Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters

Poly(ethylene terephthalate) (PET) which is one of the most commercially important polymers, has for many years been an interesting candidate for the production of high performance fibres and tapes. In current study, we focus on investigating the effects of the various processing variables on the me...

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Main Authors: Jian Min Zhang, Qingsong Hua, Christopher T. Reynolds, Yuling Zhao, Zuoqiang Dai, Emiliano Bilotti, Jie Tang, Ton Peijs
Format: Article
Language:English
Published: Wiley 2017-01-01
Series:International Journal of Polymer Science
Online Access:http://dx.doi.org/10.1155/2017/2781425
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author Jian Min Zhang
Qingsong Hua
Christopher T. Reynolds
Yuling Zhao
Zuoqiang Dai
Emiliano Bilotti
Jie Tang
Ton Peijs
author_facet Jian Min Zhang
Qingsong Hua
Christopher T. Reynolds
Yuling Zhao
Zuoqiang Dai
Emiliano Bilotti
Jie Tang
Ton Peijs
author_sort Jian Min Zhang
collection DOAJ
description Poly(ethylene terephthalate) (PET) which is one of the most commercially important polymers, has for many years been an interesting candidate for the production of high performance fibres and tapes. In current study, we focus on investigating the effects of the various processing variables on the mechanical properties of PET produced by a distinctive process of melt spinning and uniaxial two-stage solid-state drawing (SSD). These processing variables include screw rotation speed during extrusion, fibre take-up speed, molecular weight, draw-ratio, and drawing temperature. As-spun PET production using a single-screw extrusion process was first optimized to induce an optimal polymer microstructure for subsequent drawing processes. It was found that less crystallization which occurred during this process would lead to better drawability, higher draw-ratio, and mechanical properties in the subsequent SSD process. Then the effect of drawing temperature (DT) in uniaxial two-stage SSD process was studied to understand how DT (<Tg or close to Tg or close to Trec) would affect the crystallization, draw-ratio, and final mechanical properties of PET. The designed process in current work is simulated to an industrial production process for PET fibres; therefore, results and analysis in this paper have significant importance for industrial production.
format Article
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institution Kabale University
issn 1687-9422
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language English
publishDate 2017-01-01
publisher Wiley
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series International Journal of Polymer Science
spelling doaj-art-070eb21764844f878e783e6de93e7ef02025-08-20T03:55:24ZengWileyInternational Journal of Polymer Science1687-94221687-94302017-01-01201710.1155/2017/27814252781425Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing ParametersJian Min Zhang0Qingsong Hua1Christopher T. Reynolds2Yuling Zhao3Zuoqiang Dai4Emiliano Bilotti5Jie Tang6Ton Peijs7School of Mechanical and Electrical Engineering, Qingdao University and Power & Energy Storage System Research Center, No. 308 Ningxia Road, Qingdao 266071, ChinaSchool of Mechanical and Electrical Engineering, Qingdao University and Power & Energy Storage System Research Center, No. 308 Ningxia Road, Qingdao 266071, ChinaSchool of Engineering and Materials Science and Materials Research Institute, Queen Mary University of London, Mile End Road, London E1 4NS, UKSchool of Mechanical and Electrical Engineering, Qingdao University and Power & Energy Storage System Research Center, No. 308 Ningxia Road, Qingdao 266071, ChinaSchool of Mechanical and Electrical Engineering, Qingdao University and Power & Energy Storage System Research Center, No. 308 Ningxia Road, Qingdao 266071, ChinaSchool of Engineering and Materials Science and Materials Research Institute, Queen Mary University of London, Mile End Road, London E1 4NS, UKSchool of Mechanical and Electrical Engineering, Qingdao University and Power & Energy Storage System Research Center, No. 308 Ningxia Road, Qingdao 266071, ChinaSchool of Engineering and Materials Science and Materials Research Institute, Queen Mary University of London, Mile End Road, London E1 4NS, UKPoly(ethylene terephthalate) (PET) which is one of the most commercially important polymers, has for many years been an interesting candidate for the production of high performance fibres and tapes. In current study, we focus on investigating the effects of the various processing variables on the mechanical properties of PET produced by a distinctive process of melt spinning and uniaxial two-stage solid-state drawing (SSD). These processing variables include screw rotation speed during extrusion, fibre take-up speed, molecular weight, draw-ratio, and drawing temperature. As-spun PET production using a single-screw extrusion process was first optimized to induce an optimal polymer microstructure for subsequent drawing processes. It was found that less crystallization which occurred during this process would lead to better drawability, higher draw-ratio, and mechanical properties in the subsequent SSD process. Then the effect of drawing temperature (DT) in uniaxial two-stage SSD process was studied to understand how DT (<Tg or close to Tg or close to Trec) would affect the crystallization, draw-ratio, and final mechanical properties of PET. The designed process in current work is simulated to an industrial production process for PET fibres; therefore, results and analysis in this paper have significant importance for industrial production.http://dx.doi.org/10.1155/2017/2781425
spellingShingle Jian Min Zhang
Qingsong Hua
Christopher T. Reynolds
Yuling Zhao
Zuoqiang Dai
Emiliano Bilotti
Jie Tang
Ton Peijs
Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters
International Journal of Polymer Science
title Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters
title_full Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters
title_fullStr Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters
title_full_unstemmed Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters
title_short Preparation of High Modulus Poly(Ethylene Terephthalate): Influence of Molecular Weight, Extrusion, and Drawing Parameters
title_sort preparation of high modulus poly ethylene terephthalate influence of molecular weight extrusion and drawing parameters
url http://dx.doi.org/10.1155/2017/2781425
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