Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting

In the development of static luminescent materials with remarkable optical-thermal performance and low cost, next-generation high-brightness laser lighting faces a key challenge. Herein, a unique composite architecture of Y3Al5O12:Ce3+ (YAG) phosphor-in-glass film coated on different heat-conducting...

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Main Authors: Xin Liu, Mingxiang Chen, Jiuzhou Zhao, Hongjin Zhang, Yang Peng, Qing Wang
Format: Article
Language:English
Published: Tsinghua University Press 2025-02-01
Series:Journal of Advanced Ceramics
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Online Access:https://www.sciopen.com/article/10.26599/JAC.2024.9221027
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author Xin Liu
Mingxiang Chen
Jiuzhou Zhao
Hongjin Zhang
Yang Peng
Qing Wang
author_facet Xin Liu
Mingxiang Chen
Jiuzhou Zhao
Hongjin Zhang
Yang Peng
Qing Wang
author_sort Xin Liu
collection DOAJ
description In the development of static luminescent materials with remarkable optical-thermal performance and low cost, next-generation high-brightness laser lighting faces a key challenge. Herein, a unique composite architecture of Y3Al5O12:Ce3+ (YAG) phosphor-in-glass film coated on different heat-conducting substrates (PiGF@HCSs), i.e., PiGF@sapphire, PiGF@Al2O3, PiGF@AlN, and PiGF@BN–AlN composites, was designed and prepared by a simple film printing and low-temperature sintering technology. The heat-conducting substrates significantly affect the luminescence saturation and phosphor conversion of PiGF@HCSs, allowing substrates with higher thermal conductivity (TC) to have a higher laser power density (LPD) and higher reflectivity to enable higher luminous efficacy (LE). As a consequence, PiGF@sapphire realizes a luminous flux (LF) of 2076 lm@12 W/mm2, which is higher than those of PiGF@Al2O3 (1890 lm@15 W/mm2) and PiGF@AlN (1915 lm@24 W/mm2), whilePiGF@BN–AlN enables a maximum LF of 3058 lm@21 W/mm2. Furthermore, the LE of PiGF@BN–AlN reaches 194 lm/W, which is 1.6 times that of PiGF@AlN, while those of PiGF@sapphire and PiGF@Al2O3 are 192 and 150 lm/W, respectively. The working temperature of PiGF@AlN is only 93.3 °C under LPD of 9 W/mm2, while those of PiGF@sapphire, PiGF@Al2O3, and PiGF@BN–AlN increase to 193.8, 133.6, and 117 °C, respectively. These findings provide guidance for commercial applications of PiGF@HCS converters in high-brightness laser lighting and displays.
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institution DOAJ
issn 2226-4108
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language English
publishDate 2025-02-01
publisher Tsinghua University Press
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series Journal of Advanced Ceramics
spelling doaj-art-070bb44cc99a4a8ea7ef3164e7e812a32025-08-20T02:47:49ZengTsinghua University PressJournal of Advanced Ceramics2226-41082227-85082025-02-01142922102710.26599/JAC.2024.9221027Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lightingXin Liu0Mingxiang Chen1Jiuzhou Zhao2Hongjin Zhang3Yang Peng4Qing Wang5State Key Laboratory of Intelligent Manufacturing Equipment and Technology, School of Mechanical Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaState Key Laboratory of Intelligent Manufacturing Equipment and Technology, School of Mechanical Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaSchool of Aerospace Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaSchool of Aerospace Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaSchool of Aerospace Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaSchool of Energy and Power Engineering, Huazhong University of Science and Technology, Wuhan 430074, ChinaIn the development of static luminescent materials with remarkable optical-thermal performance and low cost, next-generation high-brightness laser lighting faces a key challenge. Herein, a unique composite architecture of Y3Al5O12:Ce3+ (YAG) phosphor-in-glass film coated on different heat-conducting substrates (PiGF@HCSs), i.e., PiGF@sapphire, PiGF@Al2O3, PiGF@AlN, and PiGF@BN–AlN composites, was designed and prepared by a simple film printing and low-temperature sintering technology. The heat-conducting substrates significantly affect the luminescence saturation and phosphor conversion of PiGF@HCSs, allowing substrates with higher thermal conductivity (TC) to have a higher laser power density (LPD) and higher reflectivity to enable higher luminous efficacy (LE). As a consequence, PiGF@sapphire realizes a luminous flux (LF) of 2076 lm@12 W/mm2, which is higher than those of PiGF@Al2O3 (1890 lm@15 W/mm2) and PiGF@AlN (1915 lm@24 W/mm2), whilePiGF@BN–AlN enables a maximum LF of 3058 lm@21 W/mm2. Furthermore, the LE of PiGF@BN–AlN reaches 194 lm/W, which is 1.6 times that of PiGF@AlN, while those of PiGF@sapphire and PiGF@Al2O3 are 192 and 150 lm/W, respectively. The working temperature of PiGF@AlN is only 93.3 °C under LPD of 9 W/mm2, while those of PiGF@sapphire, PiGF@Al2O3, and PiGF@BN–AlN increase to 193.8, 133.6, and 117 °C, respectively. These findings provide guidance for commercial applications of PiGF@HCS converters in high-brightness laser lighting and displays.https://www.sciopen.com/article/10.26599/JAC.2024.9221027luminescent materialsphosphor-in-glass film (pigf)heat-conducting substrate (hcs)laser lightingoptical–thermal performances
spellingShingle Xin Liu
Mingxiang Chen
Jiuzhou Zhao
Hongjin Zhang
Yang Peng
Qing Wang
Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting
Journal of Advanced Ceramics
luminescent materials
phosphor-in-glass film (pigf)
heat-conducting substrate (hcs)
laser lighting
optical–thermal performances
title Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting
title_full Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting
title_fullStr Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting
title_full_unstemmed Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting
title_short Unique composite architecture of phosphor-in-glass film coated on different heat-conducting substrates for high-brightness laser lighting
title_sort unique composite architecture of phosphor in glass film coated on different heat conducting substrates for high brightness laser lighting
topic luminescent materials
phosphor-in-glass film (pigf)
heat-conducting substrate (hcs)
laser lighting
optical–thermal performances
url https://www.sciopen.com/article/10.26599/JAC.2024.9221027
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