of Integrated Optoelectronics, College of Electronic Science and Engineering, Jilin UniversityDepartment of Chemistry, Korea UniversityAbstract The rising flexible and intelligent electronics greatly facilitate the noninvasive and timely tracking of physiological information in telemedicine healthcare. Meticulously building bionic-sensitive moieties is vital for designing efficient electronic skin with advanced cognitive functionalities to pluralistically capture external stimuli. However, realistic mimesis, both in the skin’s three-dimensional interlocked hierarchical structures and synchronous encoding multistimuli information capacities, remains a challenging yet vital need for simplifying the design of flexible logic circuits. Herein, we construct an artificial epidermal device by in situ growing Cu3(HHTP)2 particles onto the hollow spherical Ti3C2T x surface, aiming to concurrently emulate the spinous and granular layers of the skin’s epidermis. The bionic Ti3C2T x @Cu3(HHTP)2 exhibits independent NO2 and pressure response, as well as novel functionalities such as acoustic signature perception and Morse code-encrypted message communication. Ultimately, a wearable alarming system with a mobile application terminal is self-developed by integrating the bimodular senor into flexible printed circuits. This system can assess risk factors related with asthmatic, such as stimulation of external NO2 gas, abnormal expiratory behavior and exertion degrees of fingers, achieving a recognition accuracy of 97.6% as assisted by a machine learning algorithm. Our work provides a feasible routine to develop intelligent multifunctional healthcare equipment for burgeoning transformative telemedicine diagnosis.https://doi.org/10.1007/s40820-024-01548-5Ti3C2T x @Cu3(HHTP)2 compositesNO2/pressure flexible sensorsHealth-monitoringMachine learning
spellingShingle Qingqing Zhou
Qihang Ding
Zixun Geng
Chencheng Hu
Long Yang
Zitong Kan
Biao Dong
Miae Won
Hongwei Song
Lin Xu
Jong Seung Kim
A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing
Nano-Micro Letters
Ti3C2T x @Cu3(HHTP)2 composites
NO2/pressure flexible sensors
Health-monitoring
Machine learning
title A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing
title_full A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing
title_fullStr A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing
title_full_unstemmed A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing
title_short A Flexible Smart Healthcare Platform Conjugated with Artificial Epidermis Assembled by Three-Dimensionally Conductive MOF Network for Gas and Pressure Sensing
title_sort flexible smart healthcare platform conjugated with artificial epidermis assembled by three dimensionally conductive mof network for gas and pressure sensing
topic Ti3C2T x @Cu3(HHTP)2 composites
NO2/pressure flexible sensors
Health-monitoring
Machine learning
url https://doi.org/10.1007/s40820-024-01548-5
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